Related papers: Nonlinear vortex dichroism in chiral molecules
Structured light, when strongly focused, generates highly confined vectorial electromagnetic field distributions which may feature a polarization component along the optical axis. Manipulating and detecting such 3D light fields is…
We generate double-charge white-light optical vortices by sending a circularly polarized partially incoherent light through an uniaxial crystal. We show that the generated polichromatic vortices are structurally stable, and their…
Controlling the polarization state of electromagnetic radiation enables the investigation of fundamental symmetry properties of matter through chiroptical processes. Many strategies have been developed to reveal structural or dynamical…
Polyalanine molecules (PA) with an {\alpha}-helix conformation gathered recently a lot of interest as the propagation of electrons through the chiral backbone structure comes along with spin polarization of the transmitted electrons. By…
Molecular chirality is an omnipresent phenomenon of fundamental significance in physics, chemistry and biology. For this reason, search for novel techniques for enantioselective control, detection and separation of chiral molecules is of…
Light polarization is a key aspect of modern optics. Current methods for polarization control utilize birefringence and dichroism of anisotropic materials or of arrays of anisotropically shaped nanostructures. Based on collective optical…
X-ray linear dichroism has been pivotal for probing electronic anisotropies, but its inherent limited spatial resolution precludes atomic-scale investigations of orbital polarization. Here we introduce a versatile electron linear dichroism…
Twisted atomic bilayers are emerging platforms for manipulating chiral light-matter interaction at the extreme nanoscale, due to their inherent magnetoelectric responses induced by the finite twist angle and quantum interlayer coupling…
We investigate electron vortex beams elastically scattered on chiral crystals. After deriving a general expression for the scattering amplitude of a vortex electron, we study its diffraction on point scatterers arranged on a helix. We…
Photoelectron circular dichroism refers to the forward/backward asymmetry in the photoelectron angular distribution with respect to the propagation axis of circularly polarized light. It has recently been demonstrated in femtosecond…
Chiroptical techniques for detecting and characterizing the chirality of matter and artificial nanostructures are traditionally based on their interaction with chiral light, typically circularly-polarized fields propagating in free space.…
Many polarisation techniques have been harnessed for decades in biological and clinical research, each based upon measurement of the vectorial properties of light or the vectorial transformations imposed on light by objects. Various…
Chiral perovskites owing to their broken mirror symmetry exhibit selective absorption of circularly polarized light manifesting a strong circular dichroism (CD). CD spectroscopy has been a key technique to understand chiral perovskites and…
Because of their central importance in chemistry and biology, water molecules have been the subject of decades of intense spectroscopic investigations. Rotational spectroscopy of water vapor has yielded detailed information about the…
We argue that the layer electric polarization of noncentrosymmetric layered heterostructures can be generically controlled by light yielding a layer photovoltaic effect (LPE). The LPE possesses a rich phenomenology and can arise from myriad…
Refracton of particles (nucleons, nuclei, $\gamma$-quanta) in matter with polarized protons (nuclei) results in revealing coherent quasi-optical phenomenon of nuclear spin precession of particles (nuclei) in the pseudomagnetic field of…
Chirality is a fundamental feature in all domains of nature, ranging from particle physics over electromagnetism to chemistry and biology. Chiral objects lack a mirror plane and inversion symmetry and therefore cannot be spatially aligned…
Spontaneous formation of polarization gratings by liquid crystals made of bent dimeric molecules is reported. The grating is formed within the temperature range of the twist bend modulated nematic phase, NTB, without the necessity to…
Single-layer transition-metal dichalcogenides provide an unique intrinsic entanglement between the spin/valley/orbital degrees of freedom and the polarization of scattered photons. This scenario gives rise to the well-assessed optical…
Chiral metal halide perovskites have emerged as promising optoelectronic materials for emission and detection of circular polarized visible light. Despite chirality being realized by adding chiral organic cations or ligands, the chiroptical…