English

Hund-Heisenberg model in superconducting infinite-layer nickelates

Superconductivity 2020-12-08 v3 Strongly Correlated Electrons

Abstract

We theoretically investigate the unconventional superconductivity in the newly discovered infinite-layer nickelates Nd1x_{1-x}Srx_{x}NiO2_{2} based on a two-band model. By analyzing the transport experiments, we propose that the doped holes dominantly enter the Ni dxyd_{xy} or/and d3z2r2d_{3z^{2}-r^{2}} orbitals as charged carriers, and form a conducting band. Via the onsite Hund coupling, the doped holes are coupled to the Ni localized holes in the dx2y2d_{x^{2}-y^{2}} orbital band. We demonstrate that this two-band model could be further reduced to a Hund-Heisenberg model. Using the reduced model, we show the non-Fermi liquid state above the critical TcT_{c} could stem from the carriers coupled to the spin fluctuations of the localized holes. In the superconducting phase, the short-range spin fluctuations mediate the carriers into Cooper pairs and establish dx2y2d_{x^{2}-y^{2}}-wave superconductivity. We further predict that the doped holes ferromagnetically coupled with the local magnetic moments remain itinerant even at very low temperature, and thus the pseudogap hardly emerges in nickelates. Our work provides a new superconductivity mechanism for strongly correlated multi-orbital systems and paves a distinct way to exploring new superconductors in transition or rare-earth metal oxides.

Keywords

Cite

@article{arxiv.1911.12731,
  title  = {Hund-Heisenberg model in superconducting infinite-layer nickelates},
  author = {Jun Chang and Jize Zhao and Yang Ding},
  journal= {arXiv preprint arXiv:1911.12731},
  year   = {2020}
}

Comments

the paper was expanded, 7 pages, 1 figure