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Related papers: A Guide to Molecular Properties from the Bethe-Sal…

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The Bethe-Salpeter equation is a widely used approach to describe optical excitations in bulk semiconductors. It leads to spectra that are in very good agreement with experiment, but the price to pay for such accuracy is a very high…

The structural properties of liquid GeSe$_2$ are studied by using first-principles molecular dynamics in conjuncton with the Becke, Lee, Yang and Parr (BLYP) generalized gradient approximation for the exchange and correlation energy. The…

Materials Science · Physics 2015-05-13 M. Micoulaut , R. Vuilleumier , C. Massobrio

Like adiabatic time-dependent density-functional theory (TD-DFT), the Bethe-Salpeter equation (BSE) formalism of many-body perturbation theory, in its static approximation, is "blind" to double (and higher) excitations, which are…

Chemical Physics · Physics 2021-06-14 Enzo Monino , Pierre-François Loos

We develop a time dependent second order Green's function theory (GF2) for calculating neutral excited states in molecules. The equation of motion for the lesser Green's function (GF) is derived within the adiabatic approximation to the…

Chemical Physics · Physics 2022-01-19 Wenjie Dou , Joonho Lee , David R. Reichman , Roi Baer , Eran Rabani

First principles calculations based on many-electron perturbation theory methods, such as the \textit{ab initio} GW and GW plus Bethe-Salpeter equation (GW-BSE) approach, are reliable ways to predict quasiparticle and optical properties of…

Materials Science · Physics 2017-01-11 Felipe H. da Jornada , Diana Y. Qiu , Steven G. Louie

We describe an all-electron implementation of the Bethe-Salpeter equation (BSE) for the calculation of optical absorption spectra in the full-potential linearized augmented-plane-wave (FLAPW) method. So far, FLAPW implementations have…

Materials Science · Physics 2026-03-27 Jörn Stöhler , Stefan Blügel , Christoph Friedrich

It is known that binding energies calculated from the Bethe-Salpeter equation in ladder approximation can be reasonably well accounted for by an energy-dependent interaction, at least for the lowest states. It is also known that none of…

Nuclear Theory · Physics 2009-11-06 A. Amghar , B. Desplanques , L. Theussl

A time-dependent formulation for electron-hole excitations in extended finite systems, based on the Bethe-Salpeter equation (BSE), is developed using a stochastic wave function approach. The time-dependent formulation builds on the…

Materials Science · Physics 2015-02-11 Eran Rabani , Roi Baer , Daniel Neuhauser

Interactions in atomic and molecular systems are dominated by electromagnetic forces and the theoretical framework must be in the quantum regime. The physical theory for the combination of quantum mechanics and electromagnetism, quantum…

Chemical Physics · Physics 2023-01-26 Edit Mátyus , Dávid Ferenc , Péter Jeszenszki , Ádám Margócsy

This work is an extension of the work in \cite{bhatnagar18} to ground and excited states of $0^{++}, 0^{-+}$, and $1^{--}$ of heavy-light ($c\overline{u}, c\overline{s}, b\overline{u}, b\overline{s}$, and $b\overline{c}$) quarkonia in the…

High Energy Physics - Phenomenology · Physics 2019-10-02 Eshete Gebrehana , Shashank Bhatnagar , Hluf Negash

We report on the use of the adaptively compressed exchange (ACE) operator to accelerate many-body perturbation theory (MBPT) calculations, including G$_0$W$_0$ and the Bethe Salpeter equation (BSE), for hybrid density functional theory…

Materials Science · Physics 2025-07-17 Victor Wen-zhe Yu , Marco Govoni

We present a simple and accurate GW implementation based on a combination of a Laplace transformation (LT) and other acceleration techniques used in post-SCF quantum chemistry, namely, natural auxiliary functions and the frozen-core…

Chemical Physics · Physics 2023-11-16 Johannes Tölle , Niklas Niemeyer , Johannes Neugebauer

We present an ab initio many-body theory of optical activity in solids within the GW-BSE framework. Dielectric spatial dispersion is formulated in two complementary forms: exciton envelope modulation and sum-over-exciton-states expansion.…

Materials Science · Physics 2026-05-13 Xiaoming Wang , Yanfa Yan

We provide an in-depth examination of the $GW$ approximation of Green's function many-body perturbation theory by detailing both its theoretical and practical aspects in the realm of quantum chemistry. First, the quasiparticle context is…

Chemical Physics · Physics 2024-03-20 Antoine Marie , Abdallah Ammar , Pierre-François Loos

We develop an improved stochastic formalism for the Bethe-Salpeter equation, based on an exact separation of the effective-interaction $W$ to two parts, $W=(W-v_W)+v_W$ where the latter is formally any translationally-invariant interaction…

Chemical Physics · Physics 2023-05-03 Nadine C. Bradbury , Tucker Allen , Minh Nguyen , Khaled Ibrahim , Daniel Neuhauser

In this review we demonstrate how the algebraic Bethe ansatz is used for the calculation of the energy spectra and form factors (operator matrix elements in the basis of Hamiltonian eigenstates) in exactly solvable quantum systems. As…

Exactly Solvable and Integrable Systems · Physics 2009-11-10 J. Links , H. -Q. Zhou , R. H. McKenzie , M. D. Gould

A new scheme has been proposed to solve the B.E. condenstates in terms of Green's function approach. It has been shown that the radial wave function of two interacting atoms, moving in a common harmonic oscillator potential modified by an…

Quantum Physics · Physics 2007-05-23 Mahendra Sinha Roy

The problem of calculating of the mass spectrum of the two-body Bethe-Salpeter equation is studied with no reduction to the three-dimensional ("quasipotential") equation. The method to find the ground state and excited states for a channel…

High Energy Physics - Phenomenology · Physics 2015-06-25 A. Yu. Umnikov , F. C. Khanna

The correlation energy of the homogeneous electron gas is evaluated by solving the Bethe-Salpeter equation (BSE) beyond the Tamm-Dancoff approximation for the electronic polarisation propagator. The BSE is expected to improve upon the…

Materials Science · Physics 2016-06-15 Emanuele Maggio , Georg Kresse

Ground State Energy Estimation (GSEE) is a central problem in quantum chemistry and condensed matter physics, demanding efficient algorithms to solve complex electronic structure calculations. This work introduces a structured benchmarking…