Related papers: $^{229}\mathrm{ThF}_4$ thin films for solid-state …
Solid-state $^{229}$Th nuclear clocks are set to provide new opportunities for precision metrology and fundamental physics. Taking advantage of a nuclear transition's inherent low sensitivity to its environment, orders of magnitude more…
The nucleus of the radioisotope thorium-229 (${}^{229}$Th) features an isomer with an exceptionally low excitation energy that enables direct laser manipulation of nuclear states. For this reason, it is a leading candidate for use in…
Motivated by recent experimental breakthroughs toward a realization of a solid-state Thorium-229 nuclear clock, we review the technology, basic physics motivation, and limitations of the present generation of atomic clocks. We then discuss…
The low-energy, long-lived isomer in $^{229}$Th, first studied in the 1970s as an exotic feature in nuclear physics, continues to inspire a multidisciplinary community of physicists. Using the nuclear resonance frequency, determined by the…
Optical atomic clocks$^{1,2}$ use electronic energy levels to precisely keep track of time. A clock based on nuclear energy levels promises a next-generation platform for precision metrology and fundamental physics studies. Thorium-229…
A low-energy nuclear transition in the isotope thorium-229 has been excited in thorium-doped crystals with laser light. This opens the perspective towards a highly stable and robust solid-state optical nuclear clock. The required laser…
We describe a novel approach to directly measure the energy of the narrow, low-lying isomeric state in $^{229}$Th. Since nuclear transitions are far less sensitive to environmental conditions than atomic transitions, we argue that the…
Here, we report the first demonstration of laser-induced conversion electron M\"{o}ssbauer spectroscopy of the $^{229}$Th nuclear isomeric state, which provides the ability to probe the nuclear transition in a material that is opaque to…
While the $^{229}$Th nuclear isomer has recently been observed and laser-excited, converting optical nuclear manipulation into a chip-scale solid-state frequency standard remains an open challenge. Here, we present a nanophotonic platform…
We conducted measurements on the photo- and radio-luminescence of thin ThF$_4$ films in both the UV and visible ranges. In the UV range, we found that both luminescences are at a similar level as the internal dark counting noise of the…
The isotope $^{229}$Th is the only nucleus known to possess an excited state $^{229m}$Th in the energy range of a few electron volts, a transition energy typical for electrons in the valence shell of atoms, but about four orders of…
We have recently described a novel method for the construction of a solid-state optical frequency reference based on doping $^{229}$Th into high energy band-gap crystals. Since nuclear transitions are far less sensitive to environmental…
The proposal for the development of a nuclear optical clock has triggered a multitude of experimental and theoretical studies. In particular the prediction of an unprecedented systematic frequency uncertainty of about $10^{-19}$ has…
We study thorium-doped CaF$_2$ crystals as a possible platform for optical spectroscopy of the Th-229 nuclear isomer transition. We anticipate two major sources of background signal that might cover the nuclear spectroscopy signal:…
The recent laser excitation of the 229Th isomeric transition in a solid-state host opens the door for a portable solid-state nuclear optical clock. However, at present the vacuum-ultraviolet laser systems required for clock operation are…
Today's most precise time and frequency measurements are performed with optical atomic clocks. However, it has been proposed that they could potentially be outperformed by a nuclear clock, which employs a nuclear transition instead of the…
The 7.8 eV nuclear isomer transition in 229 Thorium has been suggested as an etalon transition in a new type of optical frequency standard. Here we discuss the construction of a "solid-state nuclear clock" from Thorium nuclei implanted into…
The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary…
The radioisotope Th-229 is renowned for its extraordinarily low-energy, long-lived nuclear first-excited state. This isomeric state can be excited by VUV lasers and the transition from the ground state has been proposed as a reference…
Quantum state-resolved spectroscopy of the low energy thorium-229 nuclear transition was recently achieved. The five allowed transitions within the electric quadrupole structure were measured to the kilohertz level in a calcium fluoride…