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The many-body theory of interacting electrons poses an intrinsically difficult problem that requires simplifying assumptions. For the determination of electronic screening properties of the Coulomb interaction, the Random Phase…

Strongly Correlated Electrons · Physics 2021-07-26 Erik G. C. P. van Loon , Malte Rösner , Mikhail I. Katsnelson , Tim O. Wehling

Starting from the general expression for the ground state correlation energy in the adiabatic connection fluctuation dissipation theorem (ACFDT) framework, it is shown that the dielectric matrix formulation, which is usually applied to…

Chemical Physics · Physics 2016-04-25 Bastien Mussard , Dario Rocca , Georg Jansen , Janos Angyan

The Random Phase Approximation (RPA) is a widely employed post Hartree-Fock or DFT method, capable of capturing van der Waal interactions and other dynamic correlation effects at relatively low costs of $\mathcal O(N^3)$ in time and…

Materials Science · Physics 2015-09-02 Felix Hummel

The relativistic mean field approach (RMF) is well known for describing accurately binding energies and nucleon distributions in atomic nuclei throughout the nuclear chart. The random phase approximation (RPA) built on top of the RMF is…

Nuclear Theory · Physics 2008-11-26 Nguyen Van Giai , Haozhao Liang , Jie Meng

The particle-particle random phase approximation (pp-RPA) has been shown to be capable of describing double, Rydberg, and charge transfer excitations, for which the conventional time-dependent density functional theory (TDDFT) might not be…

Computational Physics · Physics 2017-04-26 Jianfeng Lu , Haizhao Yang

We use continuum mechanics [Tao \emph{et al}, PRL{\bf 103},086401] to approximate the dynamic density response of interacting many-electron systems. Thence we develop a numerically efficient exchange-correlation energy functional based on…

Mesoscale and Nanoscale Physics · Physics 2012-08-28 Tim Gould , John F. Dobson

Perfect adaptation is a phenomenon whereby the output variables of a system can maintain certain values despite external disturbances. Robust perfect adaptation (RPA) refers to an adaptation property that does not require fine-tuning of…

Molecular Networks · Quantitative Biology 2023-07-17 Yuji Hirono , Ankit Gupta , Mustafa Khammash

We study the correlation energy associated with the pair fluctuations in BCS theory. We use a schematic two-level pairing model and discuss the behavior of the correlation energy across shell closures, including the even-odd differences. It…

Nuclear Theory · Physics 2009-11-06 K. Hagino , G. F. Bertsch

We investigate static correlation and delocalization errors in the self-consistent GW and random-phase approximation (RPA) by studying molecular dissociation of the H_2 and LiH molecules. Although both approximations contain topologically…

Strongly Correlated Electrons · Physics 2015-04-10 Maria Hellgren , Fabio Caruso , Daniel R. Rohr , Xinguo Ren , Angel Rubio , Matthias Scheffler , Patrick Rinke

We present an extensive set of surface and chemisorption energies calculated using state of the art many-body perturbation theory. In the first part of the paper we consider ten surface reactions in the low coverage regime where…

Materials Science · Physics 2018-02-01 Per Simmendefeldt Schmidt , Kristian Sommer Thygesen

We consider several spin-unrestricted random-phase approximation (RPA) variants for calculating correlation energies, with and without range separation, and test them on datasets of atomization energies and reaction barrier heights. We show…

Chemical Physics · Physics 2016-03-01 Bastien Mussard , Peter Reinhardt , Janos Angyan , Julien Toulouse

A relativistic mean field description of collective excitations of atomic nuclei is studied in the framework of a fully self-consistent relativistic random phase approximation (RRPA). In particular, results of RRPA calculations of multipole…

Nuclear Theory · Physics 2009-11-07 Zhong-yu Ma , A. Wandelt , Nguyen Van Giai , D. Vretenar , P. Ring , Li-gang Cao

The dynamical effects of ground state correlations for excitation energies and transition strengths near the superfluid phase transition are studied in the soluble two level pairing model, in the context of the particle-particle self…

Nuclear Theory · Physics 2008-11-26 E. J. V. de Passos , A. F. R. de Toledo Piza , F. Krmpotić

In the derivation of low-energy effective models for solids targeting the bands near the Fermi level, the constrained random phase approximation (cRPA) has become an appreciated tool to compute the effective interactions. The Wick-ordered…

Strongly Correlated Electrons · Physics 2015-07-15 Michael Kinza , Carsten Honerkamp

Quantum phase estimation (QPE) is a promising quantum algorithm for obtaining molecular ground-state energies with chemical accuracy. However, its computational cost, dominated by the Hamiltonian 1-norm $\lambda$ and the cost of the block…

We present a new density-functional method of the self-consistent electronic-structure calculation which does not exploit any local density approximations (LDA). We use the exchange-correlation energy which consists of the exact exchange…

Statistical Mechanics · Physics 2009-10-30 Takao Kotani

We present a low-scaling algorithm for the random phase approximation (RPA) with \textbf{k}-point sampling in the framework of tensor hypercontraction (THC) for electron repulsion integrals (ERIs). The THC factorization is obtained via a…

Materials Science · Physics 2023-12-01 Chia-Nan Yeh , Miguel A. Morales

The self-consistent random phase approximation (RPA) approach with the residual interaction derived from a relativistic point-coupling energy functional is applied to evaluate the isospin symmetry-breaking corrections {\delta}c for the…

Nuclear Theory · Physics 2015-03-19 Z. X. Li , J. M. Yao , H. Chen

The optimized random phase approximation (ORPA) for classical liquids is re-examined in the framework of the generating functional approach to the integral equations. We show that the two main variants of the approximation correspond to the…

Chemical Physics · Physics 2009-10-30 G. Pastore , O. Akinlade , F. Matthews , Z. Badirkhan

We revisit the connection between equation-of-motion coupled cluster (EOM-CC) and random phase approximation (RPA) explored recently by Berkelbach [J. Chem. Phys. 149, 041103 (2018)] and unify various methodological aspects of these diverse…

Chemical Physics · Physics 2020-12-17 Varun Rishi , Ajith Perera , Rodney J. Bartlett
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