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The optical hybridization of the electronic states in strongly coupled molecule-cavity systems have revealed unique properties such as lasing, room temperature polariton condensation, and the modification of excited electronic landscapes…

In the last decade, much theoretical research has focused on studying the strong coupling between organic molecules (or quantum emitters, in general) and light modes. The description and prediction of polaritonic phenomena emerging in this…

Multilayer assemblies of metal nanoparticles can act as photonic structures, where collective plasmon resonances hybridize with cavity modes to create plasmon-polariton states. For sufficiently strong coupling, plasmon polaritons…

Hybrid structures formed between organic molecules and inorganic quantum dots can accomplish unique photophysical transformations by taking advantage of their disparate properties. The electronic coupling between these materials is…

We review both the fundamental aspects and the applications of functional magneto-optic and opto-magnetic metamaterials displaying collective and coupling effects on the nanoscale, where the concepts of optics and magnetism merge to produce…

Materials Science · Physics 2020-03-12 Nicolò Maccaferri

The coherent strong coupling of molecules with confined light fields to create polaritons - part matter, part light - is opening exciting opportunities ranging from extended exciton transport and inter-molecular energy transfer to modified…

Over the past decade, advances in super-resolution microscopy and particle-based modeling have driven an intense interest in investigating spatial heterogeneity at the level of single molecules in cells. Remarkably, it is becoming clear…

Molecular Networks · Quantitative Biology 2013-11-19 Andrew Mugler , Pieter Rein ten Wolde

When the coupling between light and matter becomes comparable to the energy gap between different excited states they hybridize, leading to the appearance of a rich and complex phenomenology which attracted remarkable interest in recent…

Transitions between solid-like and fluid-like states in living tissues have been found in steps of embryonic development and in stages of disease progression. Our current understanding of these transitions has been guided by experimental…

Soft Condensed Matter · Physics 2024-11-20 Steven J. Chisolm , Emily Guo , Vignesh Subramaniam , Kyle D. Schulze , Thomas E. Angelini

Coherence and correlations represent two related properties of a compound system. The system can be, for instance, the polarization of a photon, which forms part of a polarization-entangled two-photon state, or the spatial shape of a…

Quantum Physics · Physics 2015-12-01 Jiří Svozilík , Adam Vallés , Jan Peřina , Juan P. Torres

The ultrafast non-radiative relaxation of a molecular ensemble coupled to a cavity mode is considered theoretically and by real-time quantum dynamics. For equal coupling strength of single molecules to the cavity mode, the non-radiative…

Chemical Physics · Physics 2018-12-26 Oriol Vendrell

Strong light-matter interactions are gaining importance in controlling the photoswitching behavior of molecules exhibiting bistability. Here, we used the strategy of electronic strong coupling of both the E and Z-isomers of azopyrrole…

Small organic molecules with a {\pi}-conjugated system that consists of only a few double or triple bonds can have significantly smaller optical excitation energies when equipped with donor- and acceptor groups, which raises the quantum…

Materials Science · Physics 2024-05-17 Ivan Biaggio

Resonant dipole-dipole interaction modifies the energy and decay rate of electronic excitations for finite one dimensional chains of ultracold atoms in an optical lattice. We show that collective excited states of the atomic chain can be…

Quantum Physics · Physics 2012-12-07 Hashem Zoubi , Helmut Ritsch

Plasmonic nanocavities enable access to the quantum properties of matter, but are often simplified to single mode models despite their complex multimode structure. Here, we show that off-resonant plasmonic modes in fact play a crucial role…

Quantum Physics · Physics 2024-11-13 Angus Crookes , Ben Yuen , Angela Demetriadou

Strong coupling between molecules and quantized fields has emerged as an effective methodology to engineer molecular properties. New hybrid states are formed when molecules interact with quantized fields. Since the properties of these…

Chemical Physics · Physics 2023-06-28 Marco Romanelli , Rosario R. Riso , Tor S. Haugland , Enrico Ronca , Stefano Corni , Henrik Koch

We study the emergence of a collective optical response of a cold and dense $^{87}$Rb atomic cloud to a near-resonant low-intensity light when the atom number is gradually increased. Experimental observations are compared with microscopic…

In this article, we show that the collective light-matter strong coupling regime, where $N$ molecular emitters couple to the photon mode of an optical cavity, can be mapped to a quantum impurity model where the photon is the impurity that…

Quantum Physics · Physics 2023-10-25 Joel Yuen-Zhou , Arghadip Koner

This letter demonstrates the formation of vibro-polaritonic states by strong coupling gaseous nitrous oxide molecules at room temperature. The ro-vibrational features of the molecule is utilized to understand the nature of the strong…

Chemical Physics · Physics 2024-01-15 Akhila Kadyan , Jino George

Strong cavity coupling of gas-phase molecules will enable studies of benchmark chemical processes under strong light-matter interactions with a high level of experimental control and no solvent effects. We recently demonstrated the…

Chemical Physics · Physics 2023-10-26 Adam D. Wright , Jane C. Nelson , Marissa L. Weichman
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