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Related papers: Nonlinear vortex dichroism in chiral molecules

200 papers

Using terahertz time domain spectroscopy we demonstrate tunable polarization rotation and circular dichroism in intrinsically nonchiral planar terahertz metamaterials without twofold rotational symmetry. The observed effect is due to…

Optics · Physics 2010-09-03 Ranjan Singh , Eric Plum , Weili Zhang , Nikolay I. Zheludev

Circular dichroism is a technologically important phenomenon contrasting the absorption and resultant emission properties between left- and right-handed circularly polarized light. While the chiral handedness of systems mainly determines…

Optics · Physics 2023-03-21 Xiuhu Zhao , Jinxing Li , Mingjun Huang , Satoshi Aya

Chiroptical effects using circularly polarized light produce signals that change sign when switching either molecular handedness (enantiosensitivity) or the light helicity (circular dichroism). Here, we break this…

Circular dichroism (CD) caused by the response of a chiral object to circularly polarized light has been well established, and the strong CD of plasmonic meta-molecules has also become of interest in recent years; however, their response if…

Optics · Physics 2020-09-30 Yangzhe Guo , Guodong Zhu , Wanlu Bian , Bin Dong , Yurui Fang

Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…

Chemical Physics · Physics 2017-02-08 Jérémy R. Rouxel , Markus Kowalewski , Shaul Mukamel

Helical dichroism (HD), originating from the interplay between chiral plasmonic structures and left and right vortex light carrying orbital angular momentum (OAM), has attracted significant attention across various disciplines owing to its…

Optics · Physics 2025-08-08 Takahiro Uto , An'an Wu , Tsutomu Shimura , Yoshito Y. Tanaka

Chirality is at the origin of life and is ubiquitous in nature. An object is deemed chiral if it is non-superimposable with its own mirror image. This relates to how circularly polarized light interacts with such object, a circular…

Chirality refers to a geometric phenomenon in which objects are not superimposable on their mirror image. Structures made of nano-scale chiral elements can display chiroptical effects, such as dichroism for left- and right- handed…

Optics · Physics 2020-02-25 Behrooz Semnani , Jeremy Flannery , Rubayet Al Maruf , Michal Bajcsy

It has been long recognized that the spatial polarization of the electronic clouds in molecules, and the spatial arrangements of atoms into chiral molecular structures, play crucial roles in physics, chemistry and biology. However, these…

Optics · Physics 2020-04-14 David Ayuso , Andres Ordonez , Piero Decleva , Misha Ivanov , Olga Smirnova

We report on a universal topological dichroism of chiral three-dimensional systems in response to the chirality of light. We show that chiral topological invariants result in integer-quantized dichroic excitation rate differences. Moreover,…

Mesoscale and Nanoscale Physics · Physics 2026-03-31 Wojciech J. Jankowski , Giandomenico Palumbo , Robert-Jan Slager

Analytical forms of the optical helicity and optical chirality of monochromatic Laguerre-Gaussian optical vortex beams are derived up to second order in the paraxial parameter $kw_0$. We show that input linearly polarised optical vortices…

Optics · Physics 2021-10-08 Kayn A. Forbes , Garth A. Jones

We develop a microscopic theory of optical absorption and structured-light dichroism in a nonlocal minimal-coupling framework. Starting from the minimal-coupling Hamiltonian, we express absorption as a bilinear functional of the…

Optics · Physics 2026-04-14 Akihito Kato , Nobuhiko Yokoshi

Chiral molecules are instrumental for molecular recognition in living organisms. Distinguishing between two opposite enantiomers, the mirror twins of the same chiral molecule, is both vital and challenging. Photoelectron circular dichroism…

Chemical Physics · Physics 2021-12-07 Andres F. Ordonez , David Ayuso , Piero Decleva , Olga Smirnova

Circular Dichroism (CD) can distinguish the handedness of chiral molecules. However, it is typically very weak due to vanishing absorption at low molecular concentrations. Here, we suggest Thermal Circular Dichroism (TCD) for chiral…

Optics · Physics 2024-07-19 Ershad Mohammadi , Giulia Tagliabue

Chirality is a fundamental asymmetry phenomenon, with chiral optical elements exhibiting asymmetric response in reflection or absorption of circularly polarized light. Recent realizations of such elements include nanoplasmonic systems with…

Two-dimensional lattices of chiral nanoholes in a plasmonic film with lattice constants being slightly larger than light wavelength are proposed for effective control of polarization and spatial properties of light beams. Effective…

Mesoscale and Nanoscale Physics · Physics 2016-03-15 V. V. Klimov , I. V. Zabkov , A. A. Pavlov , R. -C. Shiu , H. -C. Chan , G. Y. Guo

Vector optical vortices exhibit complex polarisation patterns due to the interplay between spin and orbital angular momenta. Here we demonstrate, both analytically and with simulations, that certain polarisation features of optical vortex…

Identifying and imaging spin textures of ever more complex magnetic structures has become a major challenge in the past decade, especially at ultrashort timescales. Most of current approaches are based on the analysis of their polarization…

Optics · Physics 2020-05-26 Thierry Ruchon , Mauro Fanciulli

We investigate the interaction between a monolayer of WS2 and a chiral plasmonic metasurface. WS2 possesses valley excitons that selectively couple with one-handed circularly polarised light. At the same time, the chiral plasmonic…

Optics · Physics 2023-10-31 Fernando Lorén , Cyriaque Genet , Luis Martín-Moreno

Investigating chiral light-matter interactions is essential for advancing applications in sensing, imaging, and pharmaceutical development. However, the chiroptical response in natural chiral molecules and subwavelength chiral structures is…