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Hyperpolarized nanoparticles (NPs) offer high polarization levels with room temperature relaxation times exceeding half an hour. In this work, we demonstrate that the achievable hyperpolarization enhancement and relaxation (decay) time at…

We report record high Si-29 spin polarization obtained using dynamic nuclear polarization in microcrystalline silicon powder. Unpaired electrons in this silicon powder are due to dangling bonds in the amorphous region of this intrinsically…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 A. E. Dementyev , D. G. Cory , C. Ramanathan

We investigate the real-time estimation protocols for the frequency shift of optically detected magnetic resonance (ODMR) of nitrogen-vacancy (NV) centers in nanodiamonds (NDs). Efficiently integrating multipoint ODMR measurements and ND…

We demonstrate a way to polarize and detect nuclear spin in a gate-defined quantum point contact operating at high Landau levels. Resistively-detected Nuclear Magnetic Resonance (RDNMR) can be achieved up to the $5$th Landau level and at a…

Mesoscale and Nanoscale Physics · Physics 2018-06-06 M. H. Fauzi , A. Noorhidayati , M. F. Sahdan , K. Sato , K. Nagase , Y. Hirayama

The temperature dependence of the magnetic resonance spectra of nitrogen-vacancy (NV-) ensembles in the range of 280-330 K was studied. Four samples prepared under different conditions were studied with NV- concentrations ranging from 10…

Mesoscale and Nanoscale Physics · Physics 2010-10-12 V. M. Acosta , E. Bauch , M. P. Ledbetter , A. Waxman , L. S. Bouchard , D. Budker

The integration on a single chip of the sensitivity-relevant electronics of nuclear magnetic resonance (NMR) and electron spin resonance (ESR) spectrometers is a promising approach to improve the limit of detection, especially for samples…

Instrumentation and Detectors · Physics 2020-03-09 Nergiz Sahin Solmaz , Marco Grisi , Alessandro Valentino Matheoud , Gabriele Gualco , Giovanni Boero

The use of hyperpolarized agents in magnetic resonance (MR), such as 13C-labeled compounds, enables powerful new imaging and detection modalities that stem from a 10,000-fold boost in signal. A major challenge for the future of the…

Mesoscale and Nanoscale Physics · Physics 2015-10-28 Ewa Rej , Torsten Gaebel , Thomas Boele , David E. J. Waddington , David J. Reilly

We propose a practical implementation of a two-qubit entanglement engine which denotes a scheme to generate quantum correlations through purely dissipative processes. On a diamond platform, the electron spin transitions of two…

Quantum Physics · Physics 2024-01-17 Shishir Khandelwal , Shashwat Kumar , Nicolas Palazzo , Géraldine Haack , Mayeul Chipaux

Diamonds melt at temperatures above 4000 K. There are no measurements of the steady-state rate of the reverse process: diamond nucleation from the melt, because experiments are difficult at these extreme temperatures and pressures. Using…

Soft Condensed Matter · Physics 2015-05-13 L. M. Ghiringhelli , C. Valeriani , E. J. Meijer , D. Frenkel

Nitrogen-vacancy (NV) centers in diamond have emerged as quantum sensors capable of detecting nuclear magnetic resonance (NMR) signals at unprecedented length scales, ranging from picoliter sample volumes down to single spins at the diamond…

Chemical Physics · Physics 2025-01-07 Nick R. von Grafenstein , Karl D. Briegel , Jorge Casanova , Dominik B. Bucher

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

We propose a new method for dynamic nuclear polarisation in a quasi one-dimensional quantum wire utilising the spin-orbit interaction, the hyperfine interaction, and a finite source-drain potential difference. In contrast with current…

Mesoscale and Nanoscale Physics · Physics 2008-03-05 V. Tripathi , A. C. H. Cheung , N. R. Cooper

We study the polarisation dependence of the homogeneously broadened nuclear spin resonance in a crystal. We employ a combinatorial method to restrict the nuclear states to a fixed polarisation and show that the centre of the resonance is…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 O. Tsyplyatyev , D. M. Whittaker

Initializing quantum registers with high fidelity is a fundamental precondition for many applications like quantum information processing and sensing. The electronic and nuclear spins of a Nitrogen-Vacancy (NV) center in diamond form an…

Quantum Physics · Physics 2020-04-06 K. Rama Koteswara Rao , Yihua Wang , Zingfu Zhang , Dieter Suter

We investigate nuclear spin hyperpolarization from nitrogen vacancy centers in isotopically enriched diamonds with $^{13}$C concentrations up to 100%. $^{13}$C enrichment leads to hyperfine structure of the nitrogen vacancy electron spin…

Nanodiamond is poised to become an attractive material for hyperpolarized 13C MRI if large nuclear polarizations can be achieved without the accompanying rapid spin-relaxation driven by paramagnetic species. Here we report enhanced and…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 T. Boele , D. E. J. Waddington , T. Gaebel , E. Rej , A. Hasija , L. J. Brown , D. R. McCamey , D. J. Reilly

Diamond samples of defects with negative charged nitrogen-vacancy (NV) centers are promising solid state spin sensors suitable for quantum information processing, high sensitive measurements of magnetic, electric and thermal fields in…

Mesoscale and Nanoscale Physics · Physics 2022-03-16 Zheng Wang , Jintao Zhang , Xiaojuan Feng , Li Xing

The optical transition linewidth and emission polarization of single nitrogen-vacancy (NV) centers are measured from 5 K to room temperature. Inter-excited state population relaxation is shown to broaden the zero-phonon line and both the…

We consider the dynamic nuclear spin polarization (DNP) using two electrons in a double quantum dot in presence of external magnetic field and spin-orbit interaction, in various schemes of periodically repeated sweeps through the S-T+…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Izhar Neder , Mark S. Rudner , Bertrand I. Halperin

Control of the crystalline orientation of nitrogen-vacancy (NV) defects in diamond is here demonstrated by tuning the temperature of chemical vapor deposition (CVD) growth on a (113)-oriented diamond substrate. We show that preferential…

Materials Science · Physics 2018-07-02 S. Chouaieb , L. J. Martínez , W. Akhtar , I. Robert-Philip , A. Dréau , O. Brinza , J. Achard , A. Tallaire , V. Jacques