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We investigate the dynamic nuclear polarization from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins coupled to them in semiconductor nanostructures. We derive the time and position dependence of the…

Materials Science · Physics 2007-05-23 Ionel Tifrea , Michael E. Flatte

The temperature dependence of $^1$H and $^{13}$C nuclear spin-lattice relaxation rate $1/T_1$ has been studied in the 1.6 K - 4.2 K temperature range in pure pyruvic acid and in pyruvic acid containing trityl radicals at a concentration of…

Soft Condensed Matter · Physics 2015-01-06 Marta Filibian , Sonia Colombo Serra , Marco Moscardini , Alberto Rosso , Fabio Tedoldi , Pietro Carretta

We investigated optical spin orientation and dynamic nuclear polarization (DNP) in individual self-assembled InGaAs/GaAs quantum dots (QDs) doped by a single Mn atom, a magnetic impurity providing a neutral acceptor A$^0$ with an effective…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 O. Krebs , E. Baudin , A. Lemaître

Magnetic resonance imaging in ultra-low fields is often limited by mediocre signal-to-noise ratio hindering a higher resolution. Overhauser dynamic nuclear polarisation (O-DNP) using nitroxide radicals has been an efficient solution for…

Solid-state NMR spectroscopy is a powerful technique for the characterization of the atomic-level structure and dynamics of materials. Nevertheless, the use of this technique is often limited by its lack of sensitivity, which can prevent…

Direct dynamic nuclear polarization of 1H nuclei in frozen water and water-ethanol mixtures is demonstrated using silicon nanoparticles as the polarizing agent. Electron spins at dangling-bond sites near the silicon surface are identified…

Mesoscale and Nanoscale Physics · Physics 2014-01-14 M. C. Cassidy , C. Ramanathan , D. G. Cory , J. W. Ager , C. M. Marcus

We present the magnetic properties of three recently synthesized binuclear molecular complexes [NiNd], [NiGd] and [ZnGd] investigated by dc magnetization and proton nuclear magnetic resonance (NMR) measurements. The high-temperature…

Mesoscale and Nanoscale Physics · Physics 2011-12-01 P. Khuntia , M. Mariani , A. V. Mahajan , A. Lascialfari , F. Borsa , T. D. Pasatoiu , M. Andruh

Recent results are reported showing the effects of thermal pairing in highly excited nuclei. It is demonstrated that thermal pairing included in the phonon damping model (PDM) is responsible for the nearly constant width of the giant dipole…

Nuclear Theory · Physics 2015-06-22 Nguyen Dinh Dang

Finite temperature results in various effects on the properties of nuclear structure and excitations of relevance for nuclear processes in hot stellar environments. Here we introduce the self-consistent finite temperature relativistic…

Nuclear Theory · Physics 2023-10-03 Amandeep Kaur , Esra Yüksel , Nils Paar

We report electrical tuning by the Stark effect of the excited-state structure of single nitrogen-vacancy (NV) centers located less than ~100 nm from the diamond surface. The zero-phonon line (ZPL) emission frequency is controllably varied…

A novel mathematical treatment is proposed for computing the time evolution of dynamic nuclear polarization processes in the low temperature thermal mixing regime. Without assuming any a priori analytical form for the electron polarization,…

Statistical Mechanics · Physics 2017-08-23 Sonia Colombo Serra , Alberto Rosso , Fabio Tedoldi

We study spin relaxation and diffusion in an electron-spin ensemble of nitrogen impurities in diamond at low temperature (0.25-1.2 K) and polarizing magnetic field (80-300 mT). Measurements exploit mode- and temperature-dependent coupling…

Mesoscale and Nanoscale Physics · Physics 2013-02-13 V. Ranjan , G. de Lange , R. Schutjens , T. Debelhoir , J. P. Groen , D. Szombati , D. J. Thoen , T. M. Klapwijk , R. Hanson , L. DiCarlo

The blue-green phosphorescence/thermoluminescence is most commonly observed in diamonds following excitation at or above the indirect band gap and has been explained by a substitutional nitrogen-boron donor-acceptor pair recombination…

Materials Science · Physics 2024-07-17 Jiahui Zhao , Ben L. Green , Ben G. Breeze , Hengxin Yuan , Troy Ardon , Wuyi Wang , Mark E. Newton

Experiments suggest that nuclear spins play a significant role in the quantum Hall effect (QHE) near integer and fractional QHE spin transitions, but many of these phenomena still remain to be understood. Here we study theoretically the…

Mesoscale and Nanoscale Physics · Physics 2026-02-03 Haotian Zhou , Yuli Lyanda-Geller

The effect of improved dielectric properties in the presence of an applied magnetic field is discussed in Pr doped polycrystalline Gd$_{0.55}$Pr$_{0.45}$MnO$_3$ complemented by the structural properties down to 50 K and magnetic properties.…

Strongly Correlated Electrons · Physics 2023-04-05 Pooja Pant , Harshit Agarwal , Suresh Bharadwaj , Archana Sagdeo , M. A. Shaz

We use dynamic nuclear polarization (DNP) enhanced nuclear magnetic resonance (NMR) at liquid helium temperatures to directly detect hydrogen attached to the surface of silicon microparticles. The proton NMR spectrum from a dry sample of…

Materials Science · Physics 2017-06-08 Mallory L. Guy , Kipp J. van Schooten , Lihuang Zhu , Chandrasekhar Ramanathan

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

A quasi-classical theoretical description of polarization and relaxation of nuclear spins in a quantum dot with one resident electron is developed for arbitrary mechanisms of electron spin polarization. The dependence of the…

Strongly Correlated Electrons · Physics 2015-05-13 I. A. Merkulov , G. Alvarez , D. R. Yakovlev , T. C. Schulthess

Macroscopic polarity and its dynamic response to external electric fields and temperature in the nominally ergodic relaxor phase of pristine lead magnesium niobate crystals and ceramics, Pb(Mg1/3Nb2/3)O3 (PMN), were investigated. Dynamic…

Materials Science · Physics 2020-11-06 Lukas M. Riemer , Kanghyun Chu , Yang Li , Hana Ursic , Andrew J. Bell , Brahim Dkhil , Dragan Damjanovic

We propose a nuclear-spin-polarization protocol in a general evolution-and-measurement framework. The protocol works in a spin-star configuration, where the central spin is coupled to the surrounding bath (nuclear) spins by flip-flop…

Quantum Physics · Physics 2022-12-07 Zhu-yao Jin , Jia-shun Yan , Jun Jing
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