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Optical clocks are the apotheosis of precision measurement, but they require frequent maintenance by scientists. The supporting laser systems are a particularly demanding component of these instruments. To reduce complexity and increase…

Atomic Physics · Physics 2023-05-24 C. A. Holliman , M. Fan , A. M. Jayich

The radiative excitation of the 8.3 eV isomeric state of thorium-229 is an outstanding challenge due to the lack of tunable far-ultraviolet (F-UV) sources. In this work, we propose an efficient two-photon pumping scheme for thorium-229…

Nuclear Theory · Physics 2023-09-01 Haowei Xu , Hao Tang , Guoqing Wang , Changhao Li , Boning Li , Paola Cappellaro , Ju Li

The isotope $^{229}$Th is the only nucleus known to possess an excited state $^{229m}$Th in the energy range of a few electron volts, a transition energy typical for electrons in the valence shell of atoms, but about four orders of…

We have produced laser-cooled Wigner crystals of 229Th3+ in a linear Paul trap. The magnetic dipole (A) and electric quadrupole (B) hyperfine constants for four low-lying electronic levels and the relative isotope shifts with respect to…

Atomic Physics · Physics 2011-10-12 C. J. Campbell , A. G. Radnaev , A. Kuzmich

Optical clocks require an ultra-stable laser to probe and precisely measure the frequency of the narrow-linewidth clock transition. We introduce a portable ultraviolet (UV) laser system for use in an aluminum quantum logic clock,…

The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large…

The 7.6(5) eV nuclear magnetic-dipole transition in a single 229Th3+ ion may provide the foundation for an optical clock of superb accuracy. A virtual clock transition composed of stretched states within the 5F5/2 electronic ground level of…

Atomic Physics · Physics 2015-05-30 C. J. Campbell , A. G. Radnaev , A. Kuzmich , V. A. Dzuba , V. V. Flambaum , A. Derevianko

Today's most precise time and frequency measurements are performed with optical atomic clocks. However, it has been proposed that they could potentially be outperformed by a nuclear clock, which employs a nuclear transition instead of the…

We propose a simple approach to measure the energy of the few-eV isomeric state in Th-229. To this end, U-229 nuclei are doped into VUV-transparent crystals, where they undergo alpha decay into Th-229, and, with a probability of 2%,…

Nuclear Experiment · Physics 2016-08-11 Simon Stellmer , Matthias Schreitl , Georgy Kazakov , Johannes Sterba , Thorsten Schumm

Optical atomic clocks$^{1,2}$ use electronic energy levels to precisely keep track of time. A clock based on nuclear energy levels promises a next-generation platform for precision metrology and fundamental physics studies. Thorium-229…

We investigate the feasibility of precision frequency metrology with large ion crystals. For clock candidates with a negative differential static polarisability, we show that micromotion effects should not impede the performance of the…

Quantum Physics · Physics 2016-10-25 Kyle Arnold , Elnur Haciyev , Eduardo Paez , Chern Hui Lee , John Bollinger , M. D. Barrett

As an alternative to state-of-the-art laser frequency stabilisation using ultra-stable cavities, it has been proposed to exploit the non-linear effects from coupling of atoms with a narrow transition to an optical cavity. Here we have…

Vacuum-ultraviolet-transparent crystals have been proposed as host lattice for the coherent driving of the unusually low-lying isomer excitation in $^{229}$Th for metrology and quantum optics applications. Here the possible collective…

Atomic Physics · Physics 2019-01-18 Brenden S. Nickerson , Wen-Te Liao , Adriana Pálffy

An ultrastable optical clock based on neutral atoms trapped in an optical lattice is proposed. Complete control over the light shift is achieved by employing the $5s^2 {}^1S_0 \to 5s5p {}^3P_0$ transition of ${}^{87}{\rm Sr}$ atoms as a…

Atomic Physics · Physics 2009-11-10 Hidetoshi Katori , Masao Takamoto , V. G. Pal'chikov , V. D. Ovsiannikov

Laser excitation of thorium-229 nuclei in doped wide bandgap crystals has been demonstrated recently, opening the possibility of developing ultrastable solid-state clocks and sensitive searches for new physics. We develop a quantitative…

LiSrAlF$_6$ crystals doped with $^{229}$Th are used in a laser-based search for the nuclear isomeric transition. Two spectroscopic features near the nuclear transition energy are observed. The first is a broad excitation feature that…

Clocks based on nuclear isomer transitions promise exceptional stability and precision. The low transition energy of the thorium-229 isomer makes it an ideal candidate, as it has been excited by a vacuum-ultraviolet laser and is highly…

High Energy Physics - Phenomenology · Physics 2025-11-25 Cédric Delaunay , Seung J. Lee , Roee Ozeri , Gilad Perez , Wolfram Ratzinger , Bingrong Yu

An active optical clock based on highly charged Nd$^{9+}$ ion is proposed for the first time. The clock can offer ultra-narrow linewidth at the $\upmu$Hz-level which is more than two-order of magnitude below the currently recorded laser…

Atomic Physics · Physics 2021-07-23 Yan-mei Yu , Duo Pan , Shaolong Chen , Hua Guan , Kelin Gao , Jingbiao Chen

For the isotope $^{229}$Th we investigate the possibility of two-photon laser spectroscopy of the nuclear clock transition (148.38 nm) using intense monochromatic laser field at twice the wavelength (296.76 nm). Our estimates show that due…

The low-energy, long-lived isomer in $^{229}$Th, first studied in the 1970s as an exotic feature in nuclear physics, continues to inspire a multidisciplinary community of physicists. Using the nuclear resonance frequency, determined by the…

Quantum Physics · Physics 2020-12-18 E. Peik , T. Schumm , M. S. Safronova , A. Pálffy , J. Weitenberg , P. G. Thirolf