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Transition metal compounds with the $(t_{2g})^4$ electronic configuration are expected to be nonmagnetic atomic singlets both in the weakly interacting regime due to spin-orbit coupling, as well as in the Coulomb dominated regime with…

Strongly Correlated Electrons · Physics 2017-01-16 Christopher Svoboda , Mohit Randeria , Nandini Trivedi

We theoretically propose a family of $f$-electron based magnets that realizes Kitaev-type bond-dependent anisotropic interactions. Based on {\it ab initio} calculations, we show that $A_2$PrO$_3$ ($A$: alkali metals) crystalize in a…

Strongly Correlated Electrons · Physics 2020-11-03 Seong-Hoon Jang , Ryoya Sano , Yasuyuki Kato , Yukitoshi Motome

Bond-dependent magnetic interactions, particularly those described by the Kitaev model, have emerged as a key pathway toward realizing unconventional magnetic states such as quantum spin liquids and topologically nontrivial excitations,…

The spin-chain compounds, Ca3CuIrO6 and Ca3CuRhO6, crystallizing in a K4CdCl6-derived monoclinic structure, are investigated by ac and dc magnetization, isothermal remnant magnetization as well as heat capacity measurements. The results…

Strongly Correlated Electrons · Physics 2009-11-10 S. Rayaprol , E. V. Sampathkumaran

The presence of spin-orbit coupling drives the anomalous magnetotransport at oxide interfaces and forms the basis for numerous intriguing properties of these 2D electron systems, such as topologically protected phases or anti-localization.…

Strongly Correlated Electrons · Physics 2018-02-28 Patrick Seiler , Jone Zabaleta , Robin Wanke , Jochen Mannhart , Thilo Kopp , Daniel Braak

The ruthenium halide $\alpha$-RuCl$_{3}$ is a promising candidate for a Kitaev spin liquid. However, the microscopic model describing $\alpha$-RuCl$_{3}$ is still debated partly because of a lack of analogue materials for…

Chiral spin liquids (CSLs) are time-reversal symmetry breaking ground states of frustrated quantum magnets that show no long-range magnetic ordering, but instead exhibit topological order and fractional excitations. Their realization in…

The moir\'e engineering of two-dimensional magnets opens unprecedented opportunities to design novel magnetic states with promises for spintronic device applications. The possibility of stabilizing skyrmions in these materials without…

Materials Science · Physics 2022-08-03 Doried Ghader , Bilal Jabakhanji , Alessandro Stroppa

Rare-earth chalcohalide REChX (RE = rare earth; Ch = O, S, Se, Te; X = F, Cl, Br, I) is a newly reported family of Kitaev spin liquid candidates. The family offers a platform where a strong spin-orbit coupling meets a van der Waals layered…

Strongly Correlated Electrons · Physics 2022-07-07 Zheng Zhang , Yanzhen Cai , Jing Kang , Zhongwen Ouyang , Zhitao Zhang , Anmin Zhang , Jianting Ji , Feng Jin , Qingming Zhang

Kitaev quantum spin liquids have attracted significant attention in condensed matter physics over the past decade. To understand their emergent quantum phenomena, high-quality single crystals of substantial size are essential. Here, we…

Strongly Correlated Electrons · Physics 2025-02-18 Bowen Zhang , Xiangjun Li , Limin Yan , Wenbo Li , Nana Li , Jianfa Zhao , Xiaobing Liu , Shun-Li Yu , Zhiwei Hu , Wenge Yang , Runze Yu

Heisenberg interactions are ubiquitous in magnetic materials and have been prevailing in modeling and designing quantum magnets. Bond-directional interactions offer a novel alternative to Heisenberg exchange and provide the building blocks…

We consider the exchange couplings present in an effective Hamiltonian of $\alpha$-RuCl$_3$, known as the K-$\Gamma$ model. This material has a honeycomb lattice, and is expected to be a representative of the Kitaev materials (which can…

Strongly Correlated Electrons · Physics 2022-04-19 Ipsita Mandal

The search for topological spin excitations in recently discovered two-dimensional (2D) van der Waals (vdW) magnetic materials is important because of their potential applications in dissipation-less spintronics. In the 2D vdW ferromagnetic…

Thermodynamic experiments as well as Raman scattering have been used to study the magnetic instabilities in the spin-tetrahedra systems Cu_2Te_2O_5X_2, X=Cl and Br. While the phase transition observed in the Cl system at T_o=18.2 K is…

Strongly Correlated Electrons · Physics 2009-11-07 P. Lemmens , K. -Y. Choi , E. E. Kaul , Ch. Geibel , K. Becker , W. Brenig , R. Valenti , C. Gros , M. Johnsson , P. Millet , F. Mila

Chiral magnetic states in two-dimensional (2D) layered noncentrosymmetric magnets, which are promising advanced spintronic materials, are usually attributed to Dzyaloshinskii-Moriya interactions (DMI). However, the role of underlying…

Materials Science · Physics 2024-03-19 Weiyi Pan , Changsong Xu , Xueyang Li , Zhiming Xu , Boyu Liu , Bing-Lin Gu , Wenhui Duan

The domain dynamics and spin-spin correlation of 2D ferromagnets Cr2X2Te6 (X=Si, Ge) are investigated by a composite magnetoelectric method. The magnetic field-temperature phase diagrams for both in-plane and out-of-plane magnetic fields…

Materials Science · Physics 2024-01-17 Yugang Zhang , Zefang Li , Jing Zhang , Long Zhang , Yonghong Li , Shuang Liu , Young Sun , Wenhong Wang , Yisheng Chai

Motivated by the recent wealth of exotic magnetic phases emerging in two-dimensional frustrated lattices, we investigate the origin of possible magnetism in the monolayer family of triangular lattice materials $MX_2$ ($M$={V, Mn, Ni},…

We investigate the chiral magnetic order in free-standing planar 3$d$-5$d$ bi-atomic metallic chains (3$d$: Fe, Co; 5$d$: Ir, Pt, Au) using first-principles calculations based on density functional theory. We found that the antisymmetric…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Vikas Kashid , Timo Schena , Bernd Zimmermann , Yuriy Mokrousov , Stefan Blügel , Vaishali Shah , H. G. Salunke

We employ density functional theory within a non-collinear framework to investigate the magnetic properties of the octanuclear molecular rings Cr$_8$ and V$_8$. Our aim is to generalize the evaluation of the effective magnetic interactions…

Materials Science · Physics 2026-04-28 Maria Barbara Maccioni , Elia Stocco , Luca Binci , Andrea Floris , Matteo Cococcioni

The Heisenberg-Kitaev (HK) model on the triangular lattice is conceptually interesting for its interplay of geometric and exchange frustration. HK models are also thought to capture the essential physics of the spin-orbital entanglement in…

Strongly Correlated Electrons · Physics 2015-04-29 Michael Becker , Maria Hermanns , Bela Bauer , Markus Garst , Simon Trebst
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