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In 2003 we have measured the absolute frequency of the $(1S, F=1, m_F=\pm 1) \leftrightarrow (2S, F'=1, m_F'=\pm 1)$ two-photon transition in atomic hydrogen. We observed a variation of $(-29\pm 57)$ Hz over a 44 months interval separating…

Improvements in atom-light coherence are foundational to progress in quantum information science, quantum optics, and precision metrology. Optical atomic clocks require local oscillators with exceptional optical coherence due to the…

We experimentally investigate an optical clock based on $^{171}$Yb ($I=1/2$) atoms confined in an optical lattice. We have evaluated all known frequency shifts to the clock transition, including a density-dependent collision shift, with a…

We present a new framework to study the time variation of fundamental constants in a model-independent way. Model independence implies more free parameters than assumed in previous studies. Using data from atomic clocks based on $^{87}$Sr,…

Optical lattice clocks are the prospective devices that can probe many subtle physics including temporal variation of the fine structure constant ($\alpha_e$). These studies necessitate high-precision measurements of atomic clock frequency…

Atomic Physics · Physics 2023-09-28 Zhi-Ming Tang , Yan-mei Yu , B. K. Sahoo , Chen-Zhong Dong , Yang Yang , Yaming Zou

A sharp resonance line that appears in three-photon transitions between the $^{1}S_{0}$ and $^{3}P_{0}$ states of alkaline earth and Yb atoms is proposed as an optical frequency standard. This proposal permits the use of the even isotopes,…

Optics · Physics 2007-05-23 Tao Hong , Claire Cramer , Warren Nagourney , E. N. Fortson

We have carried out calculations towards the goal of reducing the inaccuracy of the Sr optical atomic clock to 1$\times10^{-17}$ and below. We calculated a.c. polarizabilities of the $5s^2 ^1S_0$ and $5s5p ^3P_0^o$ clock states that are…

Atomic Physics · Physics 2010-04-29 S. G. Porsev , Andrew D. Ludlow , Martin M. Boyd , Jun Ye

We present a compact, long-term nearly continuous operation of a room-temperature Ca$^+$ optical clock setup towards a transportable clock, achieving an overall systematic uncertainty of $4.8\times 10^{-18}$ and an uptime rate of 97.8% over…

We report on the spectroscopy of radio-frequency transitions between nearly-degenerate, opposite-parity excited states in atomic dysprosium (Dy). Theoretical calculations predict that these states are very sensitive to variation of the…

Atomic Physics · Physics 2013-08-14 N. Leefer , C. T. M. Weber , A. Cingöz , J. R. Torgerson , D. Budker

A Wannier-Stark optical lattice clock has demonstrated unprecedented measurement precision for optical atomic clocks. We present a systematic evaluation of the lattice light shift, a necessary next step for establishing this system as an…

Atomic Physics · Physics 2023-03-29 Kyungtae Kim , Alexander Aeppli , Tobias Bothwell , Jun Ye

The exquisite control exhibited over quantum states of individual particles has revolutionized the field of precision measurement, as exemplified by the most accurate atomic clock realized in single trapped ions. Whereas many-atom lattice…

We have constructed an optical clock with a fractional frequency inaccuracy of 8.6e-18, based on quantum logic spectroscopy of an Al+ ion. A simultaneously trapped Mg+ ion serves to sympathetically laser-cool the Al+ ion and detect its…

Quantum Physics · Physics 2013-05-29 C. -W. Chou , D. B. Hume , J. C. J. Koelemeij , D. J. Wineland , T. Rosenband

State-resolved laser spectroscopy at the 10$^{-12}$ precision level recently reported in $arXiv$:2406.18719 determined the fractional change in nuclear quadrupole moment between the ground and isomeric state of $^{229}\rm{Th}$, $\Delta…

We report a single-ion optical atomic clock with fractional frequency uncertainty of $5.5\times10^{-19}$ and fractional frequency stability of $3.5 \times10^{-16}/\sqrt{\tau/\mathrm{s}}$, based on quantum logic spectroscopy of a single…

Accurate measurements of different transition frequencies between atomic levels of the electronic and hyperfine structure over time are used to investigate temporal variations of the fine structure constant $\alpha$ and the…

Atomic Physics · Physics 2014-12-01 N. Huntemann , B. Lipphardt , Chr. Tamm , V. Gerginov , S. Weyers , E. Peik

We describe an optical atomic clock based on quantum-logic spectroscopy of the $^1$S$_0$ $\leftrightarrow$ $^3$P$_0$ transition in $^{27}$Al$^{+}$ with a systematic uncertainty of ${9.4 \times 10^{-19}}$ and a frequency stability of…

A possibility for fundamental constants to vary in time is suggested by theories unifying gravity with other interactions. In this article we examine proposals to use optical transitions of Sr, Dy, YbII and YbIII for the search of the time…

Atomic Physics · Physics 2009-02-05 V. A. Dzuba , V. V. Flambaum , M. V. Marchenko.

We propose a novel class of atomic clocks based on highly charged ions. We consider highly-forbidden laser-accessible transitions within the $4f^{12}$ ground-state configurations of highly charged ions. Our evaluation of systematic effects…

Atomic Physics · Physics 2016-10-05 Andrei Derevianko , V. A. Dzuba , V. V. Flambaum

We investigate the leading systematic effects in ro-vibrational spectroscopy of the molecular hydrogen ions H2+ and HD+, in order to assess their potential for the realization of optical clocks that would be sensitive to possible variations…

Atomic Physics · Physics 2017-02-20 Jean-Philippe Karr

Appraising the projected $10^{-18}$ fractional uncertainty in the optical frequency standards using singly ionized ions, we estimate the black-body radiation (BBR) shifts due to the magnetic dipole (M1) and electric quadrupole (E2)…

Atomic Physics · Physics 2015-05-30 Bindiya Arora , D. K. Nandy , B. K. Sahoo