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We use molecular dynamics (MD) simulations to study surface-directed spinodal decomposition (SDSD) in unstable binary ($AB$) fluid mixtures at wetting surfaces. The thickness of the wetting layer $R_1$ grows with time $t$ as a power-law…

Soft Condensed Matter · Physics 2012-04-04 Prabhat K. Jaiswal , Sanjay Puri , Subir K. Das

We present results from the molecular dynamics (MD) simulation of surface-directed spinodal decomposition (SDSD) in binary fluid mixtures ($A+B$) with off-critical compositions. The aim is to elucidate the role of composition ratio in the…

Soft Condensed Matter · Physics 2024-08-19 Syed Shuja Hasan Zaidi , Saumya Suvarna , Madhu Priya , Sanjay Puri , Prabhat K. Jaiswal

We employ a molecular dynamics (MD) study to explore pattern selection in binary fluid mixtures ($AB$) undergoing surface-directed spinodal decomposition on a chemically patterned amorphous substrate. We chose a checkerboard pattern with…

Soft Condensed Matter · Physics 2025-12-12 Syed Shuja Hasan Zaidi , Hema Teherpuria , Santosh Mogurampelly , Prabhat K. Jaiswal

We present comprehensive molecular dynamics (MD) results for the kinetics of surface-directed spinodal decomposition (SDSD) and surface enrichment (SE) in binary mixtures at wetting surfaces. We study the surface morphology and the growth…

Soft Condensed Matter · Physics 2010-11-30 Prabhat K. Jaiswal , Sanjay Puri , Subir K. Das

We use molecular dynamics (MD) to simulate an unstable homogeneous mixture of binary fluids (AB), confined in a slit pore of width $D$. The pore walls are assumed to be flat and structureless, and attract one component of the mixture (A)…

Disordered Systems and Neural Networks · Physics 2009-11-11 S. K. Das , S. Puri Jawaharlal , J. Horbach , Kurt Binder

The surface directed spinodal decomposition of a binary liquid confined inside cylindrical pore is investigated using molecular dynamics simulation. One component of the liquid wets the pore surface while the other remains neutral. A…

Soft Condensed Matter · Physics 2023-09-19 Daniya Davis , Bhaskar Sen Gupta

This paper is the second in a two-part exposition on {\it surface-directed spinodal decomposition} (SDSD), i.e., the interplay of kinetics of wetting and phase separation at a surface which is wetted by one of the components of a binary…

Statistical Mechanics · Physics 2020-08-25 Prasenjit Das , Prabhat K. Jaiswal , Sanjay Puri

In our previous work [J. Chem. Phys. \textbf{136}, 024502 (2012)], we reported a demixing phase transition of a two-dimensional, binary Heisenberg fluid mixture driven by the ferromagnetic interactions of the magnetic species. Here, we…

Soft Condensed Matter · Physics 2015-06-16 Ken Lichtner , Sabine H. L. Klapp

We study the diffusion-driven kinetics of phase separation of a symmetric binary mixture (AB), confined in a thin-film geometry between two parallel walls. We consider cases where (a) both walls preferentially attract the same component…

Soft Condensed Matter · Physics 2009-11-11 Subir K. Das , Sanjay Puri , Juergen Horbach , Kurt Binder

We present simulation results from a comprehensive molecular dynamics (MD) study of surface-directed spinodal decomposition (SDSD) in unstable symmetric binary mixtures at wetting surfaces. We consider long-ranged and short-ranged surface…

Soft Condensed Matter · Physics 2022-06-27 Syed Shuja Hasan Zaidi , Prabhat K. Jaiswal , Madhu Priya , Sanjay Puri

By performing lattice Boltzmann simulations of a binary mixture, we scrutinize the dynamical scaling hypothesis for the spinodal decomposition of binary mixtures for the crossover region, i.e. the region of parameters in the growth curve…

Soft Condensed Matter · Physics 2007-05-23 Ignacio Pagonabarraga , Alexander J. Wagner , M. E. Cates

We consider the phase separation of binary fluids in contact with a surface which is preferentially wetted by one of the components of the mixture. We review the results available for this problem and present new numerical results obtained…

Statistical Mechanics · Physics 2007-05-23 Sorin Bastea , Sanjay Puri , Joel L. Lebowitz

The surface phase behavior of binary mixtures of colloidal hard rods in contact with a solid substrate (hard wall) is studied, with special emphasis on the region of the phase diagram that includes the smectic A phase. The colloidal rods…

Soft Condensed Matter · Physics 2010-12-17 Daniel de las Heras , Yuri Martínez-Ratón , Enrique Velasco

{\it Surface-directed spinodal decomposition} (SDSD) is the kinetic interplay of phase separation and wetting at a surface. This process is of great scientific and technological importance. In this paper, we report results from a numerical…

Soft Condensed Matter · Physics 2020-07-20 Prasenjit Das , Prabhat K. Jaiswal , Sanjay Puri

Density functional theory is used to study binary colloidal fluids consisting of hard spheres and thin platelets in their bulk and near a planar hard wall. This system exhibits liquid-liquid coexistence of a phase that is rich in spheres…

Soft Condensed Matter · Physics 2009-11-10 L. Harnau , S. Dietrich

Using large-scale molecular dynamics simulations of a two-component Lennard-Jones model in three dimensions, we show that the late-time dynamics of spinodal decomposition in concentrated binary fluids reaches a viscous scaling regime with a…

Condensed Matter · Physics 2009-10-28 Mohamed Laradji , Soeren Toxvaerd , Ole G. Mouritsen

We study the wetting behaviour of a symmetrical binary fluid below the demixing temperature at a non-selective attractive wall. Although it demixes in the bulk, a sufficiently thin liquid film remains mixed. On approaching liquid/vapour…

Statistical Mechanics · Physics 2009-10-31 F. Schmid , N. B. Wilding

We have used mesoscale simulations to study the effect of immobile particles on microstructure formation during spinodal decomposition in ternary mixtures such as polymer blends. Specifically, we have explored a regime of interparticle…

Materials Science · Physics 2017-06-12 Supriyo Ghosh , Arnab Mukherjee , T. A. Abinandanan , Suryasarathi Bose

We carried out three-dimensional simulations, with about 1.4 million particles, of phase segregation in a low density binary fluid mixture, described mesoscopically by energy and momentum conserving Boltzmann-Vlasov equations. Using a…

patt-sol · Physics 2008-02-03 S. Bastea , J. L. Lebowitz

Results are presented for the phase separation process of a binary mixture subject to an uniform shear flow quenched from a disordered to a homogeneous ordered phase. The kinetics of the process is described in the context of the…

Condensed Matter · Physics 2012-04-05 F. Corberi , G. Gonnella , A. Lamura
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