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We investigate the electronic structure of nickelate superconductor NdNiO2 upon hole doping, by means of density-functional theory and dynamical mean-field theory. We demonstrate the strong intrinsic hybridization between strongly…

Strongly Correlated Electrons · Physics 2021-01-13 Zhao Liu , Chenchao Xu , Chao Cao , W. Zhu , Z. F. Wang , Jinlong Yang

The recent discovery of superconductivity in Nd$_{1-x}$Sr$_{x}$NiO$_2$ has drawn significant attention in the field. A key open question regards the evolution of the electronic structure with respect to hole doping. Here, we exploit x-ray…

The recent observation of superconductivity in infinite-layer Nd$_{1-x}$Sr$_x$NiO$_2$ thin films has attracted a lot of attention, since this compound is electronically and structurally analogous to the superconducting cuprates. Due to the…

Motivated by recent angle-resolved photoemission spectroscopy (ARPES) experiments on infinite-layer (IL) nickelates, we employ determinant quantum Monte Carlo (DQMC) to study the three-orbital Emery model ($d$-$p$ model) coupled to an…

Strongly Correlated Electrons · Physics 2026-03-24 Yan Peng , Rui Peng , Mi Jiang

The correlated electronic structure of the infinite-layer compounds NdNiO$_2$ and SrCuO$_2$ at stoichiometry and with finite hole doping is compared. Key differences are elucidated from an advanced first-principles many-body perspective.…

Strongly Correlated Electrons · Physics 2020-03-06 Frank Lechermann

We investigate charge distribution in the recently discovered high-$T_c$ superconductors, layered nickelates. With increasing value of charge-transfer energy we observe the expected crossover from the cuprate to the local triplet regime…

Strongly Correlated Electrons · Physics 2021-10-13 Tharathep Plienbumrung , Michael Schmid , Maria Daghofer , Andrzej M. Oleś

Using first-principles density functional theory calculations, we investigated the effect of charge doping in a LaNiO$_3$/SrTiO$_3$ superlattice. The detailed analysis based on two different simulation methods for doping clearly shows that…

Strongly Correlated Electrons · Physics 2015-06-04 Heung-Sik Kim , Myung Joon Han

We theoretically investigate the unconventional superconductivity in the newly discovered infinite-layer nickelates Nd$_{1-x}$Sr$_{x}$NiO$_{2}$ based on a two-band model. By analyzing the transport experiments, we propose that the doped…

Superconductivity · Physics 2020-12-08 Jun Chang , Jize Zhao , Yang Ding

Using a combination of {\it ab initio} bandstructure methods and dynamical mean-field theory we study the single-particle spectrum of the prototypical charge-transfer insulator NiO. Good agreement with photoemission and…

Strongly Correlated Electrons · Physics 2015-06-25 J. Kunes , V. I. Anisimov , A. V. Lukoyanov , D. Vollhardt

The recent discovery of high-T$_{c}$ superconductivity (HTS) in Sr-doped NdNiO$_2$ has sparked a renewed interest in investigating nickelates as cuprate counterparts. Parent cuprates [Cu$^{2+}$: d$^9$] are antiferromagnetic charge-transfer…

Superconductivity · Physics 2021-01-04 Jyoti Krishna , Harrison LaBollita , Adolfo O. Fumega , Victor Pardo , Antia S. Botana

The superconducting infinite-layer (IL) nickelates offer a new platform for investigating the long-standing problem of high-temperature superconductivity. Many models were proposed to understand its superconducting mechanisms based on the…

The recent observation of superconductivity in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$ has raised fundamental questions about the hierarchy of the underlying electronic structure. Calculations suggest that this system falls in the Mott-Hubbard regime,…

The novel nickelate superconductors of infinite-layer type feature challenging electronic pecularities in the normal-state phase diagram with doping. Distinct many-body behavior and different dispersion regimes of the entangled…

Strongly Correlated Electrons · Physics 2021-04-29 Frank Lechermann

Using \emph{ab initio} band structure methods and DFT+dynamical mean-field theory approach we explore the possible formation of spin and charge stripes in the Ni-O plane of hole-doped infinite-layer nickelates, $R$NiO$_2$. Our results…

Strongly Correlated Electrons · Physics 2022-10-12 K. G. Slobodchikov , I. V. Leonov

In cuprates, electron doping yields a much lower superconducting $T_c$ than hole doping. For recently discovered nickelate superconductors, the analogous doping strategies become more challenging. Consequently, while hole-doped…

Superconductivity · Physics 2026-05-21 Xun Liu , Chao Deng , Wenfeng Wu , Liang Si , Mi Jiang

Rare-earth nickelates R$^{3+}$Ni$^{3+}$O$_3$ (R=Lu-Pr, Y) show a striking metal-insulator transition in their bulk phase whose temperature can be tuned by the rare-earth radius. These compounds are also the parent phases of the newly…

Materials Science · Physics 2021-07-21 Lucia Iglesias , Manuel Bibes , Julien Varignon

Using the DFT+dynamical mean-field theory approach we study the effects of electronic correlations and doping on the normal state electronic structure of the double-layer nickelate superconductor La$_3$Ni$_2$O$_7$ under pressure. In…

Strongly Correlated Electrons · Physics 2026-04-27 I. V. Leonov

To understand the superconductivity recently discovered in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, we carried out LDA+DMFT (local density approximation plus dynamical mean-field theory) and magnetic force response calculations. The on-site correlation…

Superconductivity · Physics 2020-02-25 Siheon Ryee , Hongkee Yoon , Taek Jung Kim , Min Yong Jeong , Myung Joon Han

We report a determinant quantum Monte Carlo study of a two-band model, inspired by infinite-layer nickelates, focusing on the influence of interlayer hybridization between $3d_{x^2-y^2}$ orbitals derived from Ni (or Ni and O) in one layer…

Strongly Correlated Electrons · Physics 2024-06-10 Fangze Liu , Cheng Peng , Edwin W. Huang , Brian Moritz , Chunjing Jia , Thomas P. Devereaux

A strong anisotropic distribution of the holes in Ni 3d and O 2p orbitals is observed in the polarization dependent O1s and Ni2p3/2 x-ray absorption spectroscopy of the linear-chain nickelate Y1-xCaxBaNiO5 (x = 0, 0.05, 0.1, 0.2), which…

Strongly Correlated Electrons · Physics 2009-11-07 Z. Hu , M. Knupfer , M. Kielwein , U. K. Roessler , M. S. Golden , J. Fink , F. M. F. de Groot , T. Ito , G. Kaindl
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