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Related papers: Nonlinear vortex dichroism in chiral molecules

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Circular dichroism is the differential rate of absorption of right- and left-handed circularly polarized light by chiral particles. Optical vortices which convey orbital angular momentum (OAM) possess a chirality associated with the…

Optics · Physics 2021-05-26 Kayn A. Forbes , Garth A. Jones

In this study, we investigate the nonlinear optical phenomena emerging from the interaction of vortex and vector beams with achiral nanoparticles or nanostructures. We reveal the conditions under which linear or nonlinear dichroism can be…

Optics · Physics 2024-06-13 Anastasia Nikitina , Kristina Frizyuk

Circular dichroism, arising from interactions with light fields of opposite spin angular momentum, has become a fundamental tool for molecular characterization. Meanwhile, helical dichroism (HD) - the dichroic response to vortex beams…

We show how both the ellipticity $\eta$ and degree of polarization $\textit{P}$ influences the extraordinary optical chirality properties of non-paraxial vortex beams. We find that, in stark contrast to paraxial optics and non-vortex modes,…

Optics · Physics 2024-12-02 Kayn A. Forbes , Dale Green

It is shown theoretically that a nonchiral, two-dimensional array of metallic spheres exhibits optical activity as manifested in calculations of circular dichroism. The metallic spheres occupy the sites of a rectangular lattice and for…

Optics · Physics 2009-11-13 Vassilios Yannopapas

Chirality is ubiquitous in nature and fundamental in science, from particle physics to metamaterials.The most established technique of chiral discrimination - photoabsorption circular dichroism - relies on the magnetic properties of a…

We perform a theoretical and numerical study of the optical properties of both direct and inverse three-dimensional (3D) chiral woodpile structures, and a corresponding chiral Bragg stack. We compute transmission spectra in the helical…

Optical beams with a new and distinctive type of helicity have become the subject of much recent interest. While circularly polarised light comprises photons with spin angular momentum, these optically engineered 'twisted beams' (optical…

Optics · Physics 2015-06-26 David L. Andrews , Luciana C. Davila Romero , Mohamed Babiker

Chirality is a structural property of molecules lacking mirror symmetry that has strong implications in diverse fields, ranging from life to materials sciences. Established spectroscopic methods that are sensitive to chirality, such as…

We report observation of electron helical dichroism on a material with chiral structure. In analogy with circular dichroism, a common technique for molecular structural fingerprinting, we use a nanofabricated forked diffraction grating to…

Materials Science · Physics 2015-07-08 Tyler R. Harvey , Jordan S. Pierce , Jordan J. Chess , Benjamin J. McMorran

Helical dichroism (HD) is a proposed method for the resolution of molecular chirality, employing the orbital angular momentum (OAM) of light. Going beyond the conventional assumptions about HD, this work proposes a rigid theoretical…

Atomic Physics · Physics 2026-01-09 Mateja Hrast , Georgios M. Koutentakis , Mikhail Maslov , Mikhail Lemeshko

Material anisotropy and chirality produce polarization-dependent light-matter interactions. Absorption leads to linear and circular dichroism, whereas elastic forward scattering produces linear and circular birefringence. Here we highlight…

Optics · Physics 2024-12-02 Kayn A. Forbes , Dale Green

Theory of optical absorption of linearly and circularly polarized light in surface and edge states in topological insulators is developed for a nonlinear in light intensity regime. The absorbance for surface states and the absorption width…

Mesoscale and Nanoscale Physics · Physics 2022-03-30 N. V. Leppenen , L. E. Golub

Photoelectron circular dichroism (PECD) is a method where randomly oriented chiral molecules are photoionized due to irradiation by circularly-polarized lasers, yielding large chiral signals in the photoelectron momentum distribution.…

Optics · Physics 2025-12-16 Gal Bouskila , Avner Fleischer , Ofer Neufeld

Chirality is ubiquitous from microscopic to macroscopic phenomena in physics and biology, such as fermionic interactions and DNA duplication. In photonics, chirality has traditionally represented differentiated optical responses for right…

Optics · Physics 2019-09-02 Sunkyu Yu , Xianji Piao , Namkyoo Park

Strong enhancement of molecular circular dichroism has the potential to enable efficient asymmetric photolysis, a method of chiral separation that has conventionally been impeded by insufficient yield and low enantiomeric excess. Here, we…

This paper presents the most complete framework to date for understanding the nonlinear optical trapping of highly absorbing nanoparticles within the dipole regime. Highly absorbing and plasmonic particles garner considerable interest due…

Optics · Physics 2024-06-05 Siavash Mirzaei-Ghormish , Kamran Qaderi , Daniel Smalley

The chiral optical absorption by a single vortex in a p_x \pm i p_y-wave superconductor is studied theoretically. The p_x \pm i p_y-wave state was recently suggested as the symmetry of the order parameter of Sr_2 Ru O_4 superconductor. Due…

Superconductivity · Physics 2009-10-31 Masashige Matsumoto , Manfred Sigrist

Circular dichroism spectroscopy is an essential technique for understanding molecular structure and magnetic materials, but spatial resolution is limited by the wavelength of light, and sensitivity sufficient for single-molecule…

Circular dichroism (CD), i.e. the differential response of a system to left and right circularly polarized light, is one of the only techniques capable of providing morphological information of certain samples. In biology, for instance, CD…

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