Related papers: Environment-imposed selection rules for nuclear-sp…
Optical spectroscopy has been the primary tool to study the electronic structure of molecules. However the strict spin selection rule has severely limited its ability to access states of different spin multiplicities. Here we propose a new…
The mechanism for interconversion between the nuclear spin isomers (NSI) of H$_2$O remains shrouded in uncertainties. The temperature dependence displayed by NSI interconversion rates for H$_2$O isolated in an Argon matrix provides evidence…
The H2 molecule has two nuclear spin isomers, the so-called ortho and para isomers. Nuclear spin conversion (NSC) between these states is forbidden in the gas phase. The energy difference between the lowest ortho and para states is as large…
Electron and nuclear spins are very promising candidates to serve as quantum bits (qubits) for proposed quantum computers, as the spin degrees of freedom are relatively isolated from their surroundings, and can be coherently manipulated…
We present a theoretical study of optical electron-spin orientation and spin-dependent Shockley-Read-Hall recombination taking into account the hyperfine coupling between the bound-electron spin and the nuclear spin of a deep paramagnetic…
We have observed millisecond-long coherent evolution of nuclear spins in a quantum wire at 1.2 K. Local, all-electrical manipulation of nuclear spins is achieved by dynamic nuclear polarization in the breakdown regime of the Integer Quantum…
Current typical methods to realize nuclear-nuclear quantum gates require a sequence of electronnuclear quantum gates by using dynamical decoupling techniques, which are implemented at low temperature because of short decoherence and…
We study coherent dynamics in a system of dipolar coupled spin qubits diluted in solid and subjected to a driving microwave field. In the case of rare earth ions, anisotropic crystal background results in anisotropic g tensor and thus…
It is well known that the association of parahydrogen (pH2) with an unsaturated molecule or a transient metalorganic complex can enhance the intensity of NMR signals; the effect is known as parahydrogen-induced polarization (PHIP). During…
We compute nuclear spin dependent structure functions using a dynamical model for bound nucleon densities and hence calculate nuclear modifications to asymmetries observed in recent doubly polarised deep inelastic scattering experiments. We…
We present a general theoretical treatment and calculations of the fine and hyperfine structures in the spectra of high-$n$ molecular Rydberg states in static uniform electric fields. The treatment combines (i) multichannel quantum-defect…
Isospin symmetry of atomic nuclei is explicitly broken by the charge-dependent interactions, primarily the Coulomb force. Within the nuclear density functional theory, isospin is also broken spontaneously. We propose a projection scheme…
Recent discoveries regarding current-induced spin-orbit torques produced by heavy-metal/ferromagnet and topological-insulator/ferromagnet bilayers provide the potential for dramatically-improved efficiency in the manipulation of magnetic…
Coupled electron-nuclear spins represent a promising quantum system, where the optically induced electron spin polarization can be dynamically transferred to nuclear spins via the hyperfine interaction. Most experiments on dynamic nuclear…
Recent theoretical work has established the presence of hidden spin and orbital textures in non-magnetic materials with inversion symmetry. Here, we propose that these textures can be detected by nuclear magnetic resonance (NMR)…
Under optical cooling of nuclei, a strongly correlated nuclear-spin polaron state can form in semiconductor nanostructures with localized charge carriers due to the strong hyperfine interaction of the localized electron spin with the…
The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…
Two-dimensional colloidal suspensions exposed to periodic external fields exhibit a variety of molecular crystalline phases. There two or more colloids assemble at lattice sites of potential minima to build new structural entities, referred…
The ability to initialise nuclear spins, which are typically in a mixed state even at low temperature, is a key requirement of many protocols used in quantum computing and simulations as well as in magnetic resonance spectroscopy and…
The water molecule occurs in two nuclear-spin isomers that differ by the value of the total nuclear spin of the hydrogen atoms, i.e., $I=0$ for para-H$_2$O and $I=1$ for ortho-H$_2$O. Spectroscopic transitions between rovibrational states…