Related papers: Combined microwave and optical spectroscopy for hy…
Clocks based on cold atoms offer unbeatable accuracy and long-term stability, but their use in portable quantum technologies is hampered by a large physical footprint. Here, we use the compact optical layout of a grating magneto-optical…
The CREMA collaboration is pursuing a measurement of the ground-state hyperfine splitting (HFS) in muonic hydrogen ($\mu$p) with 1 ppm accuracy by means of pulsed laser spectroscopy. In the proposed experiment, the $\mu$p atom is excited by…
Optical frequency measurements of the intercombination line $(6s^{2})\,^{1}S_{0} -(6s6p)\,^{3}P_{1}$ in the isotopes of ytterbium are carried out with the use of sub-Doppler fluorescence spectroscopy on an atomic beam. A dispersive signal…
We measure the hyperfine structure of $nP_{1/2}$ Rydberg states using mm-wave spectroscopy on an ensemble of laser-cooled $^{85}$Rb atoms. Systematic uncertainties in our measurement from the Zeeman splittings induced by stray magnetic…
Vibrational sum frequency generation (SFG) spectroscopy is a powerful technique for investigating molecular structures, orientations, and dynamics at surfaces. However, its spatial resolution is fundamentally restricted to the micrometer…
An all-optical measurement of high-order fractional molecular echoes is demonstrated by using high-order harmonic generation (HHG). Excited by a pair of time-delayed short laser pulses, the signatures of full and high order fractional (1/2…
We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…
We demonstrate a technique to measure hyperfine structure using a frequency-stabilized diode laser and an acousto-optic modulator locked to the frequency difference between two hyperfine peaks. We use this technique to measure hyperfine…
We present a versatile confocal microscopy setup for optical second harmonic generation (SHG) and multi-photon spectroscopy that enables polarization-resolved studies of semiconductor bulk crystals and low-dimensional structures. The system…
Frequency metrology lies at the heart of precision measurement. Optical frequency combs provide a coherent link uniting the microwave and optical domains in the electromagnetic spectrum, with profound implications in timekeeping, sensing…
We excite spin-waves with spatially inhomogeneous pulses and study the resulting frequency shifts of a chip-scale atomic clock of trapped $^{87}$Rb. The density-dependent frequency shifts of the hyperfine transition simulate the s-wave…
Two-photon UV-photolysis of hydrogen sulfide molecules is applied to produce hydrogen molecules in highly excited vibrational levels in the \X\ electronic ground state, up to the dissociation energy and into the quasibound region.…
The recently demonstrated trapping and laser cooling of $^{133}$Ba$^+$ has opened the door to the use of this nearly ideal atom for quantum information processing. However, before high fidelity qubit operations can be performed, a number of…
We present a new independent evaluation of the hadronic and QCD contributions to the QED running coupling \alpha(M_Z) and to the muonium hyperfine splitting \nu. We obtain: \Delta\alpha_{had}=2770(17)10^{-5} and \Delta\nu_{had}=232.5(2.5)…
Attempts are made to unify gravity with the other three fundamental forces of nature. As suggested by higher dimensional models, this unification may require space and time variation of some dimensionless fundamental constants. In this…
We study ultranarrow $5s_{1/2}$ - $4f_{5/2}$ transitions in Nd$^{13+}$ and Sm$^{15+}$ and demonstrate that they lie in the optical region. The transitions are insensitive to external perturbations. At the same time they are sensitive to the…
We present a method for recovery of narrow homogeneous spectral features out of broad inhomogeneous overlapped profile based on second-derivative processing of the absorption spectra of alkali metal atomic vapor nanocells. The method is…
QED theory of the hyperfine splitting of the $1s$ and $2s$ state in hydrogen isotopes and helium-3 ion is considered. We develop an accurate theory of a specific difference 8E_{HFS}(2s)-E_{HFS}(1s). We take into account fourth order…
We present improved constraints on the coupling of ultralight bosonic dark matter to photons based on long-term measurements of two optical frequency ratios. In these optical clock comparisons, we relate the frequency of the ${}^2S_{1/2}…
Quantum state-resolved spectroscopy of the low energy thorium-229 nuclear transition was recently achieved. The five allowed transitions within the electric quadrupole structure were measured to the kilohertz level in a calcium fluoride…