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Optical second harmonic generation is a second-order nonlinear process that combines two photons of a given frequency into a third photon at twice the frequency. Due to the symmetry constraints, it is widely used as a sensitive probe to…

High harmonic generation (HHG) from condensed matter phase holds promise to promote future cutting-edge research in the emerging field of attosecond nanoscopy. The key for the progress of the field relies on the capability of the existing…

Optics · Physics 2021-07-07 Hicham Agueny

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information…

This research will examine the computational methods to calculate the nonlinear optical process of second harmonic generation (SHG) that will be hypothesized to be present during lithium ion insertion into silicon nanowires. First it will…

Optics · Physics 2021-10-19 Donald C. Boone

Black phosphorene (BP) has emerged as a promising platform for tunable nonlinear photonics due to its layer-dependent bandgap, high carrier mobility, and remarkable in-plane anisotropy. This study investigates the second-harmonic generation…

Mesoscale and Nanoscale Physics · Physics 2025-10-14 Yan Meng , Kainan Chang , Yanyan Qian , Luxia Wang , Jin Luo Cheng

The effective second-harmonic generation (SHG) coefficient is a crucial data that quantifies the efficiency of transforming fundamental frequency light into its second harmonic. With the help of the symmetry of nonlinear optical…

Optimization and Control · Mathematics 2026-02-24 Die Xiao , Yisheng Song

Second-harmonic generation (SHG) has emerged as a promising tool for detecting electronic and magnetic structures in noncentrosymmetric materials, but 100$\%$ spin-polarized SHG has not been reported. In this work, we demonstrate nearly…

Materials Science · Physics 2023-09-06 Y. Q. Liu , M. S. Si , G. P. Zhang

In this paper we present a theoretical examination of second-harmonic generation (SHG) in a graphene monolayer integrated within an attenuated total internal reflection (ATR) configuration. By embedding graphene in this optical setup, we…

Second harmonic generation (SHG) microscopy is a valuable tool for optical microscopy. SHG microscopy is normally performed as a point scanning imaging method, which lacks phase information and is limited in spatial resolution by the…

Plasmonic enhancement of nonlinear optical processes confront severe limitations arising from the strong dispersion of metal susceptibilities and small interaction volumes that hamper desirable phase-matching-like conditions. Maximizing…

We report on theoretical study of second-harmonic generation (SHG) in plasmonic nanostructures interacting with two-level quantum emitters (QE) under incoherent energy pump. We generalize driven-dissipative Tavis-Cummings model by…

Optics · Physics 2021-03-17 Maxim Sukharev , Oleksiy Roslyak , Andrei Piryatinski

We report the observations of unexpected layer-dependent, strong, and anisotropic second harmonic generations (SHGs) in atomically thin ReS2. Appreciable (negligible) SHGs are obtained from even (odd) numbers of ReS2 layers, which is…

Optics · Physics 2018-08-20 Yu Song , Siqi Hu , Miao-Ling Lin , Xuetao Gan , Ping-Heng Tan , Jianlin Zhao

The controlled assembly of twisted 2D structures requires precise determination of the crystal orientation of their component layers. In the established procedure, the second-harmonic generation (SHG) intensity of a noncentrosymmetric layer…

Rotational anisotropy second harmonic generation (RA-SHG) is a nonlinear optical technique used to probe the symmetry of condensed matter systems. Measuring the dependence of the SHG susceptibility on one or more external parameters,…

Materials Science · Physics 2025-04-08 Karna A. Morey , Bryan T. Fichera , Baiqing Lv , Zonqi Shen , Nuh Gedik

It is of fundamental importance but challenging to simultaneously identify atomic and magnetic configurations of two-dimensional van der Waals materials. In this work, we show that the nonreciprocal second-harmonic generation (SHG) can be a…

Materials Science · Physics 2020-07-15 Wenshen Song , Ruixiang Fei , Li Yang

A comprehensive analysis of second harmonic generation (SHG) in a diatomic zincblende crystal based on the Simplified Bond Hyperpolarizability Model (SBHM), Group Theory (GT) is presented. The third rank tensor between the two approaches…

Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher…

Second harmonic generation (SHG) spectroscopy ubiquitously enables the investigation of surface chemistry, interfacial chemistry as well as symmetry properties in solids. Polarization-resolved SHG spectroscopy in the visible to infrared…

Nonlinear metamaterials show potential for realizing flat nonlinear optical devices but generally lack in terms of achievable conversion efficiencies. Recent work has focused on enhancing nonlinear processes by utilizing high quality factor…

We have studied on optical second harmonic generations (SHGs) from atomically thin MoTe2 flakes with 2H and 1T' phases. From 2H-MoTe2 samples with odd (even) numbers of layers, strong (negligible) SHGs are observed due to the…

Optics · Physics 2018-05-25 Yu Song , Ruijuan Tian , Jiulong Yang , Rui Yin , Jianlin Zhao , Xuetao Gan
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