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Nonlinear optical (NLO) phenomena such as harmonic generation, Kerr, and Pockels effects are of great technological importance for lasers, frequency converters, modulators, switches, etc. Recently, two-dimensional (2D) materials have drawn…

The response functions of a material characterize its behavior under external stimuli, such as electromagnetic radiation. Such responses may grow linearly with the amplitude of the incident radiation, as is the case of absorption, or may be…

Mesoscale and Nanoscale Physics · Physics 2019-08-07 Liang Z. Tan , Andrew M. Rappe

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu

Nonlinear optical frequency conversion, where optical fields interact with a nonlinear medium to generate new frequencies, is a key phenomenon in modern photonic systems. However, a major challenge with these techniques lies in the…

Materials Science · Physics 2024-12-05 Simone Grillo , Elena Cannuccia , Maurizia Palummo , Olivia Pulci , Claudio Attaccalite

We report about the experimental observation and characterization of nonlinear optical properties of individual silicon nanowires of different dimensions. Our results show that the nonlinear light has different components, one of them…

Mesoscale and Nanoscale Physics · Physics 2017-04-13 Peter R. Wiecha , Arnaud Arbouet , Houssem Kallel , Priyanka Periwal , Thierry Baron , Vincent Paillard

Second harmonic generation (SHG) is a coherent nonlinear phenomenon that plays an important role in laser color conversion. Lithium niobate (LN), which features both a large band gap and outstanding second-order nonlinearities, acts as an…

The recent, rapid advances in nonlinear chipscale nanophotonics in the visible and near-infrared have been largely driven by manipulating the local dielectric environment proximate to decades-old workhorse bulk nonlinear optical materials,…

Nonlinear optical microscopy such as in the optical second-harmonic generation (SHG) modality has become a popular tool today for probing materials in the physical and biological sciences. While imaging and spectroscopy are widely used in…

Optical coating, an integral part of many optical systems, is prone to damage from environmental exposure and laser irradiation. This underscores the need for reliable and sensitive coating diagnostics. We introduce second harmonic…

The second-order nonlinear optical susceptibility ($\chi_{abc}^{(2)}$) and linear electro-optical coefficient ($r_{abc}$) of a large number of single-walled zigzag, armchair and chiral SiC nanotubes (SiC-NTs) as well as bulk SiC polytypes…

Materials Science · Physics 2009-11-13 I. J. Wu , G. Y. Guo

All-optical signal processing based on nonlinear optical devices is promising for ultrafast information processing in optical communication systems. Recent advances in two-dimensional (2D) layered materials with unique structures and…

Optics · Physics 2024-03-07 David J. Moss

Nonlinear optical (NLO) materials for generating lasers via second harmonic generation (SHG) are highly sought in today's technology. However, discovering novel materials with considerable SHG is challenging due to the time-consuming and…

Materials Science · Physics 2025-04-29 Yomn Alkabakibi , Congwei Xie , Artem R. Oganov

Due to their abundant use in all-solid-state lasers, nonlinear optical (NLO) crystals are needed for many applications across diverse fields such as medicine and communication. However, because of conflicting requirements, the design of…

Materials Science · Physics 2025-08-13 Victor Trinquet , Matthew L. Evans , Gian-Marco Rignanese

Optical second harmonic generation (SHG) is a nonlinear optical effect widely used for nonlinear optical microscopy and laser frequency conversion. Closed-form analytical solution of the nonlinear optical responses is essential for…

This research will examine the computational methods to calculate the nonlinear optical process of second harmonic generation (SHG) that will be hypothesized to be present during lithium ion insertion into silicon nanowires. First it will…

Optics · Physics 2021-10-19 Donald C. Boone

Optical spectroscopy based on second-order nonlinearity is a critical technique for characterizing two-dimensional (2D) crystals as well as bioimaging and quantum optics. It is generally believed that second-harmonic generation (SHG) in…

Mesoscale and Nanoscale Physics · Physics 2026-01-14 Haoning Tang , Zhitong Ding , Tianyi Ruan , Zeyu Hao , Kenji Watanabe , Takashi Taniguchi , Haozhe Wang , Ali Javey , Feng Wang , Yuan Cao

Two-dimensional (2D) materials with large band gaps and strong and tunable second-harmonic generation (SHG) coefficients play an important role in the miniaturization of deep-ultraviolet (DUV) nonlinear optical (NLO) devices. Despite the…

Mesoscale and Nanoscale Physics · Physics 2025-03-04 Linlin Liu , Congwei Xie , Abudukadi Tudi , Keith Butler , Zhihua Yang

The random laser action with coherent feedback by second-harmonic generation (SHG) was experimentally demonstrated in this paper. Compared with the conventional random laser action based on photoluminescence effect, which needs strong…

Optics · Physics 2016-11-24 Yanqi Qiao , Yuanlin Zheng , Zengyan Cai , Xianfeng Chen

Diffractive neural networks (DNNs) are an emerging approach for the realization of photonic artificial intelligence, especially due to their suitability for machine-vision applications and high-dimensional photonic information processing at…

Optics · Physics 2026-03-27 Marie Braasch , Anna Kartashova , Elena Goi , Thomas Pertsch , Sina Saravi
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