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Light is one of the most powerful and precise tools allowing us to control, shape and create new phases of matter. In this task, the magnetic component of a light wave has so far played a unique role in defining the wave's helicity, but its…

Investigating chiral light-matter interactions is essential for advancing applications in sensing, imaging, and pharmaceutical development. However, the chiroptical response in natural chiral molecules and subwavelength chiral structures is…

Polarization-dependent photon spectroscopy (dichroism) of the second-harmonic generation (SHG) response is shown to reveal chiral and magnetic properties of a sample. Two dichroic signals are allowed with electric-dipole (E1) and…

Strongly Correlated Electrons · Physics 2019-12-11 S. W. Lovesey , G. van der Laan

Chirality is probably the most mysterious among all symmetry transformations. Very readily broken in biological systems, it is practically absent in naturally occurring inorganic materials and is very challenging to create artificially.…

Chiroptical techniques for detecting and characterizing the chirality of matter and artificial nanostructures are traditionally based on their interaction with chiral light, typically circularly-polarized fields propagating in free space.…

Halide perovskite semiconductors are a promising material for high-efficiency solar cells. Their optical properties can vary within and between crystallographic grains. We present spatially-resolved cathodoluminescence (CL) spectroscopy at…

The generation of high-order harmonics in a medium of chiral molecules driven by intense bi-elliptical laser fields can lead to strong chiroptical response in a broad range of harmonic numbers and ellipticities [D. Ayuso et al, J. Phys. B…

Optics · Physics 2018-07-04 David Ayuso , Piero Decleva , Serguei Patchkovskii , Olga Smirnova

In NiTe$_3$O$_6$ with a chiral crystal structure, we report on a giant natural optical rotation of the lowest-energy magnon. This polarization rotation, as large as 140 deg/mm, corresponds to a path difference between right and left…

2D organic-inorganic hybrid perovskites (2DHPs) consist of alternating anionic metal-halide and cationic organic layers. They have widely tunable structural and optical properties. We review the role of the organic cation in defining the…

Materials Science · Physics 2022-04-28 Daniel B. Straus , Cherie R. Kagan

Magneto-optical effect refers to a rotation of polarization plane, which has been widely studied in traditional ferromagnetic metal and insulator films and scarcely in two-dimensional layered materials. Here we uncover a new nonreciprocal…

Small organic molecules with a {\pi}-conjugated system that consists of only a few double or triple bonds can have significantly smaller optical excitation energies when equipped with donor- and acceptor groups, which raises the quantum…

Materials Science · Physics 2024-05-17 Ivan Biaggio

Hybrid-halide perovskite (HHP) films exhibit exceptional photo-electric properties. These materials are utilized for highly efficient solar cells and photoconductive technologies. Both ion migration and polarization have been proposed as…

Applied Physics · Physics 2021-04-21 Rohit Saraf , Cecile Saguy , Vivek Maheshwari , Hemaprabha Elangovan , Yachin Ivry

Strong-field methods in solids enable new strategies for ultrafast nonlinear spectroscopy and provide all-optical insights into the electronic properties of condensed matter in reciprocal and real space. Additionally, solid-state media…

Directional radiation and scattering play an essential role in light manipulation for various applications in integrated nanophotonics, antenna and metasurface designs, quantum optics, etc. The most elemental system with this property is…

Classical Physics · Physics 2023-06-21 Yuqiong Cheng , Kayode Adedotun Oyesina , Bo Xue , Dangyuan Lei , Alex M. H. Wong , Shubo Wang

Polar and chiral crystal symmetries confer a variety of potentially useful functionalities upon solids by coupling otherwise noninteracting mechanical, electronic, optical, and magnetic degrees of freedom. We describe two unstudied phases…

We study nonlinear response of a dimer composed of two identical Mie-resonant dielectric nanoparticles illuminated normally by a circularly polarized light. We develop a general theory describing hybridization of multipolar modes of the…

Gluon field configurations with nonzero topological charge generate chirality, inducing P- and CP-odd effects. When a magnetic field is applied to a system with nonzero chirality, an electromagnetic current is generated along the direction…

High Energy Physics - Phenomenology · Physics 2009-09-01 Dmitri E. Kharzeev , Harmen J. Warringa

Chirality, either of light or matter, has proved to be very practical in biosensing and nanophotonics. However, the fundamental understanding of its temporal dynamics still needs to be discovered. A realistic setup for this are the…

The optical properties of nanoparticle clusters vary with the spatial arrangement of the constituent particles, but also the overall orientation of the cluster with respect to the incident light. This is particularly important in the…

Optics · Physics 2021-11-02 Atefeh Fazel-Najafabadi , Baptiste Auguié

Fundamental and harmonic magneto-dielectricity studied for varied perovskite systems-- Pb0.98Gd0.02(Mg1/3Nb2/3)0.995O3 (A-site co-doped PGMN magneto-relaxor), La0.95Ca0.05CoO3 (A-site doped spin-state LCCO), and La2NiMnO6 (double-perovskite…

Materials Science · Physics 2020-04-22 Pooja Sahlot , Suchita Pandey , Adityanarayan Pandey , A. M. Awasthi