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We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed…

Strongly Correlated Electrons · Physics 2007-05-23 J. S. Helton , K. Matan , M. P. Shores , E. A. Nytko , B. M. Bartlett , Y. Yoshida , Y. Takano , A. Suslov , Y. Qiu , J. -H. Chung , D. G. Nocera , Y. S. Lee

The emergence of a quantum spin liquid (QSL), a state of matter that can result when electron spins are highly correlated but do not become ordered, has been the subject of a considerable body of research in condensed matter physics. Spin…

It has been suggested that the nearest-neighbour (NN) antiferromagnetic Heisenberg (HAF) model on the Kagome lattice may be a good starting point to understand the quantum spin-liquid (QSL) behaviour discovered in Herbertsmithite. We…

Strongly Correlated Electrons · Physics 2014-01-16 Tyler Dodds , Subhro Bhattacharjee , Yong Baek Kim

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

Strongly Correlated Electrons · Physics 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

Inspired by the recent theoretical suggestion that the random-bond $S=1/2$ antiferromagnetic Heisenberg model on the triangular and the kagome lattices might exhibit a randomness-induced quantum spin liquid (QSL) behavior when the strength…

Strongly Correlated Electrons · Physics 2015-10-28 Tokuro Shimokawa , Ken Watanabe , Hikaru Kawamura

Numerous experiments on pyrochlore oxides Pr$_2$(Zr, Sn, Hf, Ir)$_2$O$_7$ with non-Kramers Pr$^{3+}$ ions suggest that they support a quantum spin liquid (QSL) ground state, but the precise nature of the QSL remains unclear. Quantum spin…

Strongly Correlated Electrons · Physics 2025-12-15 Tony An , Félix Desrochers , Yong Baek Kim

Despite tremendous investigations, a quantum spin liquid state realized in spin-1/2 kagome Heisenberg antiferromagnet remains largely elusive. In herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, a quantum spin liquid candidate on the perfect kagome…

Strongly Correlated Electrons · Physics 2021-06-15 H. Murayama , T. Tominaga , T. Asaba , A. de Oliveira Silva , Y. Sato , H. Suzuki , Y. Ukai , S. Suetsugu , Y. Kasahara , R. Okuma , I. Kimchi , Y. Matsuda

Spin-1/2 kagome-lattice Heisenberg antiferromagnet is theoretically known to have a quantum spin liquid ground state, one of the frontiers of condensed matter physics. The search for the model substances has been continued for a long time,…

Strongly Correlated Electrons · Physics 2024-08-21 Hidekazu Tanaka

We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices---barlowite Cu$_{4}$(OH)$_{6}$FBr. Magnetic susceptibility gives $\theta_{CW}$ = $-$136 K, while long-range order does not happen…

Strongly Correlated Electrons · Physics 2014-12-05 Tian-Heng Han , John Singleton , John A. Schlueter

The rare-earth-based geometrically frustrated triangular magnets have attracted considerable attention due to the intricate interplay between strong spin-orbit coupling and the crystal electric field (CEF), which often leads to effective…

The emergent behavior of spin liquids that are born out of geometrical frustration makes them an intriguing state of matter. We show that in the quantum kagome antiferromagnet ZnCu$_3$(OH)$_6$SO$_4$ several different correlated, yet…

Strongly Correlated Electrons · Physics 2016-03-02 M. Gomilsek , M. Klanjsek , M. Pregelj , F. C. Coomer , H. Luetkens , O. Zaharko , T. Fennell , Y. Li , Q. M. Zhang , A. Zorko

Neutron scattering measurements have been performed on deuterated powder samples of claringbullite and Zn-doped claringbullite (Zn$_x$Cu$_{4-x}$(OD)$_{6}$FCl). At low temperatures, claringbullite Cu$_4$(OD)$_{6}$FCl forms a distorted…

Strongly Correlated Electrons · Physics 2023-01-26 M. Georgopoulou , B. Fåk , D. Boldrin , J. R. Stewart , C. Ritter , E. Suard , J. Ollivier , A. S. Wills

One main theme in current condensed matter physics is the search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature without static order. However, there is no…

Strongly Correlated Electrons · Physics 2023-01-10 Chengpeng Tu , Dongzhe Dai , Xu Zhang , Chengcheng Zhao , Xiaobo Jin , Bin Gao , Tong Chen , Pengcheng Dai , Shiyan Li

Quantum spin liquids (QSLs) represent a novel state where spins are highly entangled but do not order even at zero temperature due to strong quantum fluctuations. Such a state is mostly studied in Heisenberg models defined on geometrically…

Dual-species arrays of ultracold neutral atoms have recently attracted increased interest due to the ability to independently control different atomic species and tune the interatomic interactions. This capability provides additional…

Quantum Physics · Physics 2026-05-06 Ahmed M. Farouk , Ilya I. Beterov , Ghadeer Suliman , Junxi Chen , Igor I. Ryabtsev

We review recent density-matrix renormalization group (DMRG) studies of lightly doped quantum spin liquids (QSLs) on the kagome lattice. While a number of distinct conducting phases, including high-temperature superconductivity, have been…

Strongly Correlated Electrons · Physics 2021-03-16 Cheng Peng , Yi-Fan Jiang , Dong-Ning Sheng , Hong-Chen Jiang

Kagome-lattice materials have attracted tremendous interest due to the broad prospect for seeking superconductivity, quantum spin liquid states, and topological electronic structures. Among them, the transition-metal kagome lattices are…

Strongly Correlated Electrons · Physics 2023-01-02 Tao Xie , Qiangwei Yin , Qi Wang , A. I. Kolesnikov , G. E. Granroth , D. L. Abernathy , Dongliang Gong , Zhiping Yin , Hechang Lei , A. Podlesnyak

Magnetic susceptibility, NMR, muSR, and inelastic neutron scattering measurements show that kapellasite, Cu3Zn(OH)6Cl2, a geometrically frustrated spin-1/2 kagome antiferromagnet polymorphous with the herbertsmithite mineral, is a gapless…

The search for quantum spin liquid (QSL) materials has attracted significant attention in the field of condensed matter physics in recent years, but until now only a handful of them are considered as candidates hosting QSL ground state.…

Strongly Correlated Electrons · Physics 2018-12-17 Zili Feng , Wei Yi , Kejia Zhu , Jie Ma , Jianlin Luo , Shiliang Li , Zi Yang Meng , Youguo Shi

We report measurements of the specific heat and magnetization of single crystal samples of the spin-1/2 kagome compound ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$ (herbertsmithite), a promising quantum spin-liquid candidate, in high magnetic fields and…