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Motivated by the recent X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS) experiments, we use a detailed impurity model to explore the nature of the parent compound and hole doped states of (La, Nd,…

Strongly Correlated Electrons · Physics 2022-10-12 Mi Jiang , Mona Berciu , George A. Sawatzky

The discovery of unconventional superconductivity in hole doped NdNiO2, similar to CaCuO2, has received enormous attention. However, different from CaCuO2, RNiO2 (R = Nd, La) has itinerant electrons in the rare-earth spacer layer. Previous…

Strongly Correlated Electrons · Physics 2020-05-18 Yuhao Gu , Sichen Zhu , Xiaoxuan Wang , Jiangping Hu , Hanghui Chen

We study the correlated electronic structure of single-layer iridates based on structurally-undistorted Ba$_2$IrO$_4$. Starting from the first-principles band structure, the interplay between local Coulomb interactions and spin-orbit…

Strongly Correlated Electrons · Physics 2015-09-02 Alexander Hampel , Christoph Piefke , Frank Lechermann

The evolution of the electronic structures of strongly correlated insulators with doping has long been a central fundamental question in condensed matter physics; it is also of great practical relevance for applications. We have studied the…

Infinite layer nickelates have garnered significant attention due to their potential for high-temperature superconductivity. Despite extensive research, the interplay between oxygen stoichiometry and electronic properties in infinite layer…

A correspondence exists between the multi-orbital Hubbard model and the bilayer Hubbard model, in which superconductivity is optimized in an incipient-band regime in both cases. In the multi-orbital system, the orbital level offset $\Delta…

Superconductivity · Physics 2026-03-13 Shu Kamiyama , Reo Kohno , Yuto Hoshi , Kensei Ushio , Daiki Nakaoka , Hirofumi Sakakibara , Kazuhiko Kuroki

The recent and exciting discovery of superconductivity in the hole-doped infinite-layer nickelate Nd 1-{\delta} Sr {\delta} NiO 2 draws strong attention to correlated quantum materials. From a theoretical view point, this new class of…

Strongly Correlated Electrons · Physics 2021-01-05 Byungkyun Kang , Corey Melnick , Patrick Semon , Siheon Ryee , Myung Joon Han , Gabriel Kotliar , Sangkook Choi

Since the discovery of superconductivity in infinite-layer nickelates RNiO$_2$ (R=La, Pr, Nd), great research efforts have been paid to unveil its underlying superconducting mechanism. However, the physical origin of the intriguing…

Strongly Correlated Electrons · Physics 2022-07-20 T. Y. Xie , Z. Liu , Chao Cao , Z. F. Wang , J. L. Yang , W. Zhu

The predominant Ni-multiorbital nature of infinite-layer neodynium nickelate at stoichiometry and with doping is revealed. We investigate the correlated electronic structure of NdNiO$_2$ at lower temperatures and show that first-principles…

Strongly Correlated Electrons · Physics 2020-10-06 Frank Lechermann

Despite exhibiting a similar $d_{x^2-y^2}$ band character to cuprates, infinite-layer nickelates host additional electron pockets that distinguish them from single-band cuprates. The elusive orbital origin of these electron pockets has led…

While both the hole and electron doped cuprates can exhibit $d_{x^2-y^2}$-wave superconductivity, the local distribution of the doped carriers is known to be significantly different with the doped holes going primarily on the O sites while…

Strongly Correlated Electrons · Physics 2015-11-11 Steven R. White , D. J. Scalapino

High-T$_c$ superconductivity has recently been discovered in Ruddlesden-Popper phase nickelates under pressure, where the low-energy electronic structure is dominated by Ni $d_{x^2 - y^2}$ and $d_{z^2}$ orbitals. However, the respective…

The normal-state transport properties of superconducting infinite-layer nickelates are investigated within an interacting three-orbital model. It includes effective Ni-$d_{z^2}$, Ni-$d_{x^2-y^2}$ bands as well as the self-doping band degree…

Superconductivity · Physics 2023-06-14 Steffen Bötzel , Ilya M. Eremin , Frank Lechermann

The electronic structure of the intercalated iron-based superconductor Ba2Ti2Fe2As4O (Tc - 21.5 K) has been investigated by using angle-resolved photoemission spectroscopy and combined local density approximation and dynamical mean field…

Significant magnetic exchange interactions have been observed in infinite-layer nickelates RNiO2 (R = La, Pr, Nd), which exhibit unconventional superconductivity upon hole doping. Despite their structural and Fermi surface similarities to…

Superconductivity · Physics 2025-05-15 Yanbing Zhou , Dan Zhao , Boyun Zeng , Chengliang Xia , Yu Wang , Hanghui Chen , Tao Wu , Xianhui Chen

Since the discovery of superconductivity in infinite-layer nickelates, there have been extensive efforts to unravel their electronic structure and pairing mechanism. In particular, understanding how the electronic structure evolves with…

Superconductivity · Physics 2026-02-11 Woo Jin Kim , Kyuho Lee , Eun Kyo Ko , Jaeseok Son , Yonghun Lee , Yijun Yu , Soon Jae Moon , Tae Won Noh , Harold Y. Hwang

The in-plane oxygen vibrations in La2NiO4 are investigated for several hole-doping concentrations both theoretically and experimentally via inelastic neutron scattering. Using an inhomogeneous Hartree-Fock plus RPA numerical method in a…

Strongly Correlated Electrons · Physics 2009-10-31 R. J. McQueeney , A. R. Bishop , Ya-Sha Yi , Z. G. Yu

In this work, we investigate collective electronic fluctuations and, in particular, the possibility of the charge density wave ordering in an infinite-layer NdNiO$_2$. We perform advanced many-body calculations for the ab-initio…

Strongly Correlated Electrons · Physics 2024-06-03 Evgeny A. Stepanov , Matteo Vandelli , Alexander I. Lichtenstein , Frank Lechermann

The recent discovery of high-$T_c$ superconductivity in Ruddlesden-Popper (RP) nickelates has motivated extensive efforts to explore higher $T_c$ superconductors. Here, we systematically investigate Nd-doped La$_3$Ni$_2$O$_7$ using density…

Superconductivity · Physics 2026-01-06 Cui-Qun Chen , Wenyuan Qiu , Zhihui Luo , Meng Wang , Dao-Xin Yao

The difficulty of determining cation concentrations and oxygen stoichiometry in infinite-layer nickelate thin films has so far prevented clear experimental identification of the nickel electron configuration in the superconducting phase. We…