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A coherent superposition of many nuclear spin states can be prepared and manipulated via the hyperfine interaction with the electronic spins by varying the Landau level filling factor through the gate voltage in appropriately designed…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 T. Maniv , Yu. A. Bychkov , I. D. Vagner

The loss of information about the relative phase between two quantum states, known as decoherence, strongly limits resolution in electron paramagnetic spectroscopy and hampers the use of molecules for quantum information processing. At low…

Quantum Physics · Physics 2025-04-28 Conor Ryan , Valerio Briganti , Cathal Hogan , Mark O'Neill , Alessandro Lunghi

We report the existence of a sizeable quantum tunnelling splitting between the two lowest electronic spin levels of mononuclear Ni complexes. The level anti-crossing, or magnetic clock transition, associated with this gap has been directly…

We study the mechanism of dynamical nuclear spin polarization by hyperfine interaction in spin-blocked double quantum dot system. We calculate the hyperfine transition rates and solve the master equations for the nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Changxue Deng , Xuedong Hu

Theoretical model of the nuclear spin conversion in formaldehyde (H2CO) has been developed. The conversion is governed by the intramolecular spin-rotation mixing of molecular ortho and para states. The rate of conversion has been found…

Chemical Physics · Physics 2009-11-06 Pavel L. Chapovsky

The main source of decoherence for an electron spin confined to a quantum dot is the hyperfine interaction with nuclear spins. To analyze this process theoretically we diagonalize the central spin Hamiltonian in the high magnetic B-field…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 Oleksandr Tsyplyatyev , Daniel Loss

At room temperature, the normal oxide spinels NiCr_2O_4 and CuCr_2O_4 are tetragonally distorted and crystallize in the I4_1/amd space group due to cooperative Jahn-Teller ordering driven by the orbital degeneracy of tetrahedral Ni$^{2+}$…

Materials Science · Physics 2012-09-11 Matthew R. Suchomel , Daniel P. Shoemaker , Lynn Ribaud , Moureen C. Kemei , Ram Seshadri

We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh

Signature effects observed in rotational bands are a consequence of an inherent D2-symmetry. This symmetry is naturally broken by the mean field cranking approximation when a tilted (non-principal) axis orientation of the nuclear spin…

Nuclear Theory · Physics 2009-10-31 F. Dönau , Jing-ye Zhang , L. L. Riedinger

A theoretical study of spin dynamics in non-relativistic particle beams with interacting angular momenta traversing static, spatially varying magnetic fields is presented. The computational framework evaluates sinusoidal magnetic field…

The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature…

Mesoscale and Nanoscale Physics · Physics 2009-07-21 P. Maletinsky , M. Kroner , A. Imamoglu

We present a complete analysis of the angular momentum selection rules and electromagnetic backgrounds that constrain any spectroscopic search for the gravitomagnetic spin-quadrupole coupling in highly charged ions. A sequence of four…

Quantum Physics · Physics 2026-04-23 Leonardo A. Pachon

A theoretical model of hyperfine spectra of nuclear spin conversion of molecular isomers has been developed. The model takes into account the nuclear spin-spin and spin-rotation interactions, as well as the saturation of intramolecular…

Chemical Physics · Physics 2009-11-06 Pavel L. Chapovsky

Nuclear spins and paramagnetic centers in a solid randomly group to form clusters featuring nearly-degenerate, hybrid states whose dynamics are central to processes involving nuclear spin-lattice relaxation and diffusion. Their…

Using first-principles calculations, we show that the magnetic properties of a two-dimensional antiferromagnetic transition-metal surface are modified on the atomic scale by the adsorption of small organic molecules. We consider benzene…

Materials Science · Physics 2015-06-16 Nuala M. Caffrey , Paolo Ferriani , Simone Marocchi , Stefan Heinze

We study theoretically the formation of the nuclear-spin polaron state in semiconductor nanosystems within the Lindblad equation approach. To this end, we derive a general Lindblad equation for the density operator that complies with the…

Mesoscale and Nanoscale Physics · Physics 2022-06-01 Iris Kleinjohann , Andreas Fischer , Mikhail M. Glazov , Frithjof B. Anders

We propose a general protocol for on-demand generation of robust entangled states of nuclear and/or electron spins of ultracold $^1\Sigma$ and $^2\Sigma$ polar molecules using electric dipolar interactions. By encoding a spin-1/2 degree of…

Quantum Physics · Physics 2023-04-10 Timur V. Tscherbul , Jun Ye , Ana Maria Rey

The possibility of appearance of spin polarized states in nuclear matter is studied within the framework of a Fermi liquid theory with Skyrme effective forces in a wide range of isospin asymmetries and densities. There are a few possible…

Nuclear Theory · Physics 2007-05-23 A. A. Isayev

In a theoretical study, we investigate the spin dynamics of interacting nitrogen-vacancy (NV) centers and quadrupolar I = 3/2 nuclear spins, specifically 11B spins in hexagonal boron nitride (h-BN) nanosheets located near the microdiamond…

Quantum Physics · Physics 2024-10-03 Lu Chen , Jiawen Jiang , Martin B. Plenio , Qiong Chen

We report results for reaction and vibrational quenching of the collision D with para-H$_2$($v,j=0$) and ortho-H$_2$($v,j=1$) at cold and ultracold temperatures. We investigate the effect of nuclear spin symmetry for barrier dominated…

Chemical Physics · Physics 2015-05-14 I. Simbotin , R. Côté