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Hyperfine-encoded qubits in alkali atoms have established themselves as robust platforms for quantum computing, while alkaline-earth-like elements expand the state manipulation toolbox through their rich spectrum of optical transitions and…

Quantum Physics · Physics 2025-08-19 Denis Mishin , Dmitry Tregubov , Nikolay Kolachevsky , Artem Golovizin

We present a spectroscopic investigation of $^{169}\mathrm{Tm}^+$ that provides two key foundations for its use as a platform for advanced quantum applications. First, we establish the complete spectroscopic road map for optical cycling…

We have measured the frequency splitting between the $(2S, F=1/2)$ and $(2S, F=3/2)$ hyperfine sublevels in atomic deuterium by an optical differential method based on two-photon Doppler-free spectroscopy on a cold atomic beam. The result…

Atomic Physics · Physics 2009-11-10 N. Kolachevsky , P. Fendel , S. G. Karshenboim , T. W. Hänsch

Recently, the thulium atom was cooled down to the Bose-Einstein condensation temperature, thus opening a pathway to quantum simulation with this atom. However, successful simulations require instruments to control and readout states of the…

Over a two-year duration, we have compared the frequency of the 199Hg+ 5d106s 2S 1/2 (F=0)<-> 5d9 6s2 2D 5/2 (F=2) electric-quadrupole transition at 282 nm with the frequency of the ground-state hyperfine splitting in neutral 133Cs. These…

We report on the improved measurement of the hyperfine structure of $4f^{12}(^3 H_6)5d_{5/2}6s^2$ $(J=9/2)$ excited state in Tm-169 which is involved in the second-stage laser cooling of Tm. To measure the absolute value of the hyperfine…

We report precise measurement of the hyperfine splitting and calculation of the Zeeman coefficients of the $^{171}$Yb$^+$ ground state. The absolute hyperfine splitting frequency is measured using high-resolution laser-microwave…

Atomic Physics · Physics 2023-09-12 J. Z. Han , B. Q. Lu , N. C. Xin , Y. M. Yu , H. R. Qin , S. T. Chen , Y. Zheng , J. G. Li , J. W. Zhang , L. J. Wang

Using a newly developed laser-microwave-laser resonance method, we observed a pair of microwave transitions between hyperfine levels of the $(n,L)=(37,35)$ state of antiprotonic helium. This experiment confirms the quadruplet hyperfine…

An angle-resolved x-ray spectroscopic scheme is presented for determining the hyperfine splitting of highly charged ions. For helium-like ions, in particular, we propose to measure either the angular distribution or polarization of the…

Atomic Physics · Physics 2017-07-12 Z. W. Wu , A. V. Volotka , A. Surzhykov , S. Fritzsche

In this work we describe the latest results for the measurements of the hyperfine structure of antiprotonic helium-3. Two out of four measurable super-super-hyperfine SSHF transition lines of the (n,L)=(36,34) state of antiprotonic helium-3…

A two-step, two-color laser spectroscopy technique has been used to measure the hyperfine splitting of the 7p$_{1/2}$ excited state in $^{203}$Tl and $^{205}$Tl, as well as the isotope shift within the 7s$_{1/2}$ - 7p$_{1/2}$ transition.…

Atomic Physics · Physics 2015-06-17 G. Ranjit , D. Kealhofer , G. D. Vukasin , P. K. Majumder

In this study, we investigated the hyperfine structure of 43 spectral lines of atomic thulium. We analyzed Fourier-transform spectra in the wavelength range from 700 nm to 2250 nm, which corresponds to the wavenumber range from 14300 cm-1…

Hyperfine-structures of highly charged ions (HCIs) are favourable spectroscopic targets for exploring fundamental physics as well as nuclear properties. Recent proposals of HCI atomic clocks highlight their importance, especially for…

The study of highly charged electronic and muonic hydrogen-like ions, provides an intriguing way to probe the internal structure of their atomic nuclei. In this work, we use nuclear structure calculations to accurately calculate the…

The work to be described falls into three parts: (1) The computer-controlled CW spectrometer was designed to supplement the Manchester pulsed microwave spectrometer in situations where rapid nuclear relaxation makes spin-echo spectroscopy…

Condensed Matter · Physics 2007-05-23 Simeon Warner

Due to the low sensitivity of the thulium optical clock to black-body radiation and good accuracy and stability estimations, it appears to be one of the most promising transportable optical clocks. One of the leading systematic effects for…

We investigate the microwave spectra of ultracold alkali metal dimers in magnetic, electric and combined fields, taking account of the hyperfine structure due to the nuclear spins. We consider the molecules 41K87Rb and 7Li133Cs, which are…

Chemical Physics · Physics 2015-05-14 Hong Ran , J. Aldegunde , Jeremy M. Hutson

The hyperfine structures of the ground states in the ${}^{3}$He$^{2+} \mu^{-} e^{-}$ and ${}^{4}$He$^{2+} \mu^{-} e^{-}$ helium-muonic atoms are investigated with the use of highly accurate variational wave functions. The differences…

Quantum Physics · Physics 2015-06-04 Alexei M. Frolov

We have measured hyperfine structure in the first-excited $P$ state ($D$ lines) of all the naturally-occurring alkali atoms. We use high-resolution laser spectroscopy to resolve hyperfine transitions, and measure intervals by locking the…

Atomic Physics · Physics 2010-08-20 Dipankar Das , Vasant Natarajan

The absolute frequency measurement for all of the hyperfine transitions of 6P1/2 -> 7S1/2 using a self-referencing frequency comb is reported. This transition can be used as a bench marker for the accurate atomic wave function, and then…

Atomic Physics · Physics 2013-03-22 Tzu-Ling Chen , Isaac Fan , Chang-Yi Lin , Hsuan-Chen Chen , Shih-En Chen , Jow-Tsong Shy , Yi-Wei Liu
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