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Two-photon double ionization of neon using an intense attosecond pulse train

Atomic Physics 2016-07-20 v1

Abstract

We present the first demonstration of two-photon double ionization of neon using an intense extreme ultraviolet (XUV) attosecond pulse train (APT) in a photon energy regime where both direct and sequential mechanisms are allowed. For an APT generated through high-order harmonic generation (HHG) in argon we achieve a total pulse energy close to 1 μ\muJ, a central energy of 35 eV and a total bandwidth of 30\sim30 eV. The APT is focused by broadband optics in a neon gas target to an intensity of 310123\cdot10^{12} W\cdotcm2^{-2}. By tuning the photon energy across the threshold for the sequential process the double ionization signal can be turned on and off, indicating that the two-photon double ionization predominantly occurs through a sequential process. The demonstrated performance opens up possibilities for future XUV-XUV pump-probe experiments with attosecond temporal resolution in a photon energy range where it is possible to unravel the dynamics behind direct vs. sequential double ionization and the associated electron correlation effects.

Keywords

Cite

@article{arxiv.1603.05439,
  title  = {Two-photon double ionization of neon using an intense attosecond pulse train},
  author = {B. Manschwetus and L. Rading and F. Campi and S. Maclot and H. Coudert-Alteirac and J. Lahl and H. Wikmark and P. Rudawski and C. M. Heyl and B. Farkas and T. Mohamed and A. L'Huillier and P. Johnsson},
  journal= {arXiv preprint arXiv:1603.05439},
  year   = {2016}
}