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Related papers: Robust spin-orbit coupling in semi-metallic SrIrO3…

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Sr$_{2}$IrO$_{4}$ has often been described via a simple, one-band pseudo-spin 1/2 model, subject to electron-electron interactions, on a square lattice, fostering analogies with cuprate superconductors, believed to be well described by a…

We investigate the metal-insulator transition in the layered Ruddelsden Popper series of strontium iridates Srn+1IrnO3n+1. Tight-binding models of t2g orbitals for n = 1, 2, and infinity are constructed, and changes in band dispersion due…

Strongly Correlated Electrons · Physics 2015-06-05 Jean-Michel Carter , V. Vijay Shankar , Hae-Young Kee

The unusual magnetic and electronic ground states of 5d iridates has been shown to be driven by intrinsically enhanced spin-orbit coupling (SOC). The influence of appreciable but reduced SOC in creating the manifested magnetic insulating…

Strongly Correlated Electrons · Physics 2015-12-01 S. Calder , L. Li , S. Okamoto , Y. Choi , R. Mukherjee , D. Haskel , D. Mandrus

Orthorhombic SrIrO3 is a typical spin-orbit-coupling correlated metal that shows diversified physical properties under the external stimuli. Here nonlinear Hall effect and weakly temperature-dependent resistance are observed in a SrIrO3…

Perovskite SrIrO3 has long been proposed as an exotic semimetal induced by the interplay between the spin-orbit coupling and electron correlations. However, its low-lying electronic structure is still lacking. We synthesize high-quality…

Strongly Correlated Electrons · Physics 2016-08-03 Z. T. Liu , M. Y. Li , Q. F. Li , J. S. Liu , W. Li , H. F. Yang , Q. Yao , C. C. Fan , X. G. Wan , Z. Wang , D. W. Shen

Iridate oxides display exotic physical properties that arise from the interplay between a large spin-orbit coupling and electron correlations. Here, we present a comprehensive study of the effects of hydrostatic pressure on the electronic…

Strongly Correlated Electrons · Physics 2020-04-21 A. G. Zaitsev , A. Beck , A. K. Jaiswal , R. Singh , R. Schneider , M. Le Tacon , D. Fuchs

We employ reactive molecular-beam epitaxy to synthesize the metastable perovskite SrIrO$_{3}$ and utilize {\it in situ} angle-resolved photoemission to reveal its electronic structure as an exotic narrow-band semimetal. We discover…

Strongly Correlated Electrons · Physics 2015-01-13 Y. F. Nie , P. D. C. King , C. H. Kim , M. Uchida , H. I. Wei , B. D. Faeth , J. P. Ruf , J. P. C. Ruff , L. Xie , X. Pan , C. J. Fennie , D. G. Schlom , K. M. Shen

Perovskite-type iridates SrIrO$_{3}$ and CaIrO$_{3}$ are a Dirac line node semimetal protected by crystalline symmetry, providing an interesting playground to investigate electron correlation effects on topological semimetals. The effect of…

Strongly Correlated Electrons · Physics 2019-11-14 Masamichi Negishi , Naoka Hiraoka , Daisuke Nishio-Hamane , Hidenori Takagi

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

Strongly Correlated Electrons · Physics 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

Iridates abound with interesting magnetic behaviours because of their strong spin-orbit coupling. Sr$_3$NiIrO$_6$ brings together the spin-orbital entanglement of the Ir$^{4+}$ ion with a 3$d$ Ni cation and a one-dimensional crystal…

Materials Science · Physics 2018-10-19 Turan Birol , Kristjan Haule , David Vanderbilt

The electronic and magnetic properties of monoclinic double perovskite Sr$_2$CeIrO$_6$ were examined based on both experiments and first-principles density functional theory calculations. From the calculations we conclude that…

Materials Science · Physics 2016-07-13 Sudipta Kanungo , Kailash Mogare , Binghai Yan , Claudia Felser , Martin Jansen

Recent theoretical studies of topologically nontrivial electronic states in Kondo insulators have pointed to the importance of spin-orbit coupling (SOC) for stabilizing these states. However, systematic experimental studies that tune the…

Strongly Correlated Electrons · Physics 2017-06-19 S. Dzsaber , L. Prochaska , A. Sidorenko , G. Eguchi , R. Svagera , M. Waas , A. Prokofiev , Q. Si , S. Paschen

We have studied in detail the electronic structure of IrO$_2$ including spin-orbit coupling (SOC) and electron-electron interaction, both within the GGA+U and GGA+DMFT approximations. Our calculations reveal that the Ir t$_{2g}$ states at…

Strongly Correlated Electrons · Physics 2014-04-25 S. K. Panda , S. Bhowal , A. Delin , O. Eriksson , I. Dasgupta

A burning question in the emerging field of spin-orbit driven insulating iridates, such as Na2IrO3 and Li2IrO3 is whether the observed insulating state should be classified as a Mott-Hubbard insulator derived from a half-filled relativistic…

Strongly Correlated Electrons · Physics 2014-01-31 I. I. Mazin , S. Manni , K. Foyevtsova , Harald O. Jeschke , P. Gegenwart , Roser Valenti

We report a magnetotransport study of spin relaxation in 1.4-21.2 nm epitaxial SrIrO$_3$ thin films coherently strained on SrTiO$_3$ substrates. Fully charge compensated semimetallic transport has been observed in SrIrO$_3$ films thicker…

Strongly Correlated Electrons · Physics 2020-06-16 L. Zhang , X. Jiang , X. Xu , X. Hong

Recent theory and experiment have revealed that strong spin-orbit coupling can have dramatic qualitative effects on the band structure of weakly interacting solids. Indeed, it leads to a distinct phase of matter, the topological band…

Strongly Correlated Electrons · Physics 2015-05-13 D. A. Pesin , Leon Balents

We present the main features of the spin-orbital superexchange which describes the magnetic and optical properties of Mott insulators with orbital degrees of freedom. In contrast to the SU(2) symmetry of spin superexchange, the orbital part…

Strongly Correlated Electrons · Physics 2022-01-25 Andrzej M. Oles

We have carried out a detailed first-principles study of a d$^{4.5}$ quaternary iridate Ba$_3$YIr$_2$O$_9$ both in its 6H-perovskite-type ambient pressure (AP) phase and also for the high pressure (HP) cubic phase. Our analysis reveals that…

Strongly Correlated Electrons · Physics 2015-11-11 S. K. Panda , S. Bhowal , Ying Li , S. Ganguly , Roser Valentí , L. L. Nordström , I. Dasgupta

We have studied the electronic structure of BaCoO$_3$ using soft x-ray absorption spectroscopy at the Co-$L_{2,3}$ and O-$K$ edges, magnetic circular dichroism at the Co-$L_{2,3}$ edges, as well as valence band hard x-ray photoelectron…

We have systematically investigated substrate-strain effects on the electronic structures of two representative Sr-iridates, a correlated-insulator Sr$_2$IrO$_4$ and a metal SrIrO$_3$. Optical conductivities obtained by the \emph{ab initio}…

Materials Science · Physics 2016-06-07 Bongjae Kim , Beom Hyun Kim , Kyoo Kim , B. I. Min