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The spin-orbit coupling (SOC) interactions, electron correlation effects and Hund coupling cooperate and compete with each other, leading to novel properties, quantum phase and non-trivial topological electronic behavior in iridium oxides.…

Strongly Correlated Electrons · Physics 2018-12-19 Xing Ming , Xiangang Wan , Carmine Autieri , Jianfeng Wen , Xiaojun Zheng

Motivated by the magnetic phase transition of a proximate Kitaev system $\alpha$-RuCl$_3$ in the presence of a magnetic field, we study the simplest but essential quantum spin model with the ferromagnetic nearest neighboring (NN) Kitaev…

Strongly Correlated Electrons · Physics 2020-10-14 Beom Hyun Kim , Shigetoshi Sota , Tomonori Shirakawa , Seiji Yunoki , Young-Woo Son

The bond-dependent Kitaev interaction $K$ is familiar in the effective spin model of transition metal compounds with octahedral ligands. In this work, we find a peculiar non-coplanar magnetic order can be formed with the help of $K$ and…

Strongly Correlated Electrons · Physics 2024-06-04 Linli Bai , Ken Chen

Honeycomb iridates such as $\gamma$-Li$_2$IrO$_3$ are argued to realize Kitaev spin-anisotropic magnetic exchange, along with Heisenberg and possibly other couplings. While systems with pure Kitaev interactions are candidates to realize a…

With octahedrally coordinated $t_{\rm 2g}$ orbitals which are active at filling $n=2$, the $\rm Sr_2CrO_4$ compound exhibits rich interplay of spin-orbital physics with tetragonal distortion induced crystal field tuning by external agent…

Strongly Correlated Electrons · Physics 2022-10-20 Shubhajyoti Mohapatra , Dheeraj Kumar Singh , Avinash Singh

Strong correlations, multiple lattice degrees of freedom, and the ease of doping make complex oxides a source of great research interest. Complex oxide heterointerfaces break inversion symmetry and can host a two dimensional carrier gas,…

Strongly Correlated Electrons · Physics 2018-08-15 V. V. Bal , Z. Huang , K. Han , Ariando , T. Venkatesan , V. Chandrasekhar

Proximity effects allow for the adjustment of magnetic properties in a physically elegant way. If two thin ferromagnetic (FM) films are brought into contact, electronic coupling alters their magnetic exchange interaction at their interface.…

The Kitaev model is a rare example of an analytically solvable and physically instantiable Hamiltonian yielding a topological quantum spin liquid ground state. Here we report signatures of Kitaev spin liquid physics in the honeycomb magnet…

Strongly Correlated Electrons · Physics 2021-01-04 Hector K. Vivanco , Benjamin A. Trump , Craig M. Brown , Tyrel M. McQueen

Recently H$_3$LiIr$_2$O$_6$ has been reported as a spin-orbital entangled quantum spin liquid (QSL) [K. Kitagawa et al., Nature {\bf 554}, 341 (2018)], albeit its connection to Kitaev QSL has not been yet identified. To unveil the related…

Strongly Correlated Electrons · Physics 2020-05-13 Shenghai Pei , Liang-Long Huang , Gaomin Li , Xiaobin Chen , Bin Xi , XinWei Wang , Youguo Shi , Dapeng Yu , Cai Liu , Le Wang , Fei Ye , Mingyuan Huang , Jia-Wei Mei

Quantum spin liquids (QSLs) represent exotic states of matter where quantum spins interact strongly yet evade long-range magnetic order down to absolute zero. Characterized by non-local quantum entanglement and resultant fractionalized…

Strongly Correlated Electrons · Physics 2025-12-05 Yuji Matsuda , Takasada Shibauchi , Hae-Young Kee

The honeycomb compound $\alpha$-RuCl$_3$ is widely discussed as a proximate Kitaev spin-liquid material. This scenario builds on spin-orbit entangled $j = 1/2$ moments arising for a $t_{2g}^5$ electron configuration with strong spin-orbit…

Strongly Correlated Electrons · Physics 2020-10-21 P. Warzanowski , N. Borgwardt , K. Hopfer , T. C. Koethe , P. Becker , V. Tsurkan , A Loidl , M. Hermanns , P. H. M. van Loosdrecht , M. Grüninger

The spin-orbit assisted Mott insulator $\alpha$-RuCl3 is proximate to the coveted quantum spin liquid (QSL) predicted by the Kitaev model. In the search for the pure Kitaev QSL, reducing the dimensionality of this frustrated magnet by…

The relation between crystal symmetries, electron correlations, and electronic structure steers the formation of a large array of unconventional phases of matter, including magneto-electric loop currents and chiral magnetism. Detection of…

X-ray magnetic circular dichroism spectroscopy has been used to characterize the electronic structure and magnetic moment of Cr$_2^+$. Our results indicate that the removal of a single electron from the $4s\sigma_g$ bonding orbital of…

We study the Ruderman-Kittel-Kasuya-Yosida interaction between magnetic impurities embedded in $p$-doped transition metal dichalcogenide triangular flakes. The role of underlying symmetries is exposed by analyzing the interaction as a…

Mesoscale and Nanoscale Physics · Physics 2016-12-26 Oscar Ávalos-Ovando , Diego Mastrogiuseppe , Sergio E. Ulloa

We investigate the fate of the Kitaev spin liquid (KSL) under the influence of an external magnetic field $h$ in the [001] direction and upon tuning bond anisotropy of the Kitaev coupling $K_z$ keeping $K_x = K_y = K$. Guided by density…

Strongly Correlated Electrons · Physics 2024-03-19 Shi Feng , Adhip Agarwala , Nandini Trivedi

Recently, great effort has been devoted to the search for two-dimensional (2D) ferromagnetic materials with inherent strong Dzyaloshinskii--Moriya interaction (DMI). Here, through a first-principles approach, we systematically investigate…

Materials Science · Physics 2022-09-14 Zhong Shen , Changsheng Song , Yufei Xue , Zebin Wu , Jiqing Wang , Zhicheng Zhong

The Kitaev spin liquid, a ground state of the bond-dependent Kitaev model in a honeycomb lattice has been a centre of attraction, since a microscopic theory to realize such an interaction in solid-state materials was discovered. A challenge…

Strongly Correlated Electrons · Physics 2022-05-20 Jiefu Cen , Hae-Young Kee

Including the orbital off-diagonal spin and charge condensates in the self consistent determination of magnetic order within a realistic three-orbital model for the $4d^4$ compound $\rm Ca_2 Ru O_4$, reveals a host of novel features…

Strongly Correlated Electrons · Physics 2021-07-05 Shubhajyoti Mohapatra , Avinash Singh

Quantum spin liquids can arise from Kitaev magnetic interactions, and exhibit fractionalized excitations with the potential for a topological form of quantum computation. This review surveys recent experimental and theoretical progress on…

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