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We present an angle-resolved photoemission study of the electronic band structure of the excitonic insulator Ta$_2$NiSe$_5$, as well as its evolution upon Sulfur doping. Our experimental data show that while the excitonic insulating phase…

In this work we perform a detailed first-principles analysis of the electronic and optical properties of NiBr$_2$ within the state-of-the-art $GW$+BSE scheme to determine whether this system displays negative excitonic energies, which would…

Materials Science · Physics 2023-03-29 Stefano Di Sabatino , Alejandro Molina-Sánchez , Pina Romaniello , Davide Sangalli

A new state of matter, an excitonic insulator (EI) state, was predicted to emerge from Bose-Einstein condensation of electron-hole pairs. Some candidate materials were suggested but it has been elusive to confirm its existence. Recent works…

Strongly Correlated Electrons · Physics 2021-05-12 Jin Mo Bok , Jungseek Hwang , Han-Yong Choi

We study the dynamical phase transition out of an excitonic insulator phase after photo-excitation using a time-dependent extension of the selfconsistent GW method. We connect the evolution of the photoemission spectra to the dynamics of…

Strongly Correlated Electrons · Physics 2016-07-20 Denis Golež , Philipp Werner , Martin Eckstein

Excitonic insulator (EI) is an intriguing insulating phase of matter, where electrons and holes are bonded into pairs, so called excitons, and form a phase-coherent state via Bose-Einstein Condensation (BEC). Its theoretical concept has…

Strongly Correlated Electrons · Physics 2020-10-22 L. Chen , T. T. Han , C. Cai , Z. G. Wang , Y. D. Wang , Z. M. Xin , Y. Zhang

Utilizing the time-dependent density-matrix renormalization group technique, we numerically prove photoinduced pairing states in the extended Falicov-Kimball model (EFKM) at half filling, both with and without internal SU(2) symmetry. In…

Strongly Correlated Electrons · Physics 2022-06-24 Satoshi Ejima , Florian Lange , Holger Fehske

In the 1960s speculations arose if a ground state exists in solid state materials with an electron and a hole bound to a pair with their spins added to integer values, i.e. excitons. Here we show that electrons and holes in TmSe0.45Te0.55…

Strongly Correlated Electrons · Physics 2008-02-25 Benno Bucher , Tuson Park , J. D. Thompson , Peter Wachter

The transition metal chalcogenide Ta$_2$NiSe$_5$ undergoes a second-order phase transition at $T_c=328$ K involving a small lattice distortion. Below $T_c$, a band gap at the center of its Brillouin zone increases up to about 0.35 eV. In…

Strongly Correlated Electrons · Physics 2020-08-07 C. Monney , M. Herzog , A. Pulkkinen , Y. Huang , J. Pelliciari , P. Olalde-Velasco , N. Katayama , M. Nohara , H. Takagi , T. Schmitt , T. Mizokawa

The fundamental idea of the excitonic insulator (EI) driven by electron-hole correlations in narrow-gap semiconductors or semimetals was originally proposed in the 1960s, and only theoretical studies had been advanced for a long time.…

Strongly Correlated Electrons · Physics 2024-12-25 Tatsuya Kaneko , Yukinori Ohta

Transition metal dichalcogenides (TMDs), whether in bulk or in monolayer form, exhibit a rich variety of charge-density-wave (CDW) phases and stronger periodic lattice distortions. While the actual role of nesting has been under debate, it…

Strongly Correlated Electrons · Physics 2018-12-12 Diego Pasquier , Oleg V. Yazyev

A variety of experiments have been carried out to establish the origin of the chiral charge-density wave transition in 1T-TiSe$_2$, which in turn has led to contradictory conclusions on the origin of this transition. Some studies suggest…

Materials Science · Physics 2020-10-05 Darshana Wickramaratne , Richard Schaller , Gary Wiederrecht , Goran Karapetrov , I. I. Mazin

We present a new high-resolution angle-resolved photoemission study of 1\textit{T}-TiSe$_{2}$ in both, its room-temperature, normal phase and its low-temperature, charge-density wave phase. At low temperature the photoemission spectra are…

Strongly Correlated Electrons · Physics 2009-11-13 H. Cercellier , C. Monney , F. Clerc , C. Battaglia , L. Despont , M. G. Garnier , H. Beck , L. Patthey , H. Berger , P. Aebi

The interplay between topology and correlations can generate a variety of quantum phases, many of which remain to be explored. Recent advances have identified monolayer WTe2 as a promising material for doing so in a highly tunable fashion.…

Transition metal dichalcogenides with superperiodic lattice distortions have been widely investigated as the platform of ultrafast structural phase manipulations. Here we performed ultrafast electron diffraction on room-temperature…

Materials Science · Physics 2024-04-15 J. Koga , Y. Chiashi , A. Nakamura , T. Akiba , H. Takahashi , T. Shimojima , S. Ishiwata , K. Ishizaka

In the presence of electron-phonon coupling, an excitonic insulator harbors two degenerate ground states described by an Ising-type order parameter. Starting from a microscopic Hamiltonian, we derive the equations of motion for the Ising…

Strongly Correlated Electrons · Physics 2020-12-25 H. Ning , O. Mehio , M. Buchhold , T. Kurumaji , G. Refael , J. G. Checkelsky , D. Hsieh

The excitonic insulator is an intriguing electronic phase of quasi-condensed excitons. A prominent candidate is the small bandgap semiconductor Ta2NiSe5, in which excitons are believed to undergo a BEC-like transition. But experimental…

We consider a dynamical phase transition induced by a short optical pulse in a system prone to thermodynamical instability. We address the case of pumping to excitons whose density contributes directly to the order parameter. To describe…

Strongly Correlated Electrons · Physics 2016-06-22 Serguei Brazovskii , Natasha Kirova

Monolayer transition metal dichalcogenides in the T' phase promise to realize the quantum spin Hall (QSH) effect at room temperature, because they exhibit a prominent spin-orbit gap between inverted bands in the bulk. Here we show that the…

Mesoscale and Nanoscale Physics · Physics 2020-03-04 Daniele Varsano , Maurizia Palummo , Elisa Molinari , Massimo Rontani

Exciton plays an important role in optics and optics-related behaviors and leads to novel correlated phases like charge order, exciton insulator, and exciton-polariton condensation. Dark exciton shows distinct properties from bright one.…

Direct-gap materials hold promises for excitonic insulator. In contrast to indirect-gap materials, here the difficulty to distinguish from a Peierls charge density wave is circumvented. However, direct-gap materials still suffer from the…

Materials Science · Physics 2018-08-29 Zeyu Jiang , Yuanchang Li , Shengbai Zhang , Wenhui Duan