Related papers: Clocking and controlling attosecond currents in a …
Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond…
The thesis explores calculating tunneling current densities between planar conducting electrodes in an STM. It considers factors like bias voltages and the separation between electrodes, using Fermi energy and work functions. Pauli blocking…
Ultrashort electron pulses with a high average current provide a powerful means of enhancing time-resolved imaging and photon generation. In this study, we report the attosecond shaping of sub-relativistic electron beams using membranes in…
Tunneling spectroscopy played a central role in the experimental verification of the microscopic theory of superconductivity in the classical superconductors. Initial attempts to apply the same approach to high-temperature superconductors…
Over the past few decades, following the first demonstration of ultrafast electron microscopy, numerous research groups have focused on achieving attosecond temporal resolution in electron microscopy with the goal of imaging electron and…
Attosecond X-ray pulses are indispensable for exploring ultrafast phenomena in matter on Angstrom and attosecond scales. Here we propose a new method to realize spatiotemporal shaping of attosecond X-rays through temporal control of the…
Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…
Attosecond angular streaking, also known as the "attoclock", employs a short elliptically polarized laser pulse to tunnel ionize an electron from an atom or a molecule and to put a time stamp on this process by deflecting the photoelectron…
Attosecond laser pulses open the door to resolve microscopic electron dynamics in time. Experiments performed include the decay of a core hole, the time-resolved measurement of photo ionization and electron tunneling. The processes…
Scanning Tunneling Microscopy (STM) is a powerful technique that utilizes quantum tunneling to visualize atomic surfaces with high precision. This study presents detailed topographic maps and evaluates the local density of states (LDOS) for…
Attosecond angular streaking measurements have revealed deep insights into the timing of tunnel ionization processes of atoms in intense laser fields. So far experiments of this type have been performed only with a cold-target recoil-ion…
Coherent control over electron dynamics in atoms and molecules using high-intensity circularly-polarized laser pulses gives rise to current loops, resulting in the emission of magnetic fields. We propose and demonstrate with ab-initio…
The generation of ultrashort light pulses is essential for the advancement of attosecond science. Here, we show that attosecond pulses approaching the Fourier limit can be generated through optimized optical driving of tunneling particles…
Electronic correlations occur on attosecond timescales, dictating how chemical bonds form, energy flows, and materials respond to light. Capturing such many-body processes requires light pulses of similar duration. The soft X-ray water…
Squeezed light has revolutionized quantum metrology by enhancing interferometry for sensitive applications such as the detection of gravitational waves. Squeezed light has also played a pivotal role in quantum information science with…
Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element…
Twenty-five years have passed since the first experimental demonstration of attosecond pulses, marking the advent of our ability to resolve and control electron motion in real time. What began as a technological breakthrough - generating…
In the last decade, advancements in attosecond spectroscopy have allowed us to study electron motion dynamics in condensed matter. The access to these electron dynamics and, consequently, its control by an ultrafast light field paves the…
A scanning tunneling microscope (STM) has been equipped with a nanoscale force sensor and signal transducer composed of a single D2 molecule that is confined in the STM junction. The uncalibrated sensor is used to obtain ultra-high…
We employ ultrafast pump-probe spectroscopy to directly monitor electron tunneling between discrete orbital states in a pair of spatially separated quantum dots. Immediately after excitation, several peaks are observed in the pump-probe…