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We present the first experimental demonstration of radiation pressure force deflection and direct laser cooling for barium monohydride (BaH) molecules resulting from multiple photon scattering. Despite a small recoil velocity (2.7 mm/s) and…

This paper reviews the recent results in high-resolution spectroscopy on cold molecules. Laser spectroscopy of cold molecules addresses issues of symmetry violation, like in the search for the electric dipole moment of the electron and the…

Atomic Physics · Physics 2016-07-05 Simone Borri , Gabriele Santambrogio

The helium dimer in its metastable triplet state is a promising candidate to be the first laser-cooled homonuclear molecule. An ultracold gas of He$_2^*$ would enable a new generation of precision measurements to test quantum…

Atomic Physics · Physics 2025-05-22 Lucía Verdegay , Bingcheng Zeng , Daniel Y. Knapp , Jack C. Roth , Maximilian Beyer

Recent theoretical investigations have indicated that rapid optical cycling should be feasible in complex polyatomic molecules with diverse constituents, geometries and symmetries. However, as a composite molecular mass grows, so does the…

Atomic Physics · Physics 2020-12-18 Konrad Wenz , Ivan Kozyryev , Rees L. McNally , Leland Aldridge , Tanya Zelevinsky

Precision measurements in molecules have advanced rapidly in recent years through developments in techniques to cool, trap, and control. The complexity of molecules makes them a challenge to study, but also offers opportunities for enhanced…

Atomic Physics · Physics 2021-01-15 Nicholas R. Hutzler

We propose to extend coherent laser cooling from narrow-band to broad-band transitions by using trains of ultrashort broadband pulses. We study analytically two possible methods to reduce the momentum spread of a distribution by several…

Only bosonic molecular species have been directly laser cooled to date, primarily due to an abundance of bosonic isotopes in nature and to their simpler hyperfine structure. Fermionic molecules provide new opportunities for ultracold…

Atomic Physics · Physics 2024-08-07 Jinyu Dai , Qi Sun , Benjamin C. Riley , Debayan Mitra , Tanya Zelevinsky

For experiments that require a quantum system to be in the ultra-cold regime, laser cooling is an essential tool. While techniques for laser cooling ions and neutral atoms have been refined and temperatures below the Doppler limit have been…

Atomic Physics · Physics 2024-10-31 Caleb Heuvel-Horwitz , S. F. Yelin

Cooling the rotation and the vibration of molecules by broadband light sources was possible for trapped molecular ions or ultracold molecules. Because of a low power spectral density, the cooling timescale has never fell below than a few…

Atomic Physics · Physics 2018-06-06 A. Cournol , P. Pillet , H. Lignier , D. Comparat

Since the first proof-of-concept demonstrations of photoluminescence-based optical refrigeration, solid-state laser cooling has developed into a credible competitor to conventional cryogenic technologies. Solid-state laser cooling continues…

Mass spectrometry is used in a wide range of scientific disciplines including proteomics, pharmaceutics, forensics, and fundamental physics and chemistry. Given this ubiquity, there is a worldwide effort to improve the efficiency and…

We have recently demonstrated that optical pumping methods combined with photoassociation of ultra-cold atoms can produce ultra-cold and dense samples of molecules in their absolute rovibronic ground state. More generally, both the external…

Atomic Physics · Physics 2013-08-01 I. Manai , R. Horchani , M. Hamamda , A. Fioretti , M. Allegrini , H. Lignier , P. Pillet , D. Comparat

We describe a simple experimental apparatus for laser ablation of barium monohydride (BaH) molecules and the study of their rovibrational spectra that are relevant to direct laser cooling. We present a detailed analysis of the properties of…

Atomic Physics · Physics 2016-03-23 M. G. Tarallo , G. Z. Iwata , T. Zelevinsky

We investigate laser cooling of an ensemble of atoms in an optical cavity. We demonstrate that when atomic dipoles are sychronized in the regime of steady-state superradiance, the motion of the atoms may be subject to a giant frictional…

Quantum Physics · Physics 2016-04-20 Minghui Xu , Simon B. Jäger , S. Schütz , J. Cooper , Giovanna Morigi , M. J. Holland

Some practical improvements are proposed for the "optical-shaker" laser-cooling technique [I.S. Averbukh and Y. Prior, Phys. Rev. Lett. 94, 153002 (2005)]. The improved technique results in an increased cooling rate and decreases the…

Atomic Physics · Physics 2009-01-14 Louis Marmet

Sideband cooling is a popular method for cooling atoms to the ground state of an optical trap. Applying the same method to molecules requires a number of challenges to be overcome. Strong tensor Stark shifts in molecules cause the optical…

Atomic Physics · Physics 2020-03-11 L. Caldwell , M. R. Tarbutt

A method of electron beam cooling is considered which can be used for linear colliders. The electron beam is cooled during collision with focused powerful laser pulse. The ultimate transverse emittances are much below those achievable by…

High Energy Physics - Experiment · Physics 2009-10-31 Valery Telnov

The particular advantages of using the diatomic molecule radium monofluoride (RaF) as a versatile molecular probe for physics beyond the Standard Model are highlighted. i) RaF was previously suggested as being potentially amenable to direct…

Chemical Physics · Physics 2020-05-25 T. A. Isaev , R. Berger

The initialization of nuclear spin to its ground state is challenging due to its small energy scale compared with thermal energy, even at cryogenic temperature. In this Letter, we propose an opto-nuclear quadrupolar effect, whereby…

Quantum Physics · Physics 2023-03-02 Haowei Xu , Guoqing Wang , Changhao Li , Hua Wang , Hao Tang , Ariel Rebekah Barr , Paola Cappellaro , Ju Li

Optical lattices have emerged as ideal simulators for Hubbard models of strongly correlated materials, such as the high-temperature superconducting cuprates. In optical lattice experiments, microscopic parameters such as the interaction…

Quantum Gases · Physics 2011-06-23 D. McKay , B. DeMarco