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We propose a computationally lean, two-stage approach that reliably predicts self-assembly behavior of complex charged molecules on a metallic surfaces under electrochemical conditions. Stage one uses ab initio simulations to provide…

Computational Physics · Physics 2020-07-15 Benedikt Hartl , Shubham Sharma , Oliver Brügner , Stijn F. L. Mertens , Michael Walter , Gerhard Kahl

Quantum computing (or generally, quantum information processing) is of prime interest for it potentially has a significant impact on present electronics and computations1-5. Essence of quantum computing is a direct usage of the…

Quantum Physics · Physics 2007-05-23 S. W. Hwang , D. Y. Jeong , M. S. Jun , M. H. Son , L. W. Engel , J. E. Oh , D. Ahn

We use a simple electrostatic treatment to model recent experiments on quantum Hall systems, in which charging of localised states by addition of integer or fractionally-charged quasiparticles is observed. Treating the localised state as a…

Mesoscale and Nanoscale Physics · Physics 2008-06-17 Ana L. C. Pereira , J. T. Chalker

Surface acoustic waves (SAWs) have been used to transport single electrons across long distances of several hundreds of microns. They can potentially be instrumental in the implementation of scalable quantum processors and quantum…

Design, epitaxial growth, and resonant spectroscopy of CdSe Quantum Dots (QDs) embedded in an innovative (Zn,Cd)Se barrier are presented. The (Zn,Cd)Se barrier enables shifting of QDs energy emission down to 1.87 eV, that is below the…

Mesoscale and Nanoscale Physics · Physics 2016-04-20 J. Piwowar , W. Pacuski , T. Smoleński , M. Goryca , A. Bogucki , A. Golnik , M. Nawrocki , P. Kossacki , J. Suffczyński

Tunnel-coupled pairs of optically active quantum dots - quantum dot molecules (QDMs) - offer the possibility to combine excellent optical properties such as strong light-matter coupling with two-spin singlet-triplet ($S-T_0$) qubits having…

We report on strong renormalization encountered in periodically driven interacting quantum dots in the non-adiabatic regime. Correlations between lead and dot electrons enhance or suppress the amplitude of driving depending on the sign of…

Strongly Correlated Electrons · Physics 2016-01-18 A. K. Eissing , V. Meden , D. M. Kennes

Radiative coupling between quantum emitters leads to a range of spectacular emission phenomena. Dicke studied the foundations of collectively enhanced and suppressed decay, commonly referred to as super- and subradiance. Collective effects…

A Berry phase can be added to the wavefunction of an isolated quantum dot by adiabatically modulating a nonuniform electric field along a time-cycle. The dot is tuned close to a three-level degeneracy, which provides a wide range of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 D. Giuliano , P. Sodano , A. Tagliacozzo

The doped Hubbard model is one of the paradigmatic platforms to engineer exotic quantum many-body states, including charge-ordered states, strange metals and unconventional superconductors. While undoped and doped correlated phases have…

Strongly Correlated Electrons · Physics 2025-02-04 Xin Huang , Jose L. Lado , Jani Sainio , Peter Liljeroth , Somesh Chandra Ganguli

Quantum dots (QDs), embedded in supercapacitors (S-C) cells exhibited capacitance amplification that peaked at certain QD concentration. More than 2.5 peak amplification was demonstrated with cyclic voltammetry (C-V) at a scan rate of 0.1…

Chemical Physics · Physics 2025-08-25 H. Grebel

Ultra-small (r<2 nm) semiconductor quantum dots (QDs) have attracted attention for applications ranging from dye sensitized solar cells to sensing due to its tunable electronic structure and band gap, and large specific surface area.…

Materials Science · Physics 2018-03-14 Bhusankar Talluri , Edamana Prasad , Tiju Thomas

Experiments have shown that pitting corrosion can develop in aluminum surfaces at potentials $> -0.5$ V relative to the standard hydrogen electrode (SHE). Until recently, the onset of pitting corrosion in aluminum has not been rigorously…

Materials Science · Physics 2023-03-29 Quinn Campbell

The unique optical properties of quantum dots (QDs), size-tunable emission and high quantum yield, make them ideal candidates for applications in secure quantum communication, quantum computing, targeted single-cell and molecular tagging,…

Asymmetrical horizontal interdot coupling was demonstrated to exist in a system of a single plane of self-assembled CdTe/ZnTe quantum dots. Photoluminescence excitation (PLE), second order photon correlation and optical orientation were…

Other Condensed Matter · Physics 2009-06-12 T. Kazimierczuk , J. Suffczynski , P. Wojnar , A. Golnik , J. A. Gaj , P. Kossacki

As a model of so-called quantum battery (QB), quantum degrees of freedom as energy storage, we study a charging protocol of a many-body QB consisting of $N$ two-level systems (TLSs) using quantum heat engines (QHEs). We focus on the…

Quantum Physics · Physics 2020-09-25 Kosuke Ito , Gentaro Watanabe

Colloidal quantum dots (QDs) are promising emitters for electroluminescence devices (QD light-emitting-diodes, QLEDs). Though QDs have been synthesized with efficient and stable photoluminescence, inheriting their superior luminescence in…

Applied Physics · Physics 2020-03-18 Chaodan Pu , Xingliang Dai , Yufei Shu , Meiyi Zhu , Yunzhou Deng , Yizheng Jin , Xiaogang Peng

Colloidal semiconductor nanocrystals are promising building blocks for optoelectronics due to their solution processability, spectral tunability, and ability to self-assemble into complex architectures. However, their use in lasing…

A highly-charged spherical colloid in a salt-free environment exerts such a powerful attraction on its counterions that a certain fraction condenses onto the surface of a particle. The degree of condensation depends on the curvature of the…

The investigation of the possibility of optical refrigeration (OR) on zinc-blende cadmium selenide/cadmium sulfide (CdSe/CdS) core/shell structure quantum dots (QDs) has been carried out. Quality samples were synthesized in our lab, and…

Materials Science · Physics 2022-09-14 Muchuan Hua , Ricardo S. Decca