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Two-dimensional (2D) transition metal dichalcogenides (TMDs) with tantalizing layer-dependent electronic and optical properties have emerged as a new paradigm for integrated flat opto-electronic devices. However, daunting challenges remain…

Chirality, a fundamental concept describing an object cannot superpose with its mirror image, is crucial in optics and photonics and leads to various exotic phenomena, such as circular dichroism, and optical activity. Recent findings reveal…

Optics · Physics 2025-01-13 Shijie Kang , Haitao Li , Jiayu Fan , Jiusi Yu , Boyang Qu , Peng Chen , Xiaoxiao Wu

Chirality arises from the asymmetry of matters, where two counterparts are the mirror image of each other. The interaction between circular-polarization light and quantum materials is enhanced in chiral space groups due to the structural…

Mesoscale and Nanoscale Physics · Physics 2023-09-13 Chang Niu , Shouyuan Huang , Neil Ghosh , Pukun Tan , Mingyi Wang , Wenzhuo Wu , Xianfan Xu , Peide D. Ye

Transition metal dichalcogenides are known to possess large optical nonlinearities and driving these materials at high intensities is desirable for many applications. Understanding their optical responses under repetitive intense excitation…

Two-dimensional (2D) compounds provide unique building blocks for novel layered devices and hybrid photonic structures. However, large surface-to-volume ratio in thin films enhances the significance of surface interactions and charging…

Recently, a series of two-dimensional (2D) nonmagnetic layered materials XSi2Y4 (X=transition metals; Y=pnictogens) having similar crystal structures with transition-metal dichalcogenides (TMDs) were proposed for their potential application…

Materials Science · Physics 2022-07-22 Tiantian Zhang , Shuichi Murakami

In the close vicinity of a chiral nanostructure, the circular dichroism of a biomolecule could be greatly enhanced, due to the interaction with the local superchiral fields. Modest enhancement of optical activity using a planar…

Structural defects in 2D-transition metal dichalcogenides are critical in modulating their optical and electrical behavior. Nevertheless, precise defect control within the monolayer regime poses a significant challenge. Herein, a…

Mesoscale and Nanoscale Physics · Physics 2025-09-30 Anagha Gopinath , Faiha Mujeeb , Subhabrata Dhar , Jyoti Mohanty

Conventional linear optical activity effects are widely used for studying chiral materials. However, poor contrast and artifacts due to sample anisotropy limit the applicability of these methods. Here we demonstrate that nonlinear…

Biological Physics · Physics 2016-02-16 Mei-Yu Chen , Mikko J. Huttunen , Che-Wei Kan , Yen-Yin Lin , Cin-Wei Ye , Meng-Jer Wu , Hsiang-Lin Liu , Shi-Wei Chu

The two-dimensional layer of molybdenum disulfide (MoS2) has recently attracted much interest due to its direct-gap property and potential applications in optoelectronics and energy harvesting. However, the synthetic approach to obtain high…

Recently developed circularly polarized X-ray light sources can probe ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism (TRCD)…

Chemical Physics · Physics 2017-02-08 Jérémy R. Rouxel , Markus Kowalewski , Shaul Mukamel

Chirality is probably the most mysterious among all symmetry transformations. Very readily broken in biological systems, it is practically absent in naturally occurring inorganic materials and is very challenging to create artificially.…

Chiral perovskites are emerging semiconducting materials with broken symmetry that can selectively absorb and emit circularly polarized light. However, most of the chiral perovskites are typically low-dimensional structures with limited…

Optical activity is the ability of chiral materials to rotate linearly-polarized (LP) electromagnetic waves. Because of their intrinsic asymmetry, traditional chiral molecules usually lack isotropic performance, or at best only possess a…

Optical chirality is central to many industrial photonic technologies including enantiomer identification, ellipsometry-based tomography and spin multiplexing in optical communication. However, a substantial chiral response requires a…

Optics · Physics 2018-07-11 Longqing Cong , Prakash Pitchappa , Nan Wang , Ranjan Singh

Transition metal dichalcogenides (TMDs) are emerging as promising two-dimensional (2d) semiconductors for optoelectronic and flexible devices. However, a microscopic explanation of their photophysics -- of pivotal importance for the…

We report polarization resolved photoluminescence from monolayer MoS2, a two-dimensional, non-centrosymmetric crystal with direct energy gaps at two different valleys in momentum space. The inherent chiral optical selectivity allows…

Materials Science · Physics 2012-08-10 G. Sallen , L. Bouet , X. Marie , G. Wang , C. R. Zhu , W. P. Han , Y. Lu , P. H. Tan , T. Amand , B. L. Liu , B. Urbaszek

Chiral superconductors, a unique class of unconventional superconductors in which the complex superconducting order parameter winds clockwise or counter-clockwise in the momentum space, represent a topologically non-trivial system with…

Monolayer transition metal dichalcogenides (TMDCs) are two-dimensional (2D) materials with many potential applications. Chemical vapour deposition (CVD) is a promising method to synthesize these materials. However, CVD-grown materials…

The light absorption and transmission of monolayer MoS$_{2}$ in a one-dimensional defective photonic crystal (d-1DPC) is theoretically investigated. The study shows that the strong interference effect decreases photon density in particular…