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Second harmonic generation (SHG) is a coherent nonlinear phenomenon that plays an important role in laser color conversion. Lithium niobate (LN), which features both a large band gap and outstanding second-order nonlinearities, acts as an…

We demonstrate unexpectedly strong second harmonic generation (SHG) in Argon gas by use of spatiotemporally focused (SF) femtosecond laser pulses. The resulting SHG by the SF scheme at a 75 cm distance shows a significantly enhanced…

Femtosecond pump-probe second-harmonic generation (SHG) and transient linear reflectivity measurements were carried out on polycrystalline Cu, Ag and Au in air to analyze whether the electron temperature affects Fresnel factors or nonlinear…

Condensed Matter · Physics 2015-06-25 J. Hohlfeld , U. Conrad , E. Matthias

Plasmonic resonances in metallic nanostructures have been shown to drastically enhance local electromagnetic fields, and thereby increase the efficiency of nonlinear optical phenomena, such as second harmonic generation (SHG). While it has…

Second harmonic generation (SHG) is a non-linear optical process, where two photons coherently combine into one photon of twice their energy. Efficient SHG occurs for crystals with broken inversion symmetry, such as transition metal…

We experimentally study the optical second harmonic generation (SHG) from deep subwavelength gold-silver heterodimer and silver-silver and gold-gold homodimers. Our results show that the SHG from the heterodimer is about an order of…

High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…

Second-harmonic generation microscopy is a powerful technique capable of probing local crystal symmetries and electric fields at interfaces. However, it often suffers from weak signal strength and is difficult to understand in multilayer…

We analyze second-harmonic generation (SHG) at a thin effectively quadratic nonlinear interface between two linear optical media. We predict multistability of SHG for both plane and localized waves, and also describe two-color localized…

patt-sol · Physics 2007-05-23 Andrey A. Sukhorukov , Yuri S. Kivshar , Ole Bang

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Spectroscopy of magnetization-induced second-harmonic generation (MSHG) is studied in magnetic Co$_{x}$Ag$_{1-x}$ granular films containing Co nanoparticles. A strong resonance of the magnetic contrast of the second-harmonic generation…

Adaptation and Self-Organizing Systems · Physics 2007-05-23 E. M. Kim , T. V. Murzina , A. F. Kravets , M. Inoue , G. Marowsky , O. A. Aktsipetrov

Silicon-based nonlinear metasurfaces were implemented only with third-order nonlinearity due to the crystal centrosymmetry and the efficiencies are considerably low, which hinders their practical applications with low-power lasers. Here, we…

Copper sulfide (CuS) has garnered significant attention in various fields of application due to its unique electronic, optical, and catalytic features. In this study, we present the chemical vapor deposition (CVD)-based synthesis of…

Materials Science · Physics 2023-05-16 Abdulsalam Aji Suleiman , Reza Rahighi , Amir Parsi , Talip Serkan Kasırga

We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

Nonlinear optics, and particularly second harmonic generation (SHG), is increasingly used in many modern disciplines from material characterization in physical sciences to bio-imaging in medicine and optical signal processing in information…

Strongly Correlated Electrons · Physics 2021-03-17 G. van der Laan , S. W. Lovesey

High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in…

By combining analytical and numerical approaches, we study resonantly enhanced second-harmonic generation (SHG) by individual high-index dielectric nanoparticles made of centrosymmetric materials. Considering both bulk and surface…

Optics · Physics 2018-01-08 Daria Smirnova , Alexander I. Smirnov , Yuri S. Kivshar

Optical spectroscopy based on second-order nonlinearity is a critical technique for characterizing two-dimensional (2D) crystals as well as bioimaging and quantum optics. It is generally believed that second-harmonic generation (SHG) in…

Mesoscale and Nanoscale Physics · Physics 2026-01-14 Haoning Tang , Zhitong Ding , Tianyi Ruan , Zeyu Hao , Kenji Watanabe , Takashi Taniguchi , Haozhe Wang , Ali Javey , Feng Wang , Yuan Cao

We have developed a numerical method for calculating the second harmonic generation (SHG) generated by an anisotropic material whose optical properties present an arbitrary modulation in one dimension. The method is based on the Berreman…

Optics · Physics 2023-05-31 J. Ortega , C. L. Folcia , J. Etxebarria

This study presents an investigation of second harmonic generation (SHG) resulting from interaction of radially polarized laser beam propagating in homogeneous, unmagnetized plasma. Lorentz force and continuity equations have been used to…

Plasma Physics · Physics 2025-09-30 Shivani Aggarwal , Saumya Singh , Dinkar Mishra , Bhupesh Kumar , Pallavi Jha