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Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the…

Strongly Correlated Electrons · Physics 2016-12-05 M. R. Norman

Quantum spin liquid (QSL) is a novel state of matter which refuses the conventional spin freezing even at 0 K. Experimentally searching for the structurally perfect candidates is a big challenge in condensed matter physics. Here we report…

The nature of quantum spin liquids is studied for the spin-$1/2$ antiferromagnetic Heisenberg model on a square lattice containing exchange interactions between nearest-neighbor sites, $J_1$, and those between next-nearest-neighbor sites,…

Strongly Correlated Electrons · Physics 2015-02-02 Satoshi Morita , Ryui Kaneko , Masatoshi Imada

Motivated by the recent experiments on the new spin half Kagome compound ZnCu3(OH)6Cl2, we study a phenomenological model of a frustrated quantum magnet. The model has a spin liquid groundstate and is constructed so as to mimic the…

Strongly Correlated Electrons · Physics 2009-11-13 R. Chitra , M. J. Rozenberg

The spin-1/2 kagom\'{e} Heisenberg antiferromagnet is generally accepted as one of the most promising two-dimensional models to realize a quantum spin liquid state. Previous experimental efforts were almost exclusively on only one…

Strongly Correlated Electrons · Physics 2022-12-28 Xiaochen Hong , Mahdi Behnami , Long Yuan , Boqiang Li , Wolfram Brenig , Bernd Büchner , Yuesheng Li , Christian Hess

The Kagome-lattice-based material, Volborthite, $\mathrm{Cu_3 V_2 O_7 (OH)_2 \cdot 2 H_2 O}$, has been considered as a promising platform for discovery of unusual quantum ground states due to the frustrated nature of spin interactions. Here…

Strongly Correlated Electrons · Physics 2017-07-19 Li Ern Chern , Kyusung Hwang , Tomonari Mizoguchi , Yejin Huh , Yong Baek Kim

We investigate the lattice dynamics in the spin-1/2 frustrated kagome compound herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ by a combination of infrared spectroscopy measurements and ab initio density functional theory calculations, and provide…

Strongly Correlated Electrons · Physics 2020-04-29 Ying Li , A. Pustogow , M. Bories , P. Puphal , C. Krellner , M. Dressel , Roser Valenti

We argue that a relatively simple model containing only SU(2)-invariant chiral three-spin interactions on a Kagome lattice of S=1/2 spins can give rise to both a gapped and a gapless quantum spin liquid. Our arguments are rooted in a…

Strongly Correlated Electrons · Physics 2014-09-09 Bela Bauer , Brendan P. Keller , Michele Dolfi , Simon Trebst , Andreas W. W. Ludwig

Quantum spin liquids represent exotic states of spin systems characterized by long-range entanglement and emergent fractionalized quasiparticles. It is generally believed that disorder is hostile to quantum spin liquids. In our study, we…

Strongly Correlated Electrons · Physics 2024-08-30 Aini Xu , Qinxin Shen , Bo Liu , Zhenyuan Zeng , Lankun Han , Liqin Yan , Jun Luo , Jie Yang , Rui Zhou , Shiliang Li

The search of quantum spin liquid (QSL), an exotic magnetic state with strongly-fluctuating and highly-entangled spins down to zero temperature, is a main theme in current condensed matter physics. However, there is no smoking-gun evidence…

Strongly Correlated Electrons · Physics 2023-10-27 Z. H. Zhu , B. L. Pan , L. P. Nie , J. M. Ni , Y. X. Yang , C. S. Chen , Y. Y. Huang , E. J. Cheng , Y. J. Yu , A. D. Hillier , X. H. Chen , T. Wu , Y. Zhou , S. Y. Li , L. Shu

A Z2 quantum spin liquid hosts one of the simplest topological orders and exhibits many exotic properties due to long-range quantum entanglements. Its elementary excitations are anyons such as spinons carrying fractionalized spin quantum…

Magnetic excitations in the spin-$\frac{1}{2}$ distorted kagome lattice antiferromagnet Cs$_2$Cu$_3$SnF$_{12}$, which has an ordered ground state owing to the strong Dzyaloshinskii-Moriya interaction, were studied using inelastic neutron…

Strongly Correlated Electrons · Physics 2017-02-17 T. Ono , K. Matan , Y. Nambu , T. J. Sato , K. Katayama , S. Hirata , H. Tanaka

Quantum spin liquids (QSLs) are long-range entangled phases of frustrated magnets exhibiting fractionalized spin excitations. In two dimensions, there is limited analytical understanding of their excitation spectra beyond parton mean-field…

Strongly Correlated Electrons · Physics 2025-08-01 Josef Willsher , Johannes Knolle

A novel cuprate Volborthite, Cu3V2O7(OH)2-2H2O, containing an S-1/2 (Cu 2+ spin) kagome-like lattice is studied by magnetic susceptibility, specific heat, and 51 V NMR measurements. Signs for neither long-range order nor spin-gapped singlet…

Strongly Correlated Electrons · Physics 2009-11-07 Z. Hiroi , M. Hanawa , N. Kobayashi , M. Nohara , H. Takagi , Y. Kato , M. Takigawa

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

Strongly Correlated Electrons · Physics 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

In the vanadium oxyfluoride compound (NH$_4$)$_2$[C$_7$H$_{14}$N][V$_7$O$_6$F$_{18}$] (DQVOF), the V$^{4+}$ (3d$^1$, $S=1/2$) ions realize a unique, highly frustrated breathing kagome lattice composed of alternately-sized, corner-sharing…

Strongly Correlated Electrons · Physics 2017-06-19 J. -C. Orain , B. Bernu , P. Mendels , L. Clark , F. H. Aidoudi , P. Lightfoot , R. E. Morris , F. Bert

A glance at recent research on magnetism turns up a curious set of articles discussing, or claiming evidence for, a state of matter called a quantum spin liquid (QSL). These articles are notable in their invocation of exotic notions of…

Strongly Correlated Electrons · Physics 2023-10-31 T. Lancaster

Quantum spin liquid is an elusive state that display strong many-body entanglement with potential applications in future quantum computing. This study reports muon spin relaxation ($\mu^+$SR) measurements on a novel high-pressure…

Na$_4$Ir$_3$O$_8$ provides a material platform to study three-dimensional quantum spin liquids in the geometrically frustrated hyperkagome lattice of Ir$^{4+}$ ions. In this work, we consider quantum spin liquids on hyperkagome lattice for…

Strongly Correlated Electrons · Physics 2017-02-03 Biao Huang , Yong Baek Kim , Yuan-Ming Lu

Low energy inelastic neutron scattering on single crystals of the kagome spin liquid compound ZnCu3(OD)6Cl2 (Herbertsmithite) reveals antiferromagnetic correlations between impurity spins for energy transfers E < 0.8 meV (~J/20). The…

Strongly Correlated Electrons · Physics 2016-08-24 Tian-Heng Han , M. R. Norman , J. -J. Wen , Jose A. Rodriguez-Rivera , Joel S. Helton , Collin Broholm , Young S. Lee