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Attosecond science is well developed for atoms and promising results have been obtained for molecules and solids. Here, we review the first steps in developing attosecond time-resolved measurements in liquids. These advances provide access…

Other Condensed Matter · Physics 2020-09-11 H. J. Wörner , A. Schild , D. Jelovina , I. Jordan , C. Perry , T. T. Luu , Z. Yin

Electric control of spins has been a longstanding goal in the field of solid state physics due to the potential for increased efficiency in information processing. This efficiency can be optimized by transferring spintronics to the atomic…

Mesoscale and Nanoscale Physics · Physics 2023-11-30 Piotr Kot , Maneesha Ismail , Robert Drost , Janis Siebrecht , Haonan Huang , Christian R. Ast

We study electron transfer between two separated nuclei using local control theory. By conditioning the algorithm in a symmetric system formed by two protons, one can favored slow transfer processes, where tunneling is the main mechanism,…

Quantum Physics · Physics 2018-04-18 Patricia Vindel-Zandbergen , Christoph Meier , Ignacio R. Sola

Ultrafast science studies the dynamics of electrons in matter with extreme temporal precision, typically in the attosecond and femtosecond time domain. Recent experimental and theoretical progress has put metal-insulator-metal (MIM)…

Mesoscale and Nanoscale Physics · Physics 2025-03-20 Boyang Ma , Michael Krüger

We present an extension of the tunneling theory for scanning tunneling microcopy (STM) to include different types of vibrational-electronic couplings responsible for inelastic contributions to the tunnel current in the strong-coupling…

We theoretically show how the spin orientation of a single magnetic adatom can be controlled by spin polarized electrons in a scanning tunneling microscope configuration. The underlying physical mechanism is spin assisted inelastic…

Mesoscale and Nanoscale Physics · Physics 2010-03-11 F. Delgado , J. J. Palacios , J. Fernandez-Rossier

In the last decade, the development of Ultrafast Electron Diffraction (UED) and Microscopy (UEM) has enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications…

Chemical Physics · Physics 2018-01-16 Mohammed Th. Hassan

With the invention of scanning probe techniques, direct imaging of single atoms and molecules became possible. Today, scanning tunnelling microscopy (STM) routinely provides angstrom-scale image resolution. At the same time, however, STM…

Mesoscale and Nanoscale Physics · Physics 2024-01-30 C. Weiss , C. Wagner , C. Kleimann , F. S. Tautz , R. Temirov

Visualizing and controlling electron dynamics over femtosecond timescale play a key role in the design of next-generation electronic devices. Using simulations, we demonstrate the electronic oscillation inside the naphthalene molecule can…

Quantum Physics · Physics 2020-12-24 Rulin Wang , Fuzhen Bi , Wencai Lu , Xiao Zheng , ChiYung Yam

In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…

Atomic Physics · Physics 2015-05-19 Jan Conrad Baggesen , Lars Bojer Madsen

Transport through quantum coherent conductors, like atomic junctions, is described by the distribution of conduction channels. Information about the number of channels and their transmission can be extracted from various sources, such as…

We study ultrafast ionization dynamics using orthogonally polarized two-color (OTC) laser pulses involving the resonant "first plus second" ($\omega+2\omega$) scheme. The scheme is illustrated by numerical simulations of the time-dependent…

Atomic Physics · Physics 2019-12-16 Hicham Agueny

Understanding and controlling decoherence in open quantum systems is of fundamental interest in science, while achieving long coherence times is critical for quantum information processing. Although great progress was made for individual,…

Mesoscale and Nanoscale Physics · Physics 2023-03-23 Lisanne Sellies , Raffael Spachtholz , Philipp Scheuerer , Jascha Repp

Controlling electrically-stimulated quantum light sources (QLS) is key for developing integrated and low-scale quantum devices. The mechanisms leading to quantum emission are complex, as a large number of electronic states of the system…

Mesoscale and Nanoscale Physics · Physics 2024-02-28 Katharina Kaiser , Anna Rosławska , Michelangelo Romeo , Fabrice Scheurer , Tomáš Neuman , Guillaume Schull

The pursuit of ever-shorter time scales is a frontier in modern physics, exemplified by the synthesis of attosecond light pulses -- an achievement made possible by coherently superimposing a broad range of photon energies, as required by…

Mesoscale and Nanoscale Physics · Physics 2025-04-25 Xin Jin , Cruz I. Velasco , F. Javier García de Abajo

Ultrafast electron microscopy (UEM) has found widespread applications in physics, chemistry, and materials science, enabling real-space imaging of dynamics on ultrafast timescales. Recent advances have pushed the temporal resolution of UEM…

State-of-the-art attosecond metrology deals with the detection and characterization of photon pulses with typical energies up to the hundreds of eV and time resolution of several tens of attoseconds. Such short pulses are used for example…

Instrumentation and Detectors · Physics 2015-06-04 Andreas Ipp , Jörg Evers , Christoph H. Keitel , Karen Z. Hatsagortsyan

Femtosecond-fast and nanometre-size pulses of electrons are emerging as unique probes for ultrafast dynamics at the nanoscale. Presently, such pulses are achievable only in highly sophisticated ultrafast electron microscopes or equally…

Scanning tunneling spectroscopy measures how a single electron with definite energy propagates between a sample surface and the tip of a scanning tunneling microscope. In the simplest description, the differential conductance measured is…

Mesoscale and Nanoscale Physics · Physics 2019-05-07 Mikko M. Ervasti , Fabian Schulz , Peter Liljeroth , Ari Harju

The Scanning Tunneling Microscope (STM) is a powerful instrument to study electronic density of states at surfaces down to atomic scale. Many interesting samples require studying variations as a function of the magnetic field, which is most…

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