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We demonstrate precision measurement and control of inhomogeneous broadening in a multi-ion clock consisting of three $^{176}$Lu$^+$ ions. Microwave spectroscopy between hyperfine states in the $^3D_1$ level is used to characterise…

For decades, improved theory and experiment of the $n=2$ $^3$P fine structure of helium have allowed for increasingly-precise tests of quantum electrodynamics, determinations of the fine-structure constant $\alpha$, and limitations on…

Atomic Physics · Physics 2018-10-10 K. Kato , T. D. G. Skinner , E. A. Hessels

We report the measurement of hyperfine splitting in the $7d$ $^{2}D_{3/2}$ state of $^{133}$Cs using high resolution Doppler-free two-photon spectroscopy in a Cs vapor cell. We determine the hyperfine coupling constants $A = 7.3509(9)$ MHz…

Atomic Physics · Physics 2022-10-05 Bubai Rahaman , Sourav Dutta

Optical atomic clocks have already overcome the eighteenth decimal digit of instability and uncertainty demonstrating incredible control over external perturbations of the clock transition frequency. At the same time there is an increasing…

Extra-laboratory atomic clocks are necessary for a wide array of applications (e.g. satellite-based navigation and communication). Building upon existing vapor cell and laser technologies, we describe an optical atomic clock, designed…

Quantum simulations with ultracold atoms typically create atomic wavefunctions with structures at optical length scales, where direct imaging suffers from the diffraction limit. In analogy to advances in optical microscopy for biological…

Quantum Gases · Physics 2019-04-10 Sarthak Subhankar , Yang Wang , Tsz-Chun Tsui , Steven L. Rolston , James V. Porto

The rotational spectrum of the molecular ion HCNH+ is revisited using double-resonance spectroscopy in an ion trap apparatus, with six transitions measured between 74 and 445 GHz. Due to the cryogenic temperature of the trap, the hyperfine…

Chemical Physics · Physics 2024-04-09 Weslley G. D. P. Silva , Luis Bonah , Philipp C. Schmid , Stephan Schlemmer , Oskar Asvany

With the development of microwave atomic clocks, the Zeeman shifts for the spectral lines of black-body radiation need to be investigated carefully. In this Letter, the frequency shifts of hyperfine splittings of atomic ground states due to…

Atomic Physics · Physics 2020-02-12 Jize Han , Yani Zuo , Jianwei Zhang , Lijun Wang

Measuring the hyperfine structure (HFS) of long-lived $^3P_2$ states of divalent atoms may offer the opportunity of extracting relatively unexplored nuclear magnetic octupole and electric hexadecapole moments. Here, using relativistic…

Atomic Physics · Physics 2009-11-13 K. Beloy , A. Derevianko , W. R. Johnson

Accurate measurements of different transition frequencies between atomic levels of the electronic and hyperfine structure over time are used to investigate temporal variations of the fine structure constant $\alpha$ and the…

Atomic Physics · Physics 2014-12-01 N. Huntemann , B. Lipphardt , Chr. Tamm , V. Gerginov , S. Weyers , E. Peik

We present a spectroscopy scheme for the 7-kHz-wide 689-nm intercombination line of strontium. We rely on shelving detection, where electrons are first excited to a metastable state by the spectroscopy laser before their state is probed…

The spectroscopic hyperfine constants for all the alkali atoms are reported. For atoms from lithium to cesium, only the long lived atomic isotopes are examined. For francium, the measured data for nuclear ground states of all available…

Atomic Physics · Physics 2024-06-19 M. Allegrini , E. Arimondo , L. A. Orozco

Optical atomic clocks$^{1,2}$ use electronic energy levels to precisely keep track of time. A clock based on nuclear energy levels promises a next-generation platform for precision metrology and fundamental physics studies. Thorium-229…

We use complementary optical spectroscopy methods to directly measure the lowest crystal-field energies of the rare-earth quantum magnet LiY$_{1-x}$Ho$_{x}$F$_{4}$, including their hyperfine splittings, with more than 10 times higher…

The operation of a frequency comb at extreme ultraviolet (XUV) wavelengths based on pair-wise amplification and nonlinear upconversion to the 15th harmonic of pulses from a frequency comb laser in the near-infrared range is reported.…

We report spectroscopic results of the \(X^2\Sigma^+(v=2) \rightarrow A^2\Pi_{1/2}(v=1)\) transition in magnesium monofluoride (MgF). Using Doppler-free Laser-Induced Fluorescence (LIF) spectroscopy on the \(X^2\Sigma^+(v=2) \rightarrow…

Atomic Physics · Physics 2026-04-01 Youngju Cho , Yongwoong Lee , Kikyeong Kwon , Seunghwan Roh , Giseok Lee , Eunmi Chae

Precision determination of the hyperfine splitting of cadmium ions is essential to study space-time variation of fundamental physical constants and isotope shifts. In this work, we present the precision frequency measurement of the…

Atomic Physics · Physics 2025-01-24 Ying Zheng , Yanmei Yu , Yiting Chen , Shengnan Miao , Wenxin Shi , Jianwei Zhang , Lijun Wang

In a frequency-modulation spectroscopy experiment, using the radiation from a single frequency diode laser, the spectra of molecular iodine hyperfine structure near 640 nm were recorded on the transition $B^3\Pi_{0_u^{+}}-X^1\Sigma^+_{g}$.…

The ground state hyperfine splitting in positronium, $\Delta _{\mathrm{HFS}}$, is sensitive to high order corrections of QED. A new calculation up to $O(\alpha ^3)$ has revealed a $3.9 \sigma$ discrepancy between the QED prediction and the…

High Energy Physics - Experiment · Physics 2014-11-20 A. Ishida , G. Akimoto , K. Kato , T. Suehara , T. Namba , S. Asai , T. Kobayashi , H. Saito , M. Yoshida , K. Tanaka , A. Yamamoto , I. Ogawa , S. Kobayashi , T. Idehara

We report on the first experimental results for microwave spectroscopy of the hyperfine structure of antiprotonic He-3. Due to the helium nuclear spin, antiprotonic He-3 has a more complex hyperfine structure than antiprotonic He-4 which…

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