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The first excited isomeric state of $^{229}$Th possesses the lowest energy among all known excited nuclear states. The expected energy is accessible with today's laser technology and in principle allows for a direct optical laser excitation…

Nuclear Experiment · Physics 2018-01-17 Benedict Seiferle , Lars von der Wense , Peter G. Thirolf

A process of the decay of the anomalously low lying nuclear isomer $^{229m}$Th$(3/2^+,8.28 \pm 0.17$ eV) in the Thorium anion (Th$^-$) via the internal conversion (IC) channel is studied. We show that the half life of the nuclear isomer in…

Nuclear Theory · Physics 2020-05-20 E. V. Tkalya , R. Si

The results of experimental studies of the low-energy isomeric state in the $^{229}$Th nucleus are presented. The work is consisted of several stages. During the first stage $^{229}$Th nuclei were excited with the inverse internal…

In the paper, a unique process of the decay of the $^{229m}$Th($3/2^+,8.28\pm 0.17$ eV) low energy nuclear isomer via the internal conversion (IC) channel on Rydberg states is considered for the first time. The Rydberg atom…

Nuclear Theory · Physics 2020-04-30 E. V. Tkalya

Decay spectroscopy of the long-lived states in $^{186}$Tl has been performed at the ISOLDE Decay Station at ISOLDE, CERN. The $\alpha$ decay from the low-spin $(2^-)$ state in $^{186}$Tl was observed for the first time and a half-life of…

Excitation of the anomalously low lying nuclear isomer $^{229m}$Th$(3/2^+, 8.28 \pm 0.17$ eV) in the process of inelastic electron scattering is studied theoretically in the framework of the perturbation theory for the quantum…

Nuclear Theory · Physics 2020-07-01 E. V. Tkalya

We propose a simple approach to measure the energy of the few-eV isomeric state in Th-229. To this end, U-229 nuclei are doped into VUV-transparent crystals, where they undergo alpha decay into Th-229, and, with a probability of 2%,…

Nuclear Experiment · Physics 2016-08-11 Simon Stellmer , Matthias Schreitl , Georgy Kazakov , Johannes Sterba , Thorsten Schumm

$^{\rm {180m}}$Ta is the rarest naturally occurring quasi-stable isotope and the longest lived metastable state which is known. Its possible decay via the $\beta^-$ or the electron capture channel has never been observed. This article…

Nuclear Experiment · Physics 2017-04-12 Björn Lehnert , Mikael Hult , Guillaume Lutter , Kai Zuber

With an expected energy of 7.8(5) eV, the isomeric first excited state in $^{229}$Th exhibits the lowest excitation energy of all known nuclei. Until today, a value for the excitation energy has been inferred only by indirect measurements.…

Instrumentation and Detectors · Physics 2017-08-23 Benedict Seiferle , Lars von der Wense , Peter G. Thirolf

We present a measurement of the low-energy (0--60$\,$keV) $\gamma$ ray spectrum produced in the $\alpha$-decay of $^{233}$U using a dedicated cryogenic magnetic micro-calorimeter. The energy resolution of $\sim$$10\,$eV, together with…

The reduced magnetic dipole and electric quadrupole transition probabilities for the radiative decay of the $^{229}$Th 7.8 eV isomer to the ground state are predicted within a detailed nuclear-structure model approach. We show that the…

Nuclear Theory · Physics 2017-06-13 Nikolay Minkov , Adriana Pálffy

We propose a laser resonance chromatography (LRC) experiment on $^{229}$Th$^{3+}$, with the goal of detecting the ion's electronic ground $5f$ $^2$F$_{5/2}$ state and metastable $7s$ $^2$S$_{1/2}$ state by means of their ion mobilities. To…

The Thorium-229 isotope features a nuclear isomer state with an extremely low energy. The currently most accepted energy value, 7.8 +- 0.5 eV, was obtained from an indirect measurement using a NASA x-ray microcalorimeter with an…

Weak decays in heavy nuclei with charge numbers Z=101-109 are studied within a microscopic formalism based on deformed self-consistent Skyrme Hartree-Fock mean-field calculations with pairing correlations. The half-lives of beta+ decay and…

Nuclear Theory · Physics 2020-11-16 Pedro Sarriguren

The results are presented on the study of the electronic structure of thorium atoms adsorbed by the liquid atomic layer deposition from aqueous solution of thorium nitrate on the surface of CaF2. The chemical state of the atoms and the…

Materials Science · Physics 2017-10-11 P. V. Borisyuk , O. S. Vasilyev , A. V. Krasavin , Yu. Yu. Lebedinskii , V. I. Troyan , E. V. Tkalya

As one of the primordial radioactive isotopes, $^{232}$Th mainly undergoes $\alpha$-decay with a half-life of $1.402 \times 10^{10}$ yr. However, it is also one of 35 double beta decay candidates in which the single $\beta$-decay is…

Nuclear Experiment · Physics 2021-02-03 M. Laubenstein , B. Lehnert , S. S. Nagorny

The physical conditions for the emergence of the extremely low-lying nuclear isomer $^{229m}$Th at approximately 8 eV are investigated in the framework of our recently proposed nuclear structure model. Our theoretical approach explains the…

Nuclear Theory · Physics 2021-02-05 Nikolay Minkov , Adriana Pálffy

Several modes of electroweak radioactive decay require an interaction between the nucleus and bound electrons within the constituent atom. Thus, the probabilities of the respective decays are not only influenced by the structure of the…

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