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We investigate the process of circularly polarized high harmonic generation in molecules using a bicircular laser field. In this context, we show that molecules offer a very robust framework for the production of circularly polarized…

Atomic Physics · Physics 2016-06-22 F Mauger , A. D. Bandrauk , T Uzer

In equilibrium hard-rod fluids, and in effective hard-rod descriptions of anisotropic soft-particle systems, the transition from the isotropic (I) phase to the nematic phase (N) is observed above the rod aspect ratio L/D = 3.70 as predicted…

Soft Condensed Matter · Physics 2023-02-22 Jayeeta Chattopadhyay , Sriram Ramaswamy , Chandan Dasgupta , Prabal K. Maiti

Materials that exhibit high nonlinear optical (NLO) susceptibilities are considered as promising candidates for a wide range of photonic and electronic applications. Here we argue that the ferroelectric nematic (NF) materials have…

Soft Condensed Matter · Physics 2022-03-22 C. L. Folcia , J. Ortega , R. Vidal , T. Sierra , J. Etxebarria

High-order harmonic generation (HHG) in solids has entered a new phase of intensive research, with envisioned band-structure mapping on an ultrashort time scale. This partly benefits from a flurry of new HHG materials discovered, but so far…

Materials Science · Physics 2018-09-12 G. P. Zhang , M. S. Si , M. Murakami , Y. H. Bai , Thomas F. George

Deviations of molecular shapes from spherical symmetry may give rise to a variety of novel phenomena, including their dynamic behavior. It has recently been predicted [Mazza \textit{et al}. Phys. Rev. Lett. \textbf{105}, 227802 (2010)] that…

The below-threshold harmonic generation in the multiphoton ionization regime for a helium atom driven by the elliptically polarized laser field is studied numerically within the framework of two-dimensional (2D) and three-dimensional (3D)…

Optics · Physics 2024-12-11 Mikhail Yu. Emelin , Mikhail Yu. Ryabikin

A flux liquid can condense into a smectic crystal in a pure layered superconductor with the magnetic field oriented nearly parallel to the layers. Similar order can arise in low temperature $^4$He films with a highly anisotropic periodic…

Condensed Matter · Physics 2016-08-31 Leon Balents , David R. Nelson

The possible symmetries of the biaxial nematic phase are examined against the implications of the presently available experimental results. Contrary to the widespread notion that biaxial nematics have orthorhombic symmetry, our study shows…

Soft Condensed Matter · Physics 2010-04-15 Panagiota K. Karahaliou , Alexandros G. Vanakaras , Demetri J. Photinos

High-harmonic generation (HHG) in solids has been touted as a way to probe ultrafast dynamics and crystal symmetries in condensed matter systems. Here, we investigate the polarization properties of high-order harmonics generated in…

A theoretical study of the variation of thermodynamic and transport properties of calamitic liquid crystals across the isotropic-nematic phase transition is carried out by calculating the {\it wavenumber (k) and time (t)} dependent…

Soft Condensed Matter · Physics 2008-02-18 Prasanth P. Jose , Biman Bagchi

High-harmonic generation (HHG) in crystalline solids have been examined so far on the basis of one-body energy-band structures arising from electron itineracy in a periodic potential. Here, we show emergence of HHG signals which are…

Strongly Correlated Electrons · Physics 2020-04-22 Shohei Imai , Atsushi Ono , Sumio Ishihara

High-order harmonic generation (HHG) results from strong-field laser matter interaction and it is one of the main processes that are used to extract electron structural and dynamical information about the atomic or molecular targets with…

Using dynamic light scattering, we measure for the first time the temperature-dependent elastic moduli and associated orientational viscosity coefficients of the nematic phase in a self-assembled lyotropic chromonic liquid crystal. The bend…

Soft Condensed Matter · Physics 2008-07-18 Yu. A. Nastishin , K. Neupane , A. R. Baldwin , O. D. Lavrentovich , S. Sprunt

We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…

Nematic liquid crystals have been known for more than a century, but it was not until the 60s-70s that, with the development of room temperature nematics, they became widely used in applications. Polar nematic phases have been long-time…

Soft Condensed Matter · Physics 2021-08-17 Richard J. Mandle , Nerea Sebastián , Josu Martinez-Perdiguero , Alenka Mertelj

We analytically and numerically investigate the emission of high-harmonic radiation from model solids by intense few-cycle mid-infrared laser pulses. In single-active-electron approximation, we expand the active electron's wavefunction in a…

Other Condensed Matter · Physics 2019-07-26 Francisco Navarrete , Marcelo F. Ciappina , Uwe Thumm

Experimental and modeling/simulation studies of phase equilibrium and growth morphologies of novel polymer-dispersed liquid crystal (PDLC) mixtures of PS (polystyrene) and liquid crystals that exhibit a direct isotropic/smectic-A (lamellar)…

Soft Condensed Matter · Physics 2015-05-13 Ezequiel R. Soule , Nasser Mohieddin Abukhdeir , Alejandro D. Rey

High-harmonic generation (HHG) in solids has typically been explored in transparent dielectrics and semiconductors. Metals have long been dismissed due to their strong reflectivity at infrared wavelengths. Here, we demonstrate HHG from…

Ferroelectric nematic liquid crystals exhibit unique non-linear optical properties, with the potential to become transformative materials for photonic applications. A promising direction relies on the fabrication of tailored polar…

High-order harmonic generation (HHG) from aligned acetylene molecules interacting with mid infra-red (IR), linearly polarized laser pulses is studied theoretically using a mixed quantum-classical approach in which the electrons are…

Atomic Physics · Physics 2018-05-18 Peter Mulholland , Daniel Dundas
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