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Transition metal chalcogenide Ta$_2$NiSe$_5$, a promising material for the excitonic insulator, is investigated on the basis of the quasi-one-dimensional three-chain Hubbard model with two conduction ($c$) bands and one valence ($f$) band.…

Strongly Correlated Electrons · Physics 2018-06-19 Kaoru Domon , Takemi Yamada , Yoshiaki Ōno

Many-body interactions can produce novel ground states in a condensed-matter system. For example, interacting electrons and holes can spontaneously form excitons, a neutral bound state, provided that the exciton binding energy exceeds the…

Appropriately designed transition metal oxide heterostructures involving small band gap Mott insulators are argued to support spatially separated electron and hole gasses at equilibrium. Spatial separations and carrier densities favoring…

Strongly Correlated Electrons · Physics 2010-08-05 Andrew J. Millis , Darrell G. Schlom

The origin of the charge density wave (CDW) phase in TiSe$_2$ is a highly debated topic, with lattice and excitonic correlations proposed as the main driving mechanisms. One of the proposed scenarios is the excitonic insulator (EI)…

Strongly Correlated Electrons · Physics 2026-02-25 Dino Novko

Coulomb interactions among electrons and holes in two-dimensional (2D) semimetals with overlapping valence and conduction bands can give rise to a correlated insulating ground state via exciton formation and condensation. One candidate…

We present both theoretical ab initio GW and experimental angle-resolved photoemission (ARPES) and scanning tunneling (STS) spectroscopy results on TiSe2. With respect to the density-functional Kohn-Sham metallic picture, the many-body GW…

Strongly Correlated Electrons · Physics 2011-07-13 M. Cazzaniga , H. Cercellier , M. Holzmann , C. Monney , P. Aebi , G. Onida , V. Olevano

Utrafast control of material physical properties represents a rapid developing field in condensed matter physics. Yet, accessing to the long-lived photoinduced electronic states is still in its early stage, especially with respect to an…

Strongly Correlated Electrons · Physics 2021-04-20 Q. M. Liu , D. Wu , Z. A. Li , L. Y. Shi , Z. X. Wang , S. J. Zhang , T. Lin , T. C. Hu , H. F. Tian , J. Q. Li , T. Dong , N. L. Wang

The electronic structure change of NiS$_{2-x}$Se$_x$ as a function of Se concentration $x$ has been studied by Ni $L$-edge X-ray absorption spectroscopy (XAS). The XAS spectra show distinct features in Ni $L_3$ edge, indicating whether the…

Strongly Correlated Electrons · Physics 2018-02-14 Jinwon Jeong , Kyung Ja Park , En-Jin Cho , Han-Jin Noh , Sung-Baek Kim , Hyeong-Do Kim

First-principles density functional theory plus Bethe-Salpeter equation calculations are employed to investigate the electronic and excitonic properties of monolayer titanium trichalcogenide alloys TiS$_{3-x}$Se$_x$ ($x$=1 and 2). It is…

Materials Science · Physics 2020-12-02 Shan Dong , Yuanchang Li

Recently, we employed electronic polarization-resolved Raman spectroscopy to reveal the strongly correlated excitonic insulator (EI) nature of Ta2NiSe5, Volkov et al. [arXiv:2007.07344], and also showed that for…

Strongly Correlated Electrons · Physics 2021-07-20 Mai Ye , Pavel A. Volkov , Himanshu Lohani , Irena Feldman , Minsung Kim , Amit Kanigel , Girsh Blumberg

Ta2NiSe5 is considered a promising excitonic insulator (EI) candidate with slight phonon contributions, since it exhibits a tiny orthorhombic-to-monoclinic structural distortion at 328 K without any superlattice structure. Our synchrotron…

Strongly Correlated Electrons · Physics 2018-08-08 Akitoshi Nakano , Takumi Hasegawa , Shinya Tamura , Naoyuki Katayama , Satoshi Tsutsui , Hiroshi Sawa

Artificial moir\'e superlattices in 2d van der Waals heterostructure is a new venue for realizing and controlling correlated electronic phenomena. Recently, twisted bilayer WSe$_2$ emerged as a new robust moir\'e system hosting a correlated…

Strongly Correlated Electrons · Physics 2020-12-02 Zhen Bi , Liang Fu

We present a constrained density functional perturbation theory scheme for the calculation of structural and harmonic vibrational properties of insulators in the presence of an excited and thermalized electron-hole plasma. The method is…

Materials Science · Physics 2021-10-13 Giovanni Marini , Matteo Calandra

Innovations in imaging technology involves finding strategies and materials suitable for detection applications over the entire infrared range. Herein, we propose a new design concept based on the unique feature of an excitonic insulator,…

Materials Science · Physics 2022-07-27 Jing Liu , Yuanchang Li

Correlated topological materials often maintain a delicate balance among physical symmetries: many topological orders are symmetry protected, while most correlated phenomena arise from spontaneous symmetry breaking. It is rare to find cases…

Layered materials enable the assembly of a new class of heterostructures where lattice-matching is no longer a requirement. Interfaces in these heterostructures therefore become a fertile ground for unexplored physics as dissimilar…

We calculate the critical temperature below which an excitonic insulator exists at the pressure-induced semiconductor-semimetal transition. Our approach is based on an effective-mass model for valence and conduction band electrons…

Strongly Correlated Electrons · Physics 2009-11-11 Franz X. Bronold , Holger Fehske

In this work, we analyze the excitonic gap generation in the strong-coupling regime of thin films of three-dimensional time-reversal-invariant topological insulators. We start by writing down the effective gauge theory in 2+1-dimensions…

Strongly Correlated Electrons · Physics 2017-09-13 N. Menezes , C. Morais Smith , Giandomenico Palumbo

Excitonic insulators (EI) arise from the formation of bound electron-hole pairs (excitons) in semiconductors and provide a solid-state platform for quantum many-boson physics. Strong exciton-exciton repulsion is expected to stabilize…

High-resolution time- and angle-resolved photoemission measurements were conducted on the topological insulator ZrTe5. With strong femtosecond photoexcitation, a possible ultrafast phase transition from a weak to a strong topological…

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