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Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

Preparation of nonclassical light with special quantum properties is essential for quantum technologies. High-harmonic generation (HHG) is a process which not only enables the creation of attosecond pulses but also has the potential to…

Quantum Physics · Physics 2026-03-03 Ákos Gombkötő , Péter Ádám , David Theidel , Tamás Kiss

We theoretically study THz-light-driven high-harmonic generation (HHG) in the spin-liquid states of the Kitaev honeycomb model with a magnetostriction coupling between spin and electric polarization. To compute the HHG spectra, we…

Strongly Correlated Electrons · Physics 2021-08-04 Minoru Kanega , Tatsuhiko N. Ikeda , Masahiro Sato

We study theoretically and experimentally High Harmonic Generation (HHG) using two non collinear driving fields focused in gases. We show that these two fields form a non stationary blazed active grating in the generation medium. The…

Optics · Physics 2019-03-13 C. Chappuis , D. Bresteau , T. Auguste , O. Gobert , T. Ruchon

The emission of above-ionization-threshold harmonics results from the recombination of two electron wavepackets moving along a "short" and a "long" trajectory in the atomic continuum. Attosecond pulse train generation has so far been…

Optics · Physics 2015-05-19 J. E. Kruse , P. Tzallas , E. Skantzakis , D. Charalambidis

High-harmonic generation - the emission of high-frequency radiation by the ionization and subsequent recombination of an atomic electron driven by a strong laser field - is widely understood using a quasiclassical trajectory formalism,…

Quantum Physics · Physics 2020-07-29 Emilio Pisanty , Marcelo F. Ciappina , Maciej Lewenstein

We calculate high-harmonic generation (HHG) by intense infrared lasers in atoms and molecules with the inclusion of macroscopic propagation of the harmonics in the gas medium. We show that the observed experimental spectra can be accurately…

We investigate, by solving the time-dependent Schr\"{o}dinger equation in the single-active-electron approximation in helium, a two-color scheme for tabletop high-order harmonic generation (HHG) that combines a mid-infrared (MIR) driving…

We study numerically the Bloch electron wave-packet dynamics in periodic potentials to simulate laser-solid interactions. We introduce a quasi-classical model in the \emph{k} space combined with the energy band structure to understand the…

Optics · Physics 2017-01-05 Tao-Yuan Du , Xue-Bin Bian

The generation of high harmonics in laser-irradiated light homonuclear diatomics (H2+, N2 and O2) compared to that in atomic counterparts (of nearly identical binding energy) is studied within the velocity gauge version of conventional…

Atomic Physics · Physics 2009-11-11 Vladimir I. Usachenko , Pavel E. Pyak , Shih-I Chu

We review the main research directions ongoing in the development of high-harmonic generation-based extreme ultraviolet sources for the synthesization and application of trains and isolated attosecond pulses to time-resolved spectroscopy. A…

Using time-dependent density functional theory, high-harmonic generation (HHG) is studied in one-dimensional structures of sizes from a single nucleus up to hundreds of nuclei. The HHG cutoff is observed to extent linearly with the system…

Atomic Physics · Physics 2018-04-27 Kenneth K. Hansen , Dieter Bauer , Lars Bojer Madsen

With the high-order harmonic generation (HHG) from plasma sur- faces it is possible to turn a laser pulse into a train of attosecond or even zeptosecond pulses in the backward radiation. These attosecond pulses may have amplitude several…

Plasma Physics · Physics 2016-11-03 Mykyta Cherednychek , Alexander Pukhov

The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…

Atomic Physics · Physics 2016-04-27 M. A. Khokhlova , V. V. Strelkov

Direct imaging of molecular dynamics is a long-standing goal in physics and chemistry. As an emerging tool, high-harmonic spectroscopy (HHS) enables accessing molecular dynamics on femtosecond to attosecond time scales. However, decoding…

Recent advances in attosecond science have made it increasingly important to develop stable, reliable and accurate algorithms and methods to model the time evolution of atoms and molecules in intense laser fields. A key process in…

Chemical Physics · Physics 2024-08-19 Simon Elias Schrader , Håkon Emil Kristiansen , Thomas Bondo Pedersen , Simen Kvaal

Solid-state high-order harmonic generation (HHG) presents unique features different from gases.Whereas the gaseous harmonics driven by counter-rotating bicircular (CRB) pulse universally peak at a "magic" field ratio approximately…

Optics · Physics 2025-07-15 Qing-Guo Fan , Kang Lai , Wen-hao Liu , Zhi Wang , Lin-Wang Wang , Jun-Wei Luo

High-order harmonic generation (HHG) in simultaneous intense near-infrared (NIR) laser light and brilliant x rays above an inner-shell absorption edge is examined. A tightly bound inner-shell electron is transferred into the continuum.…

High-harmonic generation (HHG), the hallmark effect of attosecond science, is a nonperturbative nonlinear process leading to the emission of high-harmonic light from gases and solids. In gases, extreme driving laser pulse intensities can…

We present the first theoretical results on the generation of short-wavelength attosecond vortex beams in semiconductors through their interactions with an intense Laguerre-Gauss beam, in the limit where non-perturbative high-order…

Atomic Physics · Physics 2024-10-21 C. Granados , B. Kumar Das , Christian Heide , Shambhu Ghimire , M. F. Ciappina