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Photoelectron spectroscopy is a powerful method that provides insight into the quantum mechanical properties of a wide range of systems. The ionized electron wavefunction carries information on the structure of the bound orbital, the ionic…

The concerted motion of two or more bound electrons governs atomic and molecular non-equilibrium processes and chemical reactions. It is thus a long-standing scientific dream to measure the dynamics of two bound correlated electrons in the…

With quantum calculations, we have investigated the multiphoton nonsequential double ionization of helium atoms in intense laser fields at ultraviolet wavelengths. Very surprisingly, we find a so-far unobserved double-circle structure in…

Atomic Physics · Physics 2014-01-06 Liao Qing , Zhou Yueming , Huang Cheng , Lu Peixiang

We analyze two-center interference effects in the yields of ionization of a dissociating hydrogen molecular ion by an ultrashort VUV laser pulse. To this end, we performed numerical simulations of the time-dependent Schr\"odinger equation…

Quantum Physics · Physics 2015-05-27 A. Picón , A. Bahabad , H. C. Kapteyn , M. M. Murnane , A. Becker

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

The strong coupling between two autoionizing states in helium is studied theoretically with the pump-probe scheme. An isolated 100-as XUV pulse is used to excite helium near the 2s2p(1P) resonance state in the presence of an intense…

Atomic Physics · Physics 2012-05-23 Wei-Chun Chu , Song-Feng Zhao , C. D. Lin

Multiphoton ionization provides a clear window into the nature of electron correlations in the helium atom. In the present study, the final state energy range extends up to the region near the $N=2$ and $N=3$ ionization thresholds, where…

Atomic Physics · Physics 2021-03-10 Yimeng Wang , Chris H. Greene

Strong-field ionization can induce electron motion in both the continuum and the valence shell of the parent ion. Here, we explore their interplay by studying laser-induced electron diffraction (LIED) patterns arising from interaction with…

We perform a systematic analysis of intra-channel quantum interference in laser-induced nonsequential double ionization with linearly polarized bichromatic fields, focusing on the recollision-excitation with subsequent ionization (RESI)…

Atomic Physics · Physics 2025-08-06 S. Hashim , D. Habibović , C. Figueira de Morisson Faria

The double-slit interference in single-photon ionization of the diatomic molecular ion $\mathrm{H}_2^+$ is theoretically studied beyond the dipole approximation. Via simulating and comparing the interactions of the prealigned…

Atomic Physics · Physics 2021-11-24 Kunlong Liu , Yibo Hu , Qingbin Zhang , Peixiang Lu

Phase-shift differences and amplitude ratios of the outgoing $s$ and $d$ continuum wave packets generated by two-photon ionization of helium atoms are determined from the photoelectron angular distributions obtained using velocity map…

A second plateau in the harmonic spectra of laser-driven two-electron atoms is observed both in the numerical solution of a low-dimensional model helium atom and using an extended strong field approximation. It is shown that the harmonics…

Atomic Physics · Physics 2009-11-13 P. Koval , F. Wilken , D. Bauer , C. H. Keitel

We present a systematic study of interchannel quantum interference in laser-induced nonsequential double ionization (NSDI) within the strong-field approximation. Focusing on the below-threshold intensity regime where the…

Atomic Physics · Physics 2026-03-17 S. Hashim , C. Figueira de Morisson Faria

We investigate single photon double ionization (PDI) of helium at photon energies of 440 and 800 eV. We observe doubly charged ions with close to zero momentum corresponding to electrons emitted back-to-back with equal energy. These slow…

We perform a systematic analysis of quantum interference in nonsequential double ionization focusing on the recollision-excitation with subsequent ionization (RESI) mechanism, employing the strong-field approximation (SFA). We find that…

Atomic Physics · Physics 2015-09-30 A. S. Maxwell , C. Figueira de Morisson Faria

We present total cross sections for single and double ionization of helium by antiproton impact over a wide range of impact energies from 10 keV/amu to 1 MeV/amu. A non-perturbative time-dependent close-coupling method (TDCC) is applied to…

Atomic Physics · Physics 2008-11-26 M. Foster , J. Colgan , M. S. Pindzola

We address the influence of the orbital symmetry and of the molecular alignment with respect to the laser-field polarization on laser-induced nonsequential double ionization of diatomic molecules, in the length and velocity gauges. We work…

Atomic Physics · Physics 2009-11-13 C. Figueira de Morisson Faria , T. Shaaran , X. Liu , W. Yang

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

The process of nonsequential two-photon double ionization of helium is studied by two complementary numerical approaches. First, the time-dependent Schr{\"o}dinger equation is solved and the final wave function is analyzed in terms of…

Quantum Physics · Physics 2010-09-13 Sølve Selstø , Tore Birkeland , Simen Kvaal , Raymond Nepstad , Morten Førre

Attosecond physics enables the study of ultrafast coherent electron dynamics in matter upon photoexcitation and photoionization, revealing spectacular effects such as hole migration and coherent Auger dynamics in molecules. In the…

Atomic Physics · Physics 2024-01-15 Marco Ruberti , Vitali Averbukh , Florian Mintert