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When laser radiation is skilfully applied, atoms and molecules can be cooled allowing precise measurements and control of quantum systems. This is essential in fundamental studies of physics as well as practical applications such as…

Laser cooling by collisional redistribution of radiation has been successfully applied in the past for cooling dense atomic gases. Here we report on progress of work aiming at the demonstration of redistribution laser cooling in a molecular…

Atomic Physics · Physics 2013-03-22 Philipp Simon , Peter Moroshkin , Lars Weller , Anne Sass , Martin Weitz

A cryogenic buffer gas beam, an electrostatic hexapole lens, and 2D transverse Doppler laser cooling are combined to produce a bright beam of barium monofluoride ($^{138}$Ba$^{19}$F) molecules. Experimental results and trajectory…

In this review, we discuss the impact of the development of lasers on ultracold atoms and molecules and their applications. After a brief historical review of laser cooling and Bose-Einstein condensation, we present important applications…

We propose a new laser cooling method for atomic species whose level structure makes traditional laser cooling difficult. For instance, laser cooling of hydrogen requires vacuum-ultraviolet laser light, while multielectron atoms need laser…

Quantum Physics · Physics 2009-11-10 David Kielpinski

Herein, we show that single molecules containing multiple optical cycling centers (CaO moieties) can exhibit superradiant phenomena. We demonstrate the accuracy of the Frenkel exciton model at describing these superradiant states via…

Laser cooling of molecules employing broadband optical pumping involves a timescale separation between laser excitation and spontaneous emission. Here, we optimize the optical pumping step using shaped laser pulses. We derive two…

Quantum Physics · Physics 2013-12-24 Daniel M. Reich , Christiane P. Koch

We investigate the microwave spectra of ultracold alkali metal dimers in magnetic, electric and combined fields, taking account of the hyperfine structure due to the nuclear spins. We consider the molecules 41K87Rb and 7Li133Cs, which are…

Chemical Physics · Physics 2015-05-14 Hong Ran , J. Aldegunde , Jeremy M. Hutson

Narrow line laser cooling is advancing the frontier for experiments ranging from studies of fundamental atomic physics to high precision optical frequency standards. In this paper, we present an extensive description of the systems and…

Atomic Physics · Physics 2009-11-10 Thomas H. Loftus , Tetsuya Ido , Martin M. Boyd , Andrew D. Ludlow , Jun Ye

Precision spectroscopic measurements in atoms and molecules play an increasingly important role in chemistry and physics, e.g., to characterize structure and dynamics at long timescales, to determine physical constants, or to search for…

We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…

Atomic Physics · Physics 2017-09-13 Chien-Yu Lien , Scott R. Williams , Brian Odom

Aluminium monofluoride (AlF) is a promising candidate for laser cooling and trapping at high densities. We show efficient production of AlF in a bright, pulsed cryogenic buffer gas beam, and demonstrate rapid optical cycling on the Q…

In order to realize more sensitive eEDM measurement, it would be worthwhile to find some new laser-cooled molecules with larger internal effective electric field (E$_{eff}$), higher electric polarizability and longer lifetime of the eEDM…

Atomic Physics · Physics 2019-03-13 Zhenghai Yang , Jing Li , Qinning Lin , Liang Xu , Hailing Wang , Tao Yang , Jianping Yin

Cooling atoms to the ground-state of optical tweezers is becoming increasingly important for high-fidelity imaging, cooling, and molecular assembly. While extensive theoretical work has been conducted on cooling in free space, fewer studies…

We propose a cavity based laser cooling and trapping scheme, providing tight confinement and cooling to very low temperatures, without degradation at high particle densities. A bidirectionally pumped ring cavity builds up a resonantly…

Quantum Physics · Physics 2009-11-10 Th. Elsaesser , B. Nagorny , A. Hemmerich

Cooling down a trapped ion into its motional ground state is a central step for trapped ions based quantum information processing. State of the art cooling schemes often work under a set of optimal cooling conditions derived analytically…

Quantum Physics · Physics 2021-10-12 Xie-Qian Li , Shuo Zhang , Jie Zhang , Wei Wu , Chu Guo , Ping-Xing Chen

We have achieved stimulated laser cooling of thermal rubidium atomic beams on a silicon chip. Following pre-collimation via a silicon microchannel array, we perform beam brightening via a blue-detuned optical molasses. Owing to the small…

Atomic Physics · Physics 2023-09-20 Chao Li , Xiao Chai , Linzhao Zhuo , Bochao Wei , Ardalan Lotfi , Farrokh Ayazi , Chandra Raman

Parallel to advances in laser cooling of atoms and ions in dilute gas phase, which has progressed immensely, resulting in physics Nobel prizes in 1997 and 2001, major progress has recently been made in laser cooling of solids. I compare the…

Optics · Physics 2015-05-13 Galina Nemova

Frequency domain super-heterodyne laser light scattering is utilized in a low angle integral measurement configuration to determine flow and diffusion in charged sphere suspensions showing moderate to strong multiple scattering. We…

Molecular ions can be held in a chain of laser-cooled atomic ions by sympathetic cooling. This system is ideal for performing high-precision molecular spectroscopy with applications in astrochemistry and fundamental physics. Here we show…

Atomic Physics · Physics 2015-08-20 Ncamiso B. Khanyile , Gang Shu , Kenneth R. Brown