Laser cooling with ultrafast pulse trains

We propose a new laser cooling method for atomic species whose level structure makes traditional laser cooling difficult. For instance, laser cooling of hydrogen requires vacuum-ultraviolet laser light, while multielectron atoms need laser light at many widely separated frequencies. These restrictions can be eased by laser cooling on two-photon transitions with ultrafast pulse trains. Laser cooling of hydrogen, antihydrogen, and carbon appears feasible, and extension of the technique to molecules may be possible.