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It has long been believed that doped quantum spin liquids (QSLs) can give rise to fascinating quantum phases, including the possibility of high-temperature superconductivity (SC) as proposed by P. W. Anderson's resonating valence bond (RVB)…

Strongly Correlated Electrons · Physics 2024-04-09 Zheng-Tao Xu , Zheng-Cheng Gu , Shuo Yang

We present the results of muon spin relaxation ($\mu$SR) and neutron scattering on the Ce-based quasikagome lattice CeRh$_{1-x}$Pd$_{x}$Sn ($x=0.1$ to 0.75). Our ZF-$\mu$SR results reveal the absence of static long-range magnetic order down…

A quantum spin liquid (QSL) is an exotic insulating phase with emergent gauge fields and fractionalized excitations. However, the unambiguous demonstration of the existence of a QSL in a "non-engineered" microscopic model (or in any…

Strongly Correlated Electrons · Physics 2025-10-01 Xun Cai , Zhaoyu Han , Zi-Xiang Li , Steven A. Kivelson , Hong Yao

We characterize the ground state and excitation spectrum of the $S=1/2$, nominally pure and perfect kagom\'{e} system ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ using the following measurements: magnetization, muon spin rotation frequency shift $K$,…

Strongly Correlated Electrons · Physics 2007-05-23 Oren Ofer , Amit Keren , Emily A. Nytko , Matthew P. Shores , Bart M. Bartlett , Daniel G. Nocera , Chris Baines , Alex Amato

The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…

Classical spin liquids (CSLs) are intriguing states of matter that do not exhibit long-range magnetic order and are characterized by an extensive ground-state degeneracy. Adding quantum fluctuations, which induce dynamics between these…

Strongly Correlated Electrons · Physics 2025-02-12 Duyu Chen , Rhine Samajdar , Yang Jiao , Salvatore Torquato

A spin-1/2 triangular-lattice antiferromagnet is a prototypical frustrated quantum magnet, which exhibits remarkable quantum many-body effects that arise from the synergy between geometric spin frustration and quantum fluctuations. It can…

Neutron spectroscopy and diffuse neutron scattering on herbertsmithite [ZnCu3 (OH)6Cl2], a near-ideal realisation of the s = 1/2 kagome antiferromagnet, reveal the hallmark property of a quantum spin liquid; instantaneous short-ranged…

Strongly Correlated Electrons · Physics 2009-12-21 M. A. de Vries , J. R. Stewart , P. P. Deen , J. O. Piatek , G. J. Nilsen , H. M. Ronnow , A. Harrison

Continuous spin excitations are widely recognized as one of the hallmarks of novel spin states in quantum magnets, such as quantum spin liquids (QSLs). Here, we report the observation of such kind of excitations in K2Ni2(SO4)3, which…

Spin-liquids -- an emergent, exotic collective phase of matter -- have garnered enormous attention in recent years. While experimentally, many prospective candidates have been proposed and realized, theoretically modeling real materials…

Strongly Correlated Electrons · Physics 2023-08-15 Manas Sajjan , Rishabh Gupta , Sumit Suresh Kale , Vinit Singh , Keerthi Kumaran , Sabre Kais

Rare-earth delafossites were recently proposed as promising candidates for the realization of an effective $S$=1/2 quantum spin liquid (QSL) on the triangular lattice. In contrast to the most actively studied triangular-lattice…

Strongly Correlated Electrons · Physics 2020-01-08 R. Sarkar , Ph. Schlender , V. Grinenko , E. Haeussler , Peter J. Baker , Th. Doert , H. -H. Klauss

In recent work, we argued that a particular algebraic spin liquid (ASL) may be the ground state of the S = 1/2 kagome lattice Heisenberg antiferromagnet. This state, which lacks a spin gap, is appealing in light of recent experiments on…

Strongly Correlated Electrons · Physics 2008-06-10 Michael Hermele , Ying Ran , Patrick A. Lee , Xiao-Gang Wen

The search for quantum spin liquids (QSL) -- topological magnets with fractionalized excitations -- has been a central theme in condensed matter and materials physics. While theories are no longer in short supply, tracking down materials…

Strongly Correlated Electrons · Physics 2022-05-11 Anish Bhardwaj , Shu Zhang , Han Yan , Roderich Moessner , Andriy H. Nevidomskyy , Hitesh J. Changlani

We report a new kagome quantum spin liquid candidate Cu$_3$Zn(OH)$_6$FBr, which does not experience any phase transition down to 50 mK, more than three orders lower than the antiferromagnetic Curie-Weiss temperature ($\sim$ 200 K). A clear…

Kagome lattice Heisenberg antiferromagnets are known to be highly sensitive to perturbations caused by structural disorder. NMR is a local probe ideally suited for investigating such disorder-induced effects, but in practice large…

Strongly Correlated Electrons · Physics 2023-01-09 Weishi Yuan , Jiaming Wang , Philip M. Singer , Rebecca W. Smaha , Jiajia Wen , Young S. Lee , Takashi Imai

Employing large-scale quantum Monte Carlo simulations, we study the extended $XXZ$ model on the kagome lattice. A $\mathbb Z_2$ quantum spin liquid phase with effective even Ising gauge field structure emerges from the delicate balance…

Strongly Correlated Electrons · Physics 2018-08-06 Yan-Cheng Wang , Xue-Feng Zhang , Frank Pollmann , Meng Cheng , Zi Yang Meng

A quantum spin liquid (QSL) arises from a highly entangled superposition of many degenerate classical ground states in a frustrated magnet, and is characterized by emergent gauge fields and deconfined fractionalized excitations (spinons).…

Strongly Correlated Electrons · Physics 2025-06-24 Bin Gao , Félix Desrochers , David W. Tam , Paul Steffens , Arno Hiess , Yixi Su , Sang-Wook Cheong , Yong Baek Kim , Pengcheng Dai

We present measurements on a series of materials, Li$_2$In$_{1-x}$Sc$_x$Mo$_3$O$_8$, that can be described as a 1/6th-filled breathing kagome lattice. Substituting Sc for In generates chemical pressure which alters the breathing parameter…

Strongly Correlated Electrons · Physics 2018-06-06 A. Akbari-Sharbaf , R. Sinclair , A. Verrier , D. Ziat , H. D. Zhou , X. F. Sun , J. A. Quilliam

A quantum spin liquid (QSL) is an exotic state of matter characterized by quantum entanglement and the absence of any broken symmetry. A long-standing open problem, which is a key for fundamental understanding the mysterious QSL states, is…

Nearest-neighbor interacting S = 1/2 spins on the ideal Kagom\'{e} lattice are predicted to form a variety of novel quantum entangled states, including quantum spin-liquid (SL) and valence bond solid (VBS) phases. In real materials, the…

Strongly Correlated Electrons · Physics 2019-10-31 N. J. Laurita , A. Ron , J. W. Han , A. Scheie , J. P. Sheckelton , R. W. Smaha , W. He , J. -J. Wen , J. S. Lee , Y. S. Lee , M. R. Norman , D. Hsieh
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