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As a step toward the full \emph{ab-initio} description of two-photon double ionization processes, we present a finite-pulse version of the virtual-sequential model for polyelectronic atoms. The model relies on the \emph{ab initio}…

Atomic Physics · Physics 2023-08-02 Siddhartha Chattopadhyay , Carlos Marante , Barry Schneider , Luca Argenti

We present an ab initio study of the nonsequential strong-field ionization dynamics of a model two-electron atom with helium character. Single- and double-ionization events are characterized and displayed using detector signals extracted at…

Atomic Physics · Physics 2023-06-14 Daniel Younis , Joseph H. Eberly

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

We develop an approximate model for the process of direct (nonsequential) two-photon double ionization of atoms. Employing the model, we calculate (generalized) total cross sections as well as energy-resolved differential cross sections of…

Quantum Physics · Physics 2016-08-17 Morten Førre , Sølve Selstø , Raymond Nepstad

We describe a numerical method that simulates the interaction of the helium atom with sequences of femtosecond and attosecond light pulses. The method, which is based on the close-coupling expansion of the electronic configuration space in…

Atomic Physics · Physics 2021-05-25 Luca Argenti , Eva Lindroth

Exchange correlation plays an important role in double-ionization of complex atoms by ultrashort laser pulse. In this work, we investigate two-photon double inner-shell electron ionization of neon induced by an attosecond extreme…

Atomic Physics · Physics 2019-06-05 Jianpeng Liu , Yongqiang Li , Jianmin Yuan

By using the B-spline numerical method, we investigate a two-photon double-ionization (TPDI) process of helium in a high-frequency laser field with its frequency ranging from 1.6~a.u. to 3.0~a.u. and the pulse duration ranging from 75 to…

Atomic Physics · Physics 2020-01-08 Fei Li , Facheng Jin , Yujun Yang , Jing Chen , Zong-Chao Yan , Xiaojun Liu , Bingbing Wang

Nonsequential double ionization (NSDI) of helium in an intense few-cycle laser pulse is investigated by applying the three-dimensional semi-classical re-scattering method. It is found that the momentum distribution of He$^{2+}$ shows a…

Atomic Physics · Physics 2015-05-13 Hongyun Li , J. Chen , Hongbing Jiang , Jie Liu , Panming Fu , Qihuang Gong , Zong-Chao Yan , Bingbing Wang

In this paper, we have investigated the correlated electron emission of the nonsequence double ionization (NSDI) in an intense linearly polarized field. The theoretical model we employed is the semiclassical rescattering model, the model…

Atomic Physics · Physics 2007-05-23 Li-Bin Fu , Jie Liu , Shi-Gang Chen

Owing to its numerical simplicity, a two-dimensional two-electron model atom, with each electron moving in one direction, is an ideal system to study non-perturbatively a fully correlated atom exposed to a laser field. Frequently made…

Atomic Physics · Physics 2009-10-30 D. Bauer

Recent experimental developments of high-intensity, short-pulse XUV light sources are enhancing our ability to study electron-electron correlations. We perform time-dependent calculations to investigate the so-called "sequential" regime…

Atomic Physics · Physics 2010-01-19 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We show that time ordering underlying time-dependent quantum dynamics is a physical observable accessible by attosecond streaking. We demonstrate the extraction of time ordering for the prototypical case of time-resolved two-photon double…

Atomic Physics · Physics 2015-03-06 Renate Pazourek , Stefan Nagele , Joachim Burgdörfer

Two XUV-photon double ionization of Ne, induced by an intense few-pulse attosecond train with a ~ 4 fs envelope duration is investigated experimentally and theoretically. The experiment is performed at ELI-ALPS utilizing the recently…

Few-photon induced breakup of helium is studied using a newly developed ab initio numerical framework for solving the six-dimensional time-dependent Schroedinger equation. We present details of the method and calculate (generalized) cross…

Atomic Physics · Physics 2010-06-11 R. Nepstad , T. Birkeland , M. Førre

Wave-particle duality is an inherent peculiarity of the quantum world. The double-slit experiment has been frequently used for understanding different aspects of this fundamental concept. The occurrence of interference rests on the lack of…

Electron-electron correlation effects play an instrumental role in our understanding of sequential (SDI) and non-sequential double ionization (NSDI) mechanisms. Here, we present a theoretical study of NSDI driven by plasmonic-enhanced…

Above 54.4 eV, two-photon double ionization of helium is dominated by a sequential absorption process, producing characteristic behavior in the single and triple differential cross sections. We show that the signature of this process is…

Atomic Physics · Physics 2009-11-13 D. A. Horner , T. N. Rescigno , C. W. McCurdy

The extension of coherent $\omega$-$2\omega$ control schemes, recently implemented in free-electron lasers (FELs), to molecular systems offers new opportunities to control chemical dynamics on the electronic timescale, potentially allowing…

We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT…

We present accurate time-dependent ab initio calculations on fully differential and total integrated (generalized) cross sections for the nonsequential two-photon double ionization of helium at photon energies from 40 to 54 eV. Our…

Atomic Physics · Physics 2008-05-07 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer
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