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We provide a theory of the deflection of polar and non-polar rotating molecules by inhomogeneous static electric field. Rainbow-like features in the angular distribution of the scattered molecules are analyzed in detail. Furthermore, we…

Chemical Physics · Physics 2015-05-20 E. Gershnabel , I. Sh. Averbukh

The recent demonstration of electron vortex beams has opened up the new possibility of studying orbital angular momentum (OAM) in the interaction between electron beams and matter. To this aim, methods to analyze the OAM of an electron beam…

Optics · Physics 2014-02-18 Giulio Guzzinati , Laura Clark , Armand Béché , Jo Verbeeck

Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…

Atomic Physics · Physics 2017-08-08 G. Z. Iwata , R. L. McNally , T. Zelevinsky

Supersonic beams of polar molecules are deflected using inhomogeneous electric fields. The quantum-state selectivity of the deflection is used to spatially separate molecules according to their quantum state. A detailed analysis of the…

We generate tightly focused optical vector beams whose electric fields spin around an axis transverse to the beams' propagation direction. We experimentally investigate these fields by exploiting the directional near-field interference of a…

Optics · Physics 2015-03-05 Martin Neugebauer , Thomas Bauer , Andrea Aiello , Peter Banzer

We study the angular deflection of the circular polarized components of a linearly polarized probe field in a weakly birefringent atomic system in tripod configuration. A spatially inhomogeneous control field incident obliquely onto an…

Quantum Physics · Physics 2016-12-06 Pardeep Kumar , Shubhrangshu Dasgupta

We present a comprehensive characterization of cold molecular beams from a cryogenic buffer-gas cell, providing an insight into the physics of buffer-gas cooling. Cold molecular beams are extracted from a cryogenic cell by electrostatic…

Chemical Physics · Physics 2018-12-04 X. Wu , T. Gantner , M. Zeppenfeld , S. Chervenkov , G. Rempe

We report high-precision measurements on the thallium fluoride $\tilde{J} = 1$ hyperfine manifold of the $B^3\Pi_1$ ($\nu = 0$) state. This state is of special interest because it is central to an optical cycling scheme that is envisioned…

We propose a filter method to generate electron beams of high polarization from bubble and blow-out wakefield accelerators. The mechanism is based on the idea to identify all electron-beam subsets with low-polarization and to filter them…

We construct an electron optical system to investigate Bragg diffraction (the crystal lattice plane, $10^{-2}$-$10^{-3}$ rad) with the objective lens turned off by adjusting the current in the intermediate lenses. A crossover was located on…

Materials Science · Physics 2019-11-06 Hiroshi Nakajima , Atsuhiro Kotani , Ken Harada , Shigeo Mori

The manipulation of the motion of neutral molecules with electric or magnetic fields has seen tremendous progress over the last decade. Recently, these techniques have been extended to the manipulation of large and complex molecules. In…

Chemical Physics · Physics 2011-04-07 Frank Filsinger , Gerard Meijer , Henrik Stapelfeldt , Henry N. Chapman , Jochen Küpper

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

The current best upper limit for electron electric dipole moment (EDM), $|d_e|<1.1\times10^{-29}\,$e$\cdot$cm ($90$% confidence), was set by the ACME collaboration in 2018. The ACME experiment uses a spin-precession measurement in a cold…

Molecular orientation techniques are becoming available in the study of elementary chemical processes, in order to highlight those structural and dynamical properties that would be concealed by random rotational motions. Recently successful…

Light-induced rotation of absorbing microscopic particles by transfer of angular momentum from light to the material raises the possibility of optically driven micromachines. The phenomenon has been observed using elliptically polarized…

Focusing optics for neutral molecules finds application in shaping and steering molecular beams. Here we present an electrostatic elliptical mirror for polar molecules consisting of an array of microstructured gold electrodes deposited on a…

In photoelectron spectroscopy, the measured electron momentum range is intrinsically related to the excitation photon energy. Low photon energies $<10$ eV are commonly encountered in laser-based photoemission and lead to a momentum range…

Fabricating an electrically switchable cylindrical Fresnel lens based on holographic polymer-dispersed liquid crystals (H-PDLC) using a Michelson interferometer is reported. Simplicity of the method and possibility of fabricating different…

Optics · Physics 2016-06-15 Hossein Jashnsaz , Ezeddin Mohajerani , Nahid Hosain Nataj

We employ heterodyne interferometry to investigate the effect of a single organic molecule on the phase of a propagating laser beam. We report on the first phase-contrast images of individual molecules and demonstrate a single-molecule…

Quantum Physics · Physics 2015-05-27 M. Pototschnig , Y. Chassagneux , J. Hwang , G. Zumofen , A. Renn , V. Sandoghdar

Stark deceleration enables the production of cold and dense molecular beams with applications in trapping, collisional studies, and precision measurement. Improving the efficiency of Stark deceleration, and hence the achievable molecular…

Chemical Physics · Physics 2020-07-22 David Reens , Hao Wu , Alexander Aeppli , Anna McAuliffe , Piotr Wcisło , Tim Langen , Jun Ye