Related papers: 229Th-doped nonlinear optical crystals for compact…
Building on recent advances of the embedded cluster approach combined with multiconfigurational theory, this work investigates the electronic states in thorium-doped CaF2 crystals. Th:CaF2 is currently establishing as a promising material…
Harmonic generation mechanisms are of great interest in nanoscience and nanotechnology, since they allow generating visible light by using near-infrared radiation, which is particularly suitable for its endless applications in…
We report the first experimental observation of discrete time-crystal phases and crystallites in an actively mode-locked semiconductor laser. By tuning either the bias current or the modulation frequency, the system undergoes a spontaneous…
The superb precision of an atomic clock is derived from its stability. Atomic clocks based on optical (rather than microwave) frequencies are attractive because of their potential for high stability, which scales with operational frequency.…
With an expected energy of 7.6(5) eV, $^{229}$Th possesses the lowest excited nuclear state in the landscape of all presently known nuclei. The energy corresponds to a wavelength of about 160 nm and would conceptually allow for an optical…
Chip-scale microwave atomic systems based on thermal atomic beams offer a promising approach to realize low-power and low-drift clocks for timing holdover applications. Miniature beam clocks are expected to suppress many of the shifts that…
Superradiant laser, which exploits the clock transition of alkaline-earth-metal-like atoms to generate ultrastable light in the bad-cavity limit, has garnered much attention in the past few decades. Unlike their odd counterpart, the even…
The population dynamics of the 229Th isomeric state is studied in a solid-state host under laser illumination. A photoquenching process is observed, where off-resonant vacuum-ultraviolet (VUV) radiation leads to relaxation of the isomeric…
Active optical clock, a new conception of atomic clock, has been proposed recently. In this report, we propose a scheme of active optical clock based on four-level quantum system. The final accuracy and stability of two-level quantum system…
The electronic defect states resulting from doping $^{229}$Th in CaF$_2$ offer a unique opportunity to excite the nuclear isomeric state $^{229m}$Th at approximately 8 eV via electronic bridge mechanisms. We consider bridge schemes…
The low-energy isomeric transition in Thorium-229 offers a unique interface between nuclear and atomic physics, presenting a resource for quantum technologies that is notably resilient to environmental decoherence. While early experiments…
In optical clocks, transitions of ions or neutral atoms are interrogated using pulsed ultra-narrow laser fields. Systematic phase chirps of the laser or changes of the optical path length during the measurement cause a shift of the…
Highly charged ions (HCIs) are insensitive to external perturbations and are attractive for the development of ultrastable clocks. However, only a few HCI candidates are known to provide optical clock transitions. In this Letter, we show…
This study investigates the dynamic control of third-order nonlinear optical absorption properties of gold nanoparticles (AuNPs) dispersed in nematic liquid crystals (LC). By leveraging the reconfigurable nature of liquid crystals under…
We study the Ho$^{14+}$ ion as a candidate for extremely accurate and stable optical atomic clock which is sensitive to the time variation of the fine structure constant. We demonstrate that the proposed system has all desired features…
The 10-minute radiative lifetime of the first excited $^{229}$Th$^{4+}$ nuclear state in ionic crystals provides narrow spectroscopic linewidths, enabling the realization of a solid-state nuclear clock. Due to the 4+ noble gas…
Noble metals with well-defined crystallographic orientation constitute an appealing class of materials for controlling light-matter interactions on the nanoscale. Nonlinear optical processes, being particularly sensitive to anisotropy, are…
The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary…
A new method for obtaining of inverse population between quadrupole sublevels of the ground state $5/2^+(0.0)$ and the isomeric state $3/2^+(7.6$ eV) of the $^{229}$Th nucleus in a dielectric crystal with a large band gap by means of…
We propose to build a bad cavity laser using forbidden transitions in large ensembles of cold ions that form a Coulomb crystal in a linear Paul trap. This laser might realize an active optical frequency standard able to serve as a local…