Related papers: Magneto-chiral nonlinear optical effect with large…
Monolayer transition metal dichalcogenides (TMDs) exhibit high nonlinear optical (NLO) susceptibilities. Experiments on MoS$_2$ have indeed revealed very large second-order ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) optical…
Nanophotonic chiral antennas exhibit orders of magnitude higher circular dichroism (CD) compared to molecular systems. Merging magnetism and structural chirality at the nanometric level allows for the efficient magnetic control of the…
To clarify the microscopic origin of chirality-induced optical effect, we develop an analytical method that extracts the chiral part of the Hamiltonian of molecular electronic states. We demonstrate this method in a model chiral molecule…
Ultrafast laser pulses provide unique tools to manipulate magnetization dynamics at femtosecond timescales, where the interaction of the electric field -- such as excitation of spin carriers to non-equilibrium states, generation of…
Nanoscopic observation of chiro-optical phenomena is essential in wide scientific areas but has measurement difficulties; hence, its physics are still unknown. Currently, in most cases, chiro-optical phenomena have been investigated by…
Chiral light-matter interactions can enable polarization to control the direction of light emission in a photonic device. Most realizations of chiral light-matter interactions require external magnetic fields to break time-reversal symmetry…
Controlling the spin degree of freedom of light at the microscale is crucial for advancing photonic information processing. Spin polarized light propagation, combined with strong optical nonlinearities, unlocks new functionalities in…
Photo-magnetic effects (PMEs), intrinsic to transition metals, arises from the interaction between light-induced angu-lar momentum and electronic spin. These effects are suppressed in noble metals with high symmetry and electron density.…
Coupling between light and material excitations underlies a wide range of optical phenomena. Polaritons are eigenstates of a coupled system with hybridized wave function. Owing to their hybrid composition, polaritons exhibit at the same…
We predict a non-thermal magneto-optical effect for magnetic insulators subject to intense light carrying orbital angular momentum (OAM). Using a classical approach to second harmonic generation in non-linear media with specific symmetry…
When circularly polarized light interacts with a nanostructure, the optical response depends on the geometry of the structure. If the nanostructure is chiral (i.e., it cannot be superimposed on its mirror image), then its optical response,…
High-harmonic generation (HHG) provides the only source of attosecond pulses -- currently the shortest accessible time intervals, and it is employed as the only table-top source of light in extreme UV and soft X-ray spectral regions. Chiral…
The nonlinear Hall effect is a new type of Hall effect that has recently attracted significant attention. For the physical origin of the nonlinear Hall effect, while orbital magnetization has long been hypothesized to underpin the nonlinear…
Conventional linear optical activity effects are widely used for studying chiral materials. However, poor contrast and artifacts due to sample anisotropy limit the applicability of these methods. Here we demonstrate that nonlinear…
Second-order nonlinearity gives rise to many distinctive physical phenomena, e.g., second-harmonic generation, which plays an important role in fundamental science and various applications. Lithium niobate, one of the most widely used…
Metasurfaces, the two-dimensional analogues of metamaterials, are ideal platforms for sensing molecular chirality at the nanoscale, e.g. of inclusions of natural optically active molecules, as they offer large accessible areas (they are…
Photons with spin angular momentum possess intrinsic chirality which underpins many phenomena including nonlinear optics1, quantum optics2, topological photonics3 and chiroptics4. Intrinsic chirality is weak in natural materials, and recent…
Optical activity is the ability of chiral materials to rotate linearly-polarized (LP) electromagnetic waves. Because of their intrinsic asymmetry, traditional chiral molecules usually lack isotropic performance, or at best only possess a…
Circularly polarized (CP) organic light-emitting diodes (OLEDs) have attracted attention in potential applications including novel display and photonic technologies. However, conventional approaches cannot meet the requirements of device…
Circular dichroism (CD), induced by chirality, is an important tool for manipulating light or for characterizing morphology of molecules, proteins, crystals and nano-structures. CD is manifested over a wide size-range, from molecules to…