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In single-junction photovoltaic (PV) devices, the maximum achievable power conversion efficiency (PCE) is mainly limited by thermalization and transmission losses, because polychromatic solar irradiation cannot be matched to a single…

The quantum efficiencies (QE) of photocathodes consisting of bulk Nb substrates coated with thin films of Cs2Te are reported. Using the standard recipe for Cs2Te deposition developed for Mo substrates (220 {\AA} Te thickness), a QE ~11% -…

We use temperature- and field-dependent resistivity measurements [Shubnikov--de Haas (SdH) quantum oscillations] and ultrahigh resolution, tunable, vacuum ultraviolet (VUV) laser-based angle-resolved photoemission spectroscopy (ARPES) to…

Materials Science · Physics 2017-05-24 Yun Wu , Na Hyun Jo , Daixiang Mou , Lunan Huang , S. L. Bud'ko , P. C. Canfield , Adam Kaminski

Phase change materials (PCMs) have long been used as a storage medium in rewritable compact disk and later in random access memory. In recent years, the integration of PCMs with nanophotonic structures has introduced a new paradigm for…

Panchromatic absorbing materials are widely regarded as a key strategy for enhancing solar energy utilization and photocurrent generation. However, in artificial molecular systems, broadening the absorption spectrum is often accompanied by…

Chemical Physics · Physics 2026-01-01 Hsien-Hsin Chou

In this article the Wells-Dawson polyoxometalate K6[P2W18O62] is grown as an interfacial layer between indium tin oxide and bulk heterojunction of poly(3-hexylthiophene) (P3HT) and [6,6]-phenyl-C61-butyric acid methyl ester (PCBM). The…

Applied Physics · Physics 2018-06-08 M. Alaaeddine , Q. Zhu , D. Fichou , G. Izzet , J. E. Rault , N. Barrett , A. Proust , L. Tortech

InSe is a promising material for a next-generation of two-dimensional electronic and optical devices, characteristics of which are largely determined by the type of band structure, direct or indirect. In general, different methods can be…

Two-dimensional crystals stack together through weak van der Waals (vdW) forces, offering unlimited possibilities to play with layer number, order and twist angle in vdW heterostructures (HSs). The realisation of high-performance…

Currently, Sb$_2$Se$_3$ thin films receive considerable research interest as a solar cell absorber material. When completed into a device stack, the major bottleneck for further device improvement is the open circuit voltage, which is the…

Among several solutions to exploit solar energy, thermophotovoltaics (TPV) have been popularized and have known great breakthroughs during the past two decades. Yet, existing systems still have low efficiencies since the wavelength range of…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Elyes Nefzaoui , Jérémie Drevillon , Karl Joulain

We have fabricated black phosphorus photodetectors and characterized their full spectral responsivity. These devices, which are effectively in the bulk thin film limit, show broadband responsivity ranging from <400 nm to the ~3.8 $\mu$m…

Metal mono-chalcogenide compounds offer a large variety of electronic properties depending on chemical composition, number of layers and stacking-order. Among them, the InSe has attracted much attention due to the promise of outstanding…

Tunable photovoltaic photodetectors are of significant relevance in the fields of programmable and neuromorphic optoelectronics. However, their widespread adoption is hindered by intricate architectural design and energy consumption…

Mesoscale and Nanoscale Physics · Physics 2023-12-12 Fan Liu , Xi Lin , Yuting Yan , Xuetao Gan , Yingchun Cheng , Xiaoguang Luo

In this report, we describe a large-area Laser Beam Induced Current (LBIC) microscope that has been adapted to perform Intensity Modulated Photocurrent Spectroscopy in an imaging mode combined with automated J-V electrical characterization.…

Instrumentation and Detectors · Physics 2022-04-26 Jamie Laird , Sandheep Ravishankar , Askhkat Jumabekov , Kevin Rietwyk , Wenxin Mao , Udo Bach , Trevor Smith

Two-dimensional (2D) ferroelectric (FE) materials offer a large variety of electronic properties depending on chemical composition, number of layers and stacking-order. Among them, alpha-In2Se3 has attracted much attention due to the…

Electron beam induced current (EBIC) is a powerful technique which measures the charge collection efficiency of photovoltaics with sub-micron spatial resolution. The exciting electron beam results in a high generation rate density of…

Materials Science · Physics 2014-10-17 Paul M. Haney , Heayoung P. Yoon , Prakash Koirala , Robert W. Collins , Nikolai B. Zhitenev

Silicon indirect bandgap fundamentally limits its ability to emit light, hindering the development of silicon-based light sources. Here, we explore a conceptually new solution to this long-standing challenge. We demonstrate ultrabroadband…

In this work we address the microscopic effects related to the implementation of a Bathophenanthroline (BPhen) exciton blocking layer (EBL) sandwiched between Ag cathode and molecular Diindenoperylene (DIP)/C60 bilayer of a photovoltaic…

Materials Science · Physics 2015-06-05 A. Steindamm , M. Brendel , A. K. Topczak , J. Pflaum

CdTe-based thin film solar cell has been modeled and enumerated with a thin CuInTe2 (CIT) current booster layer. CdTe-based n-CdS/p-CdTe/p+-CIT/p++-WSe2 heterojunction device has been evaluated for the highest performance. It is revealed…

We report the fabrication and measurement of thermophotovoltaic (TPV) cells with efficiencies of >40%, which is a record high TPV efficiency and the first experimental demonstration of the efficiency of high-bandgap tandem TPV cells. TPV…