English

Expanding the momentum field of view in angle-resolved photoemission systems with hemispherical analyzers

Instrumentation and Detectors 2021-12-17 v2 Materials Science Strongly Correlated Electrons

Abstract

In photoelectron spectroscopy, the measured electron momentum range is intrinsically related to the excitation photon energy. Low photon energies <10<10 eV are commonly encountered in laser-based photoemission and lead to a momentum range that is smaller than the Brillouin zones of most materials. This can become a limiting factor when studying condensed matter with laser-based photoemission. An additional restriction is introduced by widely used hemispherical analyzers that record only electrons photoemitted in a solid angle set by the aperture size at the analyzer entrance. Here, we present an upgrade to increase the effective solid angle that is measured with a hemispherical analyzer. We achieve this by accelerating the photoelectrons towards the analyzer with an electric field that is generated by a bias voltage on the sample. Our experimental geometry is comparable to a parallel plate capacitor and, therefore, we approximate the electric field to be uniform along the photoelectron trajectory. With this assumption, we developed an analytic, parameter-free model that relates the measured angles to the electron momenta in the solid and verify its validity by comparing with experimental results on the charge density wave material TbTe3_3. By providing a larger field of view in momentum space, our approach using a bias potential considerably expands the flexibility of laser-based photoemission setups.

Keywords

Cite

@article{arxiv.2108.08772,
  title  = {Expanding the momentum field of view in angle-resolved photoemission systems with hemispherical analyzers},
  author = {Nicolas Gauthier and Jonathan A. Sobota and Heike Pfau and Alexandre Gauthier and Hadas Soifer and Maja D. Bachmann and Ian R. Fisher and Zhi-Xun Shen and Patrick S. Kirchmann},
  journal= {arXiv preprint arXiv:2108.08772},
  year   = {2021}
}

Comments

11 pages, 7 figures